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Chirality in Magnetic Multilayers Probed by the Symmetry and the Amplitude of Dichroism in X-Ray Resonant Magnetic Scattering

Jean-Yves Chauleau, William Legrand, Nicolas Reyren, Davide Maccariello, Sophie Collin, Horia Popescu, Karim Bouzehouane, Vincent Cros, Nicolas Jaouen, and Albert Fert
Phys. Rev. Lett. 120, 037202 – Published 18 January 2018

Abstract

Chirality in condensed matter has recently become a topic of the utmost importance because of its significant role in the understanding and mastering of a large variety of new fundamental physical mechanisms. Versatile experimental approaches, capable to reveal easily the exact winding of order parameters, are therefore essential. Here we report x-ray resonant magnetic scattering as a straightforward tool to reveal directly the properties of chiral magnetic systems. We show that it can straightforwardly and unambiguously determine the main characteristics of chiral magnetic distributions: i.e., its chiral nature, the quantitative winding sense (clockwise or counterclockwise), and its type, i.e., Néel [cycloidal] or Bloch [helical]. This method is model independent, does not require a priori knowledge of the magnetic parameters, and can be applied to any system with magnetic domains ranging from a few nanometers (wavelength limited) to several microns. By using prototypical multilayers with tailored magnetic chiralities driven by spin-orbit-related effects at Co|Pt interfaces, we illustrate the strength of this method.

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  • Received 22 September 2017

DOI:https://doi.org/10.1103/PhysRevLett.120.037202

© 2018 American Physical Society

Physics Subject Headings (PhySH)

Condensed Matter, Materials & Applied Physics

Authors & Affiliations

Jean-Yves Chauleau1,2,*, William Legrand2, Nicolas Reyren2, Davide Maccariello2, Sophie Collin2, Horia Popescu1, Karim Bouzehouane2, Vincent Cros2,†, Nicolas Jaouen1, and Albert Fert2

  • 1Synchrotron SOLEIL, L’Orme des Merisiers, 91192 Gif-sur-Yvette, France
  • 2Unité Mixte de Physique, CNRS, Thales, Université Paris-Sud, Université Paris-Saclay, 91767 Palaiseau, France

  • *Corresponding author. Jean-Yves.Chauleau@cea.fr
  • Corresponding author. vincent.cros@cnrs-thales.fr

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Issue

Vol. 120, Iss. 3 — 19 January 2018

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Images

  • Figure 1
    Figure 1

    (a) XRMS measurement principle and experimental configuration. (b) 6×6μm2 MFM phase image showing the out-of-plane magnetic contrast of the [Ir(1)|Co(0.6)|Pt(1)]×5 multilayer with its corresponding FFT pattern (inset) evidencing a 180±30nm period disordered magnetic stripe pattern. Corresponding diffracted patterns for a CL (c) and CR (d) polarized incident x-ray beam. (e) Resulting sum image of the diffracted pattern (CL+CR), confirming that the diffraction corresponds to the magnetic domains observed by MFM. (f) Normalized difference image (CLCR/CL+CR) evidencing a pronounced magnetic asymmetry. Note that the straight black area crossing the diffraction ring is the shadow of a beamstop used to block the specular reflection.

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  • Figure 2
    Figure 2

    (a) Diagram of a Bloch (helicoidal) winding and of a (b) Néel (cycloidal) winding. (c) Calculated orthoradial profile of the circular dichroism of different magnetic textures: CW (orange) and CCW (green) Bloch (dashed) and Néel (solid) windings for an incident angle θ=17.5°. (d) Comparison with the experimental magnetic asymmetry orthoradial profile of a [Ir(1)|Co(0.8)|Pt(1)]×5 multilayer for the same incident angle θ=17.5° (dots). Note that the red rectangles indicate the position of the beamstop.

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  • Figure 3
    Figure 3

    Comparison of two samples with inverted stacking [Ir(1)|Co(0.8)|Pt(1)]×5 (a)–(c) and [Pt(1)|Co(0.8)|Ir(1)]×5 (d),(e). The corresponding magnetization textures are obtained by micromagnetic simulations based on material parameters (a),(d). (b),(e) MFM images with labyrinth-shape domains and their Fourier transform in the inset. (c),(f) Normalized magnetic asymmetry signal (ICLICR)/(ICL+ICR) measured on sample a (e) and sample b (f). The diffraction sum images are shown in the inset, confirming again that the diffraction corresponds to the magnetic domains.

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