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Chiral spin liquid and quantum criticality in extended S=12 Heisenberg models on the triangular lattice

Alexander Wietek and Andreas M. Läuchli
Phys. Rev. B 95, 035141 – Published 24 January 2017
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Abstract

We investigate the J1J2 Heisenberg model on the triangular lattice with an additional scalar chirality term and show that a chiral spin liquid is stabilized in a sizable region of the phase diagram. This topological phase is situated in between a coplanar 120 Néel ordered and a noncoplanar tetrahedrally ordered phase. Furthermore we discuss the nature of the spin-disordered intermediate phase in the J1J2 model. We compare the ground states from exact diagonalization with a Dirac spin liquid wave function and propose a scenario where this wave function describes the quantum critical point between the 120 magnetically ordered phase and a putative Z2 spin liquid.

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  • Received 10 June 2016
  • Revised 21 December 2016

DOI:https://doi.org/10.1103/PhysRevB.95.035141

©2017 American Physical Society

Physics Subject Headings (PhySH)

  1. Research Areas
Condensed Matter, Materials & Applied Physics

Authors & Affiliations

Alexander Wietek* and Andreas M. Läuchli

  • Institut für Theoretische Physik, Universität Innsbruck, A-6020 Innsbruck, Austria

  • *alexander.wietek@uibk.ac.at

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Issue

Vol. 95, Iss. 3 — 15 January 2017

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Images

  • Figure 1
    Figure 1

    Approximate T=0 phase diagram of the J1J2Jχ model on the triangular lattice, cf. Eq. (1). The extent of phases is inferred from excitation spectra from ED on a periodic 36-site triangular simulation cluster; see main text for details. Orange: S=1 K.A1 (120 Néel); light blue: S=0 Γ.E2b (CSL); green: S=0 Γ.E2a, Γ.E2b degenerate (Dirac/Z2 spin liquid); dark blue: S=0 Γ.A1, Γ.E2a, Γ.E2b degenerate (stripy magnetic order); dark red / light red: S=1 M.A / S=0 Γ.E2a (tetrahedral magnetic order).

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  • Figure 2
    Figure 2

    Order parameters and variational energies of model wave functions. Left: static spin structure factor S(q). evaluated at K and M point. Middle: nematic order parameter N as in Eq. (2) and (disconnected) scalar chirality correlation X as in Eq. (3). Right: Variational energies ε=(EmodelEED)/EED for the chiral and Dirac spin liquid.

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  • Figure 3
    Figure 3

    Excitation spectra of the model (1) from ED for Jχ=0.24 and overlaps with the two CSL wave functions on a 36-site cluster. Full (empty) symbols denote even (odd) spin levels; different types of symbols denote different space-group representations. The numbers denote the summed overlaps OGWEDα as in Eq. (4). We find overlaps up to 0.92.

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  • Figure 4
    Figure 4

    ED spectra for Jχ=0 and spectral decomposition of several model wave functions for J2=0.12 and J2=0.15. Full (empty) symbols correspond to even (odd) spin. The diameter of the poles is proportional to the square overlap |ψED|ψModel|2. Besides the CSL and Dirac spin liquid wave functions the three wave functions denoted by Γ.A1, Γ.A2, and Γ.E2b are the ground states in the respective symmetry sectors at J2=0.3.

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  • Figure 5
    Figure 5

    Overlaps of DSL wave function with ED eigenstates and decay of spin-spin and twist-twist correlation functions (S0×S1)·(Si×Sj) of the DSL from VMC on a 144-site lattice. The maximum ground-state overlap is attained at J2=0.1. The correlations decay algebraically over distance.

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