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Spin structure factor of the frustrated quantum magnet Cs2CuCl4

Denis Dalidovich, Rastko Sknepnek, A. John Berlinsky, Junhua Zhang, and Catherine Kallin
Phys. Rev. B 73, 184403 – Published 3 May 2006

Abstract

The ground state properties and neutron structure factor for the two-dimensional antiferromagnet on the triangular lattice, with unidirectional anisotropy in the nearest-neighbor exchange couplings and a weak Dzyaloshinskii-Moriya (DM) interaction, are studied. This Hamiltonian has been used to interpret neutron scattering measurements on the spin 12 spiral spin-density-wave system, Cs2CuCl4 [R. Coldea et al., Phys. Rev. B 68, 134424 (2003)]. Calculations are performed using a 1S expansion, taking into account interactions between spin waves. The ground state energy, the shift of the ordering wave vector, Q, and the local magnetization are all calculated to order 1S2. The neutron structure factor, obtained using anharmonic spin-wave Green's functions to order 1S, is shown to be in reasonable agreement with published neutron data, provided that slightly different parameters are used for the exchange and DM interactions than those inferred from measurements in high magnetic field.

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  • Received 20 January 2006

DOI:https://doi.org/10.1103/PhysRevB.73.184403

©2006 American Physical Society

Authors & Affiliations

Denis Dalidovich, Rastko Sknepnek, A. John Berlinsky, Junhua Zhang, and Catherine Kallin

  • Department of Physics and Astronomy, McMaster University, Hamilton, Ontario L8S 4M1, Canada

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Vol. 73, Iss. 18 — 1 May 2006

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Images

  • Figure 1
    Figure 1
    Exchange couplings between the different sites of the triangular lattice within a single layer.Reuse & Permissions
  • Figure 2
    Figure 2
    The total value of sublattice magnetization M, Eq. (54), calculated up to the second order in 1(2S) as a function of Dzyaloshinskii-Moriya interaction D, is shown by the solid line. The dashed, dotted and dashed-dotted lines are the results for the quantum corrections ΔM(1), ΔMI(2), and ΔMII(2), respectively, divided by S=12.Reuse & Permissions
  • Figure 3
    Figure 3
    (Color online) The two panels present the results for the bare and renormalized energy spectra for the cases of D=0 and D=0.02meV. Spin-wave energies are shown together with the inverse lifetime Γk. The path in the two-dimensional Brillouin zone sweeps from (00) point to (10). kx, ky are measured in units of 2π and 2π3 respectively.Reuse & Permissions
  • Figure 4
    Figure 4
    (Color online) Intensity of the scattered neutrons for scan G in Eq. (78), in the presence of Dzyaloshinskii-Moriya interaction D=0.02meV. The energy and momentum resolutions are taken to be Δω=0.016meV and Δk=0.085 respectively. The thick solid line is the total scattering intensity, Eq. (64). Other lines represent the various contributions appearing in Eqs. (67, 68, 69, 70, 71).Reuse & Permissions
  • Figure 5
    Figure 5
    (Color online) Intensity of the scattered neutrons corresponding to scan G, for the value of Dzyaloshinskii-Moriya interaction D=0.01meV. Upper panel: The total structure factor with the energy (momentum) resolution ΔE=0.016meV (Δk=0.085). Inset: Experimental data from Ref. 14. Lower panel: Different components which contribute to the structure factor [see Eqs. (67, 68, 69, 70, 71) in the text].Reuse & Permissions
  • Figure 6
    Figure 6
    (Color online) Intensity of the scattered neutrons corresponding to scan J, Eq. (78), in the presence of Dzyaloshinskii-Moriya interaction D=0.02meV. The different components are displayed as in Figs. 4, 5.Reuse & Permissions
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