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Beyond the freshman's dream: Classical fractal spin liquids from matrix cellular automata in three-dimensional lattice models

Sounak Biswas, Yves H. Kwan, and S. A. Parameswaran
Phys. Rev. B 105, 224410 – Published 21 June 2022

Abstract

We construct models hosting classical fractal spin liquids on two realistic three-dimensional (3D) lattices of corner-sharing triangles: trillium and hyperhyperkagome (HHK). Both models involve the same form of three-spin Ising interactions on triangular plaquettes as the Newman-Moore (NM) model on the 2D triangular lattice. However, in contrast to the NM model and its 3D generalizations, their degenerate ground states and low-lying excitations cannot be described in terms of scalar cellular automata (CA), because the corresponding fractal structures lack a simplifying algebraic property, often termed the “freshman's dream.” By identifying a link to matrix CAs—that makes essential use of the crystallographic structure—we show that both models exhibit fractal symmetries of a distinct class to the NM-type models. We devise a procedure to explicitly construct low-energy excitations consisting of finite sets of immobile defects or “fractons,” by flipping arbitrarily large self-similar subsets of spins, whose fractal dimensions we compute analytically. We show that these excitations are associated with energetic barriers which increase logarithmically with system size, leading to “fragile” glassy dynamics, whose existence we confirm via classical Monte Carlo simulations. We also discuss consequences for spontaneous fractal symmetry breaking when quantum fluctuations are introduced by a transverse magnetic field, and propose multispin correlation function diagnostics for such transitions. Our findings suggest that matrix CAs may provide a fruitful route to identifying fractal symmetries and fractonlike behavior in lattice models, with possible implications for the study of fracton topological order.

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  • Received 3 March 2022
  • Accepted 1 June 2022

DOI:https://doi.org/10.1103/PhysRevB.105.224410

©2022 American Physical Society

Physics Subject Headings (PhySH)

Condensed Matter, Materials & Applied PhysicsStatistical Physics & Thermodynamics

Authors & Affiliations

Sounak Biswas*, Yves H. Kwan*, and S. A. Parameswaran

  • Rudolf Peierls Centre for Theoretical Physics, Parks Road, Oxford OX1 3PU, United Kingdom

  • *These authors contributed equally to this work.

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Vol. 105, Iss. 22 — 1 June 2022

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Images

  • Figure 1
    Figure 1

    Annealing a 2n-sized three-fracton excitation (left) away by sequentially applying spin-flips which create 2n1-sized excitations requires an intermediate four-defect configuration. Yellow dots indicate fractons. Green shading represents the application of a Sierpinski triangle of spin flips.

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  • Figure 2
    Figure 2

    The lattice structure of trillium, with the four sublattices in the home unit cell labeled by α,β,γ,andδ. Grey balls indicate sites outside the home cell. One plaquette of each type is outlined in red.

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  • Figure 3
    Figure 3

    The cubic unit cell of HHK network of corner-sharing triangular plaquettes, with 12 sites in a unit cell. Each site is shared by three triangular plaquettes.

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  • Figure 4
    Figure 4

    The set of spins flipped to create an elementary fractonic cluster (EFC) for trillium is a fractal, with the fractons lying on the center and corners of a regular octahedron. (Left) Flipped spins in the upper half of the octahedron. The flipped spins on the faces of the octahedron resemble the Sierpinski triangle (red dots). (Right) Flipped spins in the plane containing the center and four vertices of the octahedron.

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  • Figure 5
    Figure 5

    For trillium, seven different EFCs of size 2n fuse to form a EFC of size 2n+1, i.e., an EFC of size 2n+1 can be created by flipping the spins corresponding to the creation of each of the seven smaller EFCs in series. For each of this excitations, all seven fractons are hosted by plaquettes of the same type. Fractons are denoted by solid red dots.

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  • Figure 6
    Figure 6

    For HHK, 6 EFCs of size 2n fuse to form an EFC of size 2n+1. A larger excitation can be created by flipping the spins corresponding to the creation of each of the six smaller excitations in series. In each of these excitations, fractons are hosted on two different kinds of plaquettes (3). The two kinds of fractons are denoted by the red and green dots.

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  • Figure 7
    Figure 7

    Relaxation of energy for annealing simulations in trillium. The temperature is cooled with as T=exp(γt). The measured value of energy stops tracking the analytical value of equilibrium energy, signaling a failure to reach equilibrium, at a temperature Tg(γ). Tg increases with γ—a signature of glassiness.

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  • Figure 8
    Figure 8

    Relaxation of energy for annealing simulations in HHK. The temperature is cooled with as T=exp(γt). Like trillium, the measured value of energy stops tracking the equilibrium energy at a cooling-rate dependent temperature Tg(γ), which increases with γ. While an exact solution of equilibrium energy is not available, we see that the energy obtained by calculation for a gas of free defects [Eq. (37)] agrees well with the energy obtained form a cluster Monte Carlo calculation.

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  • Figure 9
    Figure 9

    Time evolution of intensive energy E/N, for trillium. Like trillium, the plateaus correspond to different stages of the hierarchical dynamics. The different plateaus visible in the figure correspond to stages of the dynamics where higher energy excitations are being annealed away. The curves approximately collapse when plotted against Tln(t), as the mean defect spacing dmtT is the dominant length scale in the problem.

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  • Figure 10
    Figure 10

    Time evolution of intensive energy E/N, for HHK. The plateaus correspond to different stages of the hierarchical dynamics. Note that the different stages do not correspond to stages where EFCs of different sizes are annealed away, but are stages where excitations of higher energy (also fractonic) are annealed away. The curves approximately collapse when plotted against Tln(t), as the mean defect spacing dmtT is the dominant lengthscale in the problem.

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  • Figure 11
    Figure 11

    An inflation rule for D, the space-time diagram generated in the long-time evolution of the CA described by the transition matrix M [Eq. (12)] relevant to trillium. D is expressed as a superposition (mod2) of 5 copies of D which are smaller by a factor of 2, and 1 inverted copy, denoted by D̃, which is also smaller by a factor of 2.

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  • Figure 12
    Figure 12

    The decomposition of a pyramid of height 2 into six nonoverlapping pyramids of height 1. This decomposition is convenient for inflation rules, and is the pictorial representation of Eq. (A2).

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  • Figure 13
    Figure 13

    The total number of down spins in elementary fractonic clusters (EFCs) plotted against the linear size of such particles in a logarithmic scale, for both trillium and HHK.

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  • Figure 14
    Figure 14

    Graph showing the constraints leading to CA description of ground states. A node of the graph is labeled by the z coordinate and the sublattice index. A directed edge from nodes i and j to node k implies a three spin interaction sisjsk, such that the si and sj determine sk in the groundstate. Nodes are grouped into layers (shaded green regions); layers are the basic units on which the CA act: specifying the spin configuration on one layer fixes, via the CA rules, all layers succeeding and preceding it.

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