Location via proxy:   [ UP ]  
[Report a bug]   [Manage cookies]                

Coherent versus incoherent light scattering from a quantum dot

K. Konthasinghe, J. Walker, M. Peiris, C. K. Shih, Y. Yu, M. F. Li, J. F. He, L. J. Wang, H. Q. Ni, Z. C. Niu, and A. Muller
Phys. Rev. B 85, 235315 – Published 19 June 2012

Abstract

We analyze the light scattered by a single InAs quantum dot interacting with a resonant continuous-wave laser. High-resolution spectra reveal clear distinctions between coherent and incoherent scattering, with the laser intensity spanning more than four orders of magnitude. We find that the fraction of coherently scattered photons can approach unity under sufficiently weak or detuned excitation, ruling out pure dephasing as a relevant decoherence mechanism. We show how spectral diffusion shapes spectra, correlation functions, and phase coherence, concealing the ideal radiatively broadened two-level system described by Mollow.

  • Figure
  • Figure
  • Figure
  • Figure
  • Received 2 April 2012

DOI:https://doi.org/10.1103/PhysRevB.85.235315

©2012 American Physical Society

Authors & Affiliations

K. Konthasinghe1, J. Walker1, M. Peiris1, C. K. Shih2, Y. Yu3, M. F. Li3, J. F. He3, L. J. Wang3, H. Q. Ni3, Z. C. Niu3, and A. Muller1,*

  • 1Department of Physics, University of South Florida, Tampa, Florida 33620, USA
  • 2University of Texas at Austin, Austin, Texas 78712, USA
  • 3Institute of Semiconductors, Chinese Academy of Sciences, Beijing 100083, P.R. China

  • *Corresponding author: mullera@usf.edu

Article Text (Subscription Required)

Click to Expand

References (Subscription Required)

Click to Expand
Issue

Vol. 85, Iss. 23 — 15 June 2012

Reuse & Permissions
Access Options
CHORUS

Article Available via CHORUS

Download Accepted Manuscript
Author publication services for translation and copyediting assistance advertisement

Authorization Required


×

Images

  • Figure 1
    Figure 1
    (a) Schematic of experimental setup. (b) QD emission spectrum, recorded with a grating spectrometer under resonant laser excitation as is [solid (black) trace], 20× magnified [dashed (gray) trace], and on a logarithmic scale [solid (red) trace] to visualize the phonon broadband. (c) QD excitation spectrum. (d) Spectrally integrated intensity of scattered light as a function of time showing flickering (dark blue trace) that is inhibited when an additional weak auxiliary laser is added (light green trace). The black trace was recorded with the auxiliary laser only.Reuse & Permissions
  • Figure 2
    Figure 2
    (a) Maps of scattered light intensity as a function of detection frequency (abscissas) and excitation frequency (ordinates) relative to the QD transition frequency, for three values of the Rabi frequency. Each panel was recorded in 200 s. At Ω/2π=0.13 GHz the detector count rate was 3×105 s1 at the input of the Fabry-Perot interferometer. Ddashed lines indicate the location of the eigenfrequencies of the coupled laser/QD system. Inset: The line section ν=ω together with the corresponding theoretical curve, obtained from Eq. (2). The faint diagonal lines parallel to the ν=ω section are due to the residual transmission at high-order modes of the Fabry-Perot interferometer and satellite modes of the laser. (b) Theoretical maps Eq. (2) corresponding to a radiatively broadened two-level system subject to spectral diffusion. (c) Theoretical maps Eq. (1) representing an ideal, radiatively broadened two-level system. (d) Theoretical maps Eq. (A11) representing a two-level system subject to radiative decay and to pure dephasing at a rate γ. γ is chosen so as to obtain the excitation linewidth in Fig. 1c.Reuse & Permissions
  • Figure 3
    Figure 3
    Power spectrum of light scattered by the QD at exact resonance (Δω=0) represented on a linear (left) and a logarithmic (right) ordinate scale, for a range of Rabi frequencies. Each spectrum was recorded in 60 s. The theoretical curve [dashed (red) line] was obtained by numerical evaluation of Eq. (2). The shaded (red) area corresponds to coherently scattered light, which dominates whenever Ωκ. If pure dephasing had a significant role in the scattering process, a broader feature would always be visible, even when Ωκ.Reuse & Permissions
  • Figure 4
    Figure 4
    (a) Photon statistics of scattered light for three Rabi frequencies. When Ω>κ, Rabi oscillations appear. (b) Plot of the total scattered light intensity [solid (red) trace] and the fraction of coherently scattered light intensity [dashed (red) trace], using the same parameters as in Fig. 3. For comparison the same, but not including spectral diffusion, are plotted in blue. (c) Same as (b), but with a laser detuned by Δω/2π=1 GHz. (d) Measurement of mutual phase coherence between the coherently scattered light and a local oscillator (LOSC) by interferometry. (e) Intensity of light at the output of the beam splitter in (d) as a function of the LOSC phase.Reuse & Permissions
×

Sign up to receive regular email alerts from Physical Review B

Log In

Cancel
×

Search


Article Lookup

Paste a citation or DOI

Enter a citation
×