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Precision spectroscopy of the 3s3p fine-structure doublet in Mg+

V. Batteiger, S. Knünz, M. Herrmann, G. Saathoff, H. A. Schüssler, B. Bernhardt, T. Wilken, R. Holzwarth, T. W. Hänsch, and Th. Udem
Phys. Rev. A 80, 022503 – Published 11 August 2009

Abstract

We apply a recently demonstrated method for precision spectroscopy on strong transitions in trapped ions to measure both fine-structure components of the 3s3p transition in M24g+ and M26g+. We deduce absolute frequency reference data for transition frequencies, isotope shifts, and fine-structure splittings that in particular are useful for comparison with quasar absorption spectra, which test possible space-time variations of the fine-structure constant. The measurement accuracy improves previous literature values, when existing, by more than two orders of magnitude.

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  • Received 26 June 2009

DOI:https://doi.org/10.1103/PhysRevA.80.022503

©2009 American Physical Society

Authors & Affiliations

V. Batteiger1, S. Knünz1, M. Herrmann1, G. Saathoff1, H. A. Schüssler2, B. Bernhardt1, T. Wilken1, R. Holzwarth1, T. W. Hänsch1,3, and Th. Udem1

  • 1Max-Planck-Institut für Quantenoptik, 85748 Garching, Germany
  • 2Department of Physics, Texas A&M University, College Station, Texas 77843, USA
  • 3Department of Physics, Ludwig-Maximilians-Universität München, 80539 München, Germany

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Vol. 80, Iss. 2 — August 2009

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Images

  • Figure 1
    Figure 1
    The Mg+ resonance doublet near 280 nm is isoelectronic to the 3s3p doublet in Na historically labeled as D1 and D2 Fraunhofer lines. From the D1 and the D2 transition frequencies measured in M24g+ and M26g+, we deduce isotope shifts and fine-structure splittings (FS). The measurement accuracy allowed us to resolve the isotope shift of the fine-structure splitting.Reuse & Permissions
  • Figure 2
    Figure 2
    (Color online) Spectroscopy technique [22]. A tightly focused laser beam cools an ion chain at one side only. A weaker spectroscopy beam is applied on axis to be insensitive to possible radial micromotion. An imaging photodetector together with software allows us to extract an essentially background free signal from a region-of-interest (ROI) around a single, sympathetically cooled ion.Reuse & Permissions
  • Figure 3
    Figure 3
    Wide scan across the M24g+ D1 resonance. Fluorescence photons were collected for 3s per data point; the scan was randomized in order. For our measurements we restricted the tuning range to 180 MHz around the line center. Inset: for comparison, we show an asymmetric M24g+ D2 line profile scanned from the low-frequency side; overlaid is a Voigt fit to the rising edge. Here the ion was essentially uncooled; only a weak cooling beam was superimposed to prevent ion loss during the scan time.Reuse & Permissions
  • Figure 4
    Figure 4
    (Color online) Schematic experimental setup. All involved lasers are phase locked (PLL) to a GPS disciplined hydrogen maser. The phase coherent link between the rf reference and the uv regime via a fiber laser frequency comb and a transfer diode laser is shown for the spectroscopy dye laser. The spectroscopy beam is intensity stabilized with an AOM and spatially filtered with a 15μm pinhole. A QWP rotates the polarization state of the spectroscopy beam. D2 cooling light is provided by a frequency quadrupled fiber laser [43]. An alternative setup generating both beams from a single laser output is shown in [22].Reuse & Permissions
  • Figure 5
    Figure 5
    (Color online) Measurement of two isotopic components of the D1 and the D2 transition. Outer dashed lines represent the error bar on the absolute transition frequencies due to correlated amplitude and phase modulation; inner dotted lines represent the reduced error bar for the relative determination of isotope shifts and fine-structure splittings. Squares indicate measurements with two-laser systems according to Fig. 4; circles indicate measurements with the double pass AOM scheme described together with the measurement of the M24g+ D2 component in [22].Reuse & Permissions
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