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Structure of As83, As85, and As87: From semimagicity to γ softness

K. Rezynkina et al.
Phys. Rev. C 106, 014320 – Published 29 July 2022

Abstract

The structure of As83, As85, and As87 have been studied in fusion-fission reaction U238+Be9. Fission fragments were identified in mass and atomic number using the VAMOS++ spectrometer and the coincident γ rays were detected in the γ-ray tracking array AGATA. New transitions in As83 and As85 are reported and placed in the level schemes. A level scheme of the excited states in As87 is proposed for the first time. The data are interpreted in frame of large-scale shell-model calculations, SU3 symmetries, and beyond mean-field frameworks. A spherical regime at magic number N=50 is predicted and the location of the proton g9/2 orbital is proposed for the first time. Development of collectivity in a prolate deformed, γ-soft regime in the open shell cases As85 and As87, most neutron-rich isotopes beyond N=50, is concluded. Data and theoretical calculations give confidence to a relatively high extrapolated excitation energy about 4 MeV of the 9/2+ state in Cu79, one proton above Ni78.

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  • Received 18 March 2022
  • Accepted 27 June 2022

DOI:https://doi.org/10.1103/PhysRevC.106.014320

©2022 American Physical Society

Physics Subject Headings (PhySH)

Nuclear Physics

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Vol. 106, Iss. 1 — July 2022

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Images

  • Figure 1
    Figure 1

    Tracked γ-ray spectrum in coincidence with As83 ions identified in VAMOS++. (♥) As83 transitions reported for the first time in this work; () As83 transitions previously observed in Refs. [12, 13, 14, 15]; () As82 contaminant transitions; and () As84 contaminant transitions.

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  • Figure 2
    Figure 2

    Left: Partial level scheme of As83, containing the transitions observed in this work. The transitions indicated in color are new. The transitions marked in green eventually decay to the 1542.6- and 1865.6-keV levels. The transitions marked in blue follow other paths. Right: LSSM predictions with the DF2882 interaction.

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  • Figure 3
    Figure 3

    (a) Tracked γ-ray spectrum in coincidence with As83 ions identified in VAMOS++. Enlargement of the region near 320 keV. The 317.2-keV transition is highlighted in green. The weak 313.2(1)-keV line is a contaminant from As84 (see text for details); (b) background-subtracted gate on 317.2-keV transition in As83 [as highlighted in panel (a)].

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  • Figure 4
    Figure 4

    Background-subtracted tracked γ-ray spectrum in coincidence with the As83 ions identified in VAMOS, gated on the 2466-keV γ-ray line.

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  • Figure 5
    Figure 5

    Tracked γ-ray spectrum in coincidence with As85 ions identified in VAMOS++. (♥) As85 transitions reported for the first time in this work; () As85 transitions previously observed in [28]; and () As84 contaminant transitions.

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  • Figure 6
    Figure 6

    Left: Partial level scheme of As85, established in this work. Right: Level scheme predicted by the LSSM calculations.

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  • Figure 7
    Figure 7

    (a) Tracked γ-ray spectrum region seen in coincidence with As85 identified in VAMOS++, fitted with three Gaussian components, (b) background-subtracted gate on the 793.6-keV transition, and (c) background-subtracted gate on the 796.6-keV transition.

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  • Figure 8
    Figure 8

    Tracked γ-ray spectrum in coincidence with As87 ions identified in VAMOS++. (♥) As87 transitions reported for the first time in this work; () Se87 contaminant transitions; and () As86 contaminant transitions.

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  • Figure 9
    Figure 9

    Tracked γ-ray spectrum observed in coincidence with the isotopically identified As87 and the 997.3-keV γ-ray.

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  • Figure 10
    Figure 10

    Left: Level scheme of As87, established in this work. Right: Predictions from the LSSM calculations.

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  • Figure 11
    Figure 11

    Excitation energy of the 9/2+ states in As (Z=33), Br (Z=35), Rb (Z=37), and Y (Z=39) isotopes. The solid lines represent experimental values from Refs. [29, 30, 31, 33] and the tentative assignments from this work. The dashed lines represent the predictions of the LSSM calculations.

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  • Figure 12
    Figure 12

    Valence mirror symmetry in N=50 isotones (top) and Z=28 isotopes (bottom).

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  • Figure 13
    Figure 13

    Zuker-Retamosa-Poves diagrams for the pseudo-SU3 proton orbitals (left) and neutron orbitals (right) limits in the case of As.87

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  • Figure 14
    Figure 14

    Potential energy surface (PES) calculated for As85 with the treatment of odd-mass nuclei by means of a cranking method following Ref. [39]. The cranked component corresponds to that of the HF minimum Ĵz=3/2. The yellow diamond symbol represents the HF minimum.

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  • Figure 15
    Figure 15

    PES for As87 obtained with the same method as in Fig. 14.

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  • Figure 16
    Figure 16

    DNO-SM calculations for As85, using 45 deformed HF states (see more details in Ref. [40]).

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  • Figure 17
    Figure 17

    DNO-SM calculations for As87, using 50 deformed HF states (see more details in Ref. [40]).

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  • Figure 18
    Figure 18

    Wave functions content in K-quantum numbers of As85. For the various states Pα(J)(K) (normalized to unity) is the contribution of a component K in the given state Jα.

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  • Figure 19
    Figure 19

    Same analysis in K-quantum numbers of As87 states as in Fig. 18.

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  • Figure 20
    Figure 20

    Structure of considered states in deformations (β,γ) of As87. The radius of circles represents the normalized probability to find a deformation (β,γ) in the corresponding state.

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