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Excitation hierarchy of the quantum sine-gordon spin chain in a strong magnetic field

Phys Rev Lett. 2004 Jul 9;93(2):027201. doi: 10.1103/PhysRevLett.93.027201. Epub 2004 Jul 6.

Abstract

The magnetic excitation spectrum of copper pyrimidine dinitrate, a material containing S = 1 / 2 antiferromagnetic chains with alternating g tensor and the Dzyaloshinskii-Moriya interaction and exhibiting a field-induced spin gap, is probed using submillimeter wave electron spin resonance spectroscopy. Ten excitation modes are resolved in the low-temperature spectrum, and their frequency-field diagram is systematically studied in magnetic fields up to 25 T. The experimental data are sufficiently detailed to make a very accurate comparison with predictions based on the quantum sine-Gordon field theory. Signatures of three breather branches and a soliton, as well as those of several multiparticle excitation modes, are identified.