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Infrared magnetospectroscopy of graphite in tilted fields

N. A. Goncharuk, L. Nádvorník, C. Faugeras, M. Orlita, and L. Smrčka
Phys. Rev. B 86, 155409 – Published 8 October 2012

Abstract

The electronic structure of Bernal-stacked graphite subjected to tilted magnetic fields has been investigated using infrared magnetotransmission experiments. With the increasing in-plane component of the magnetic field B, we observe significant broadening and partially also splitting of interband inter-Landau-level transitions, which originate at the H point of the graphite Brillouin zone, where the charge carriers behave as massless Dirac fermions. The observed behavior is attributed to the lifting of the twofold degeneracy of Landau levels at the H point—a degeneracy which in graphite complements the standard spin and valley degeneracies typical of graphene.

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  • Received 10 August 2012

DOI:https://doi.org/10.1103/PhysRevB.86.155409

©2012 American Physical Society

Authors & Affiliations

N. A. Goncharuk1,*, L. Nádvorník1,2, C. Faugeras3, M. Orlita2,3,†, and L. Smrčka1,‡

  • 1Institute of Physics, Academy of Science of the Czech Republic, v.v.i., Cukrovarnická 10, 162 53 Prague 6, Czech Republic
  • 2Charles University in Prague, Faculty of Mathematics and Physics, Ke Karlovu 3, 121 16 Praha 2, Czech Republic
  • 3Laboratoire National des Champs Magnétiques Intenses, CNRS-UJF-UPS-INSA, 25, avenue des Martyrs, 38042 Grenoble, France

  • *Present address: ABB s.r.o., Semiconductors, R&D, Novodvorská 1768/138a, 14221 Prague, Czech Republic.
  • orlita@karlov.mff.cuni.cz
  • smrcka@fzu.cz

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Issue

Vol. 86, Iss. 15 — 15 October 2012

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Images

  • Figure 1
    Figure 1
    Transmission of a thin graphite specimen measured at magnetic field tilted by ϕ=0,15, and 30 with respect to the c axis of graphite. Values nearby individual curves always denote the component of the magnetic field perpendicular to the graphite layer B. The missing parts of spectra correspond to regions in which the supporting tape is completely opaque. The energy axis for each curve is rescaled by a factor of B to facilitate identification of spectral features originating at the H point of graphite. Vertical lines correspond to positions of van Hove singularities in the joint density of states as calculated using the minimal nearest-neighbor tight-binding model.[43] Since the lifting of degeneracy exactly at the H point is governed by the coupling constants Tn,n+1Btan(ϕ), the positions of these van Hove singularities remain constant in these figures. For clarity, successive spectra in (a)–(c) are shifted vertically by 0.1.Reuse & Permissions
  • Figure 2
    Figure 2
    Relative magnetotransmission spectra for tilting angles ϕ=0,15,20,25,35, and 50 taken with the same perpendicular component of the field B=7 T. The broadening of the lines with increasing angle, i.e., with the increasing in-plane component of the field B, is well visible, e.g., on the C line, the width of which increases roughly linearly with B. A sample different from Fig. 1 has been used (with higher density of crystallites and their average thickness). For clarity, successive spectra are shifted vertically by 0.1.Reuse & Permissions
  • Figure 3
    Figure 3
    Landau sub-bands in the vicinity of the H points, kzd=π/2, at B= 5 T. The solid and dashed lines describe the kz dependence of energies Ene and Eno in even and odd graphene sheets at ϕ=0,15, and 30.Reuse & Permissions
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