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Quantum Order by Disorder and Accidental Soft Mode in Er2Ti2O7

M. E. Zhitomirsky, M. V. Gvozdikova, P. C. W. Holdsworth, and R. Moessner
Phys. Rev. Lett. 109, 077204 – Published 16 August 2012

Abstract

Motivated by recent neutron scattering experiments, we derive and study an effective “pseudodipolar” spin-1/2 model for the XY pyrochlore antiferromagnet Er2Ti2O7. While a bond-dependent in-plane exchange anisotropy removes any continuous symmetry, it does lead to a one-parameter ‘accidental’ classical degeneracy. This degeneracy is lifted by quantum fluctuations in favor of the noncoplanar spin structure observed experimentally—a rare experimental instance of quantum order by disorder. A non-Goldstone low-energy mode is present in the excitation spectrum in accordance with inelastic neutron scattering data. Our theory also resolves the puzzle of the experimentally observed continuous ordering transition, absent from previous models.

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  • Received 2 April 2012

DOI:https://doi.org/10.1103/PhysRevLett.109.077204

© 2012 American Physical Society

Authors & Affiliations

M. E. Zhitomirsky1, M. V. Gvozdikova1, P. C. W. Holdsworth2, and R. Moessner3

  • 1Service de Physique Statistique, Magnétisme et Supraconductivité, UMR-E9001 CEA-INAC/UJF, 17 rue des Martyrs, 38054 Grenoble Cedex 9, France
  • 2Laboratoire de Physique, École Normale Supérieure de Lyon, CNRS 69364 Lyon Cedex 07, France
  • 3Max-Planck-Institut für Physik komplexer Systeme, 01187 Dresden, Germany

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Issue

Vol. 109, Iss. 7 — 17 August 2012

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Images

  • Figure 1
    Figure 1
    Possible q=0 spin structures of the XY pyrochlore antiferromagnet in zero applied field: ψ2 state (a) and ψ3 state (b).Reuse & Permissions
  • Figure 2
    Figure 2
    Inset: the ground-state energy in units of J for degenerate classical configurations parameterized by the angle φ; see Eq. (4). Main panel: the quantum spin reduction in the noncoplanar state ψ2 versus the bond-dependent exchange anisotropy parameter ja=Ja/J.Reuse & Permissions
  • Figure 3
    Figure 3
    Zero-field dispersion of magnons in Er2Ti2O7 along the [100] direction. Wave vectors are measured in units of 2π. Solid lines are calculated for J=0.28meV and ja=1, while dashed lines are for J=0.33meV and ja=0.5. Open squares are experimental data points [14].Reuse & Permissions
  • Figure 4
    Figure 4
    Main panel: temperature dependence of the sublattice magnetization for the classical XY pyrochlore antiferromagnet with in-plane anisotropic exchange on periodic cluster with L=12. Inset: the fourth-order Binder cumulant for several lattice sizes at fixed ja=0.5.Reuse & Permissions
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