Abstract
Current energy demand and environmental pollution issues are growing due to global urbanization and development in many countries, leading to amplified energy/material consumption, serious and irreparable damage to the ecosystem with simultaneous waste formation. The world energy demand is mainly accomplished by finite fossil fuel-based reserves, which have a crucial impact on the ecosystem/environment, and consequently, there is a need for a sustainable and/or low-carbon bioeconomy. Hydrogen (H2) generation from renewable biomass/waste is a promising bioenergy system that can generate low-carbon hydrogen and reduce GHG (greenhouse gas) emissions by 2050. Waste-to-biohydrogen (WtBH) can become a portion of the zero-emissions fuel replacement for natural gas and serve as one of the sustainable cleaner hydrogen sources which are environmentally friendly and economically feasible. In this view, bio-H2 is considered appropriate because of its high potential as a green, clean, and sustainable carbon-neutral energy source in the emerging low-carbon hydrogen bioeconomy. Nanostructured systems based on renewable biomass/waste sources depict a high potential to produce sustainable and low carbon biohydrogen economy because of their excellent physicochemical structures, such as high efficiency, high surface/volume ratio, non/low-toxicity, high chemical/mechanical stability, biodegradability/biocompatibility, availability, sustainability, cost-effectiveness, and unusual electrical/mechanical and magnetic properties. Renewable biomass and waste materials are extensively considered green sources to prepare greener and more sustainable sorts of mono- or bi-metallic nanomaterials using facile approaches. This review summarizes the deployment of thermochemical and biochemical approaches for WtBH using nanobiocatalysts towards a low-carbon bioeconomy.
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Abbreviations
- AC:
-
activated carbon
- Atm:
-
atmospheres
- BPS:
-
banana pseudo-stem
- Bio-MtH:
-
biomass to hydrogen
- CH4:
-
methane
- CNT:
-
carbon nanotube
- CO:
-
carbon monoxide
- CO2:
-
carbon dioxide
- DFT:
-
density functional theory
- EG:
-
ethylene glycol
- GHG:
-
greenhouse gas
- Gly:
-
glycerol
- GNS:
-
graphene nanosheet
- H2:
-
hydrogen
- HDPE:
-
high-density polyethylene
- HT:
-
hydrothermal
- IEA:
-
International Energy Agency
- IM:
-
impregnation
- LC:
-
life cycle
- LDPE:
-
low-density polyethylene
- MNP:
-
metal nanoparticle
- MSW:
-
municipal solid waste
- MW:
-
municipal wastewater
- MWCNT:
-
multi-walled carbon nanotube
- NP:
-
nanoparticle
- PAD:
-
photo-assisted deposition
- PE:
-
polyethylene
- PET:
-
polyethylene-terephthalate
- PP:
-
polypropylene
- QDs:
-
quantum dots
- ROS:
-
reactive oxygen species
- S/B :
-
steam to biomass ratio
- UV:
-
ultraviolet
- SCW:
-
supercritical water
- Vis:
-
visible
- VLI:
-
visible light irradiation
- WP:
-
waste plastic
- WtH:
-
waste-to-hydrogen
- WtBH:
-
waste-to-biohydrogen
- WWTP:
-
wastewater treatment plant
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Funding
This study received financial supports from Zhejiang Normal University (Grant No. YS304221928), Natural Science Foundation of Zhejiang Province (Nos. LD21E080001), and Zhejiang Provincial Ten Thousand Talent Program (ZJWR0302055).
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Karimi-Maleh, H., Orooji, Y., Karimi, F. et al. Integrated approaches for waste to biohydrogen using nanobiomediated towards low carbon bioeconomy. Adv Compos Hybrid Mater 6, 29 (2023). https://doi.org/10.1007/s42114-022-00597-x
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DOI: https://doi.org/10.1007/s42114-022-00597-x