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Modeling huge photoinduced spin polarons in intrinsic magnetic semiconductors

S. C. P. van Kooten, X. Gratens, and A. B. Henriques
Phys. Rev. B 103, 035202 – Published 15 January 2021

Abstract

In intrinsic magnetic semiconductors, the absorption of a single photon can generate a spin polaron, whose magnetic moment reaches many thousands of Bohr magnetons. Here we investigate these huge photoinduced spin polarons, using Monte Carlo simulations. In antiferromagnetic semiconductors, photoinduced spin polarons are most efficiently generated in the whole temperature interval up to the phase transition, whereas in ferromagnetic semiconductors much larger spin polarons can be photoinduced, but only around the phase transition temperature. Because Monte Carlo simulations are computationally expensive, we developed an analytical model, based on Weiss field theory. Although the Weiss model does not provide as much information as a Monte Carlo simulation, such as spin texture and fluctuations, it yields formulas that can be used to estimate instantly the expected photoinduced spin polaron size in many intrinsic magnetic semiconductors.

  • Figure
  • Received 12 November 2020
  • Revised 10 December 2020
  • Accepted 23 December 2020

DOI:https://doi.org/10.1103/PhysRevB.103.035202

©2021 American Physical Society

Physics Subject Headings (PhySH)

Condensed Matter, Materials & Applied Physics

Authors & Affiliations

S. C. P. van Kooten, X. Gratens, and A. B. Henriques*

  • Instituto de Fisica, Universidade de Sao Paulo, 05315-970 Sao Paulo, Brazil

  • *andreh@if.usp.br

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Issue

Vol. 103, Iss. 3 — 15 January 2021

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Images

  • Figure 1
    Figure 1

    (a) Results of the Monte Carlo simulations. Experimental results for EuTe (squares), EuSe (circles), and EuS (triangles) are also shown, from Refs. [7], [1], and [2], respectively. The inset shows a contour plot of the spin polarization projection onto the spin of the photoexcited electron - assumed in direction [001] - in a plane going through the center of the spin polaron, in EuSe, at 6.2 K. The displacements are given in units of the lattice parameter. (b) Results of the Weiss field model.

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