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Emergent Edge Modes in Shifted Quasi-One-Dimensional Charge Density Waves

Song-Bo Zhang, Xiaoxiong Liu, Md Shafayat Hossain, Jia-Xin Yin, M. Zahid Hasan, and Titus Neupert
Phys. Rev. Lett. 130, 106203 – Published 8 March 2023
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Abstract

We propose and study a two-dimensional phase of shifted charge density waves (CDW), which is constructed from an array of weakly coupled 1D CDW wires whose phases shift from one wire to the next. We show that the fully gapped bulk CDW has topological properties, characterized by a nonzero Chern number, that imply edge modes within the bulk gap. Remarkably, these edge modes exhibit spectral pseudoflow as a function of position along the edge, and are thus dual to the chiral edge modes of Chern insulators with their spectral flow in momentum space. Furthermore, we show that the CDW edge modes are stable against interwire coupling. Our predictions can be tested experimentally in quasi-1D CDW compounds such as Ta2Se8I.

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  • Received 12 April 2022
  • Revised 5 November 2022
  • Accepted 10 February 2023

DOI:https://doi.org/10.1103/PhysRevLett.130.106203

© 2023 American Physical Society

Physics Subject Headings (PhySH)

Condensed Matter, Materials & Applied Physics

Authors & Affiliations

Song-Bo Zhang1,*, Xiaoxiong Liu1, Md Shafayat Hossain2, Jia-Xin Yin3, M. Zahid Hasan2,4,5,6, and Titus Neupert1,†

  • 1Department of Physics, University of Zürich, Winterthurerstrasse 190, 8057, Zürich, Switzerland
  • 2Laboratory for Topological Quantum Matter and Advanced Spectroscopy (B7), Department of Physics, Princeton University, Princeton, New Jersey 08540, USA
  • 3Department of physics, Southern University of Science and Technology, Shenzhen, Guangdong 518055, China
  • 4Princeton Institute for the Science and Technology of Materials, Princeton University, Princeton, New Jersey 08540, USA
  • 5Materials Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, California 94720, USA
  • 6Quantum Science Center, Oak Ridge, Tennessee 37831, USA

  • *songbo.zhang@physik.uzh.ch
  • neupert@physik.uzh.ch

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Issue

Vol. 130, Iss. 10 — 10 March 2023

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Images

  • Figure 1
    Figure 1

    Duality between the coupled SLLs (left) and shifted CDWs (right). (a) Schematic of the coupled SLLs. It leads to a Chern insulator. The dashed lines separate areas with unit magnetic flux Φ0. (b) Chiral edge modes (red) with energies in the bulk gap (black) of the Chern insulator, which exhibit spectral flow as a function of momentum kx along the edge. (c) Chiral edge modes in position space, which are translation invariant along the edge. (d) Schematic of the shifted CDW. The phases of the wires shift with the x position, as depicted by the varying background color. (e) CDW edge modes with energies inside the bulk CDW gap, which are dispersion-free in kx. (f) CDW edge modes in position space, which exhibit spectral pseudoflow as a function of x along the edge.

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  • Figure 2
    Figure 2

    (a) Band structure of a CDW wire with PBC. (b) Band structure as a function of ϕ at ky=π/(4λy). There are two CDW gaps of size V and characterized by Chern numbers ±2. (c) LDOS near the upper gap. Edge modes with energies controllable by ϕ appear in the gap. Parameters: Ly=85, ϕ0=0.6π, EF=tysin(π/λy), and kBT=0.03V in (c).

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  • Figure 3
    Figure 3

    (a)–(c) Energy spectra for tx=0, 0.3ty, and 0.8ty, respectively. The bulk continuum and edge discrete spectra are indicated by gray and red color, respectively. PBC (OBC) are imposed in the x(y) direction. (d),(e) LDOS for tx=0 and 0.3ty, respectively. (f) ΔCDW (thick lines) and one edge bandwidths δEedge (circle lines) as functions of tx. We consider λx=10 (blue), 15 (orange), and 21 (green) for illustration. (g) tc as a function of λx for V=0.2, 0.3, and 0.5 eV, respectively. Ly=421 and ϕ=0 in all panels, λx=21 and Lx=10λx in (d),(e), and other parameters are the same as Fig. 2.

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  • Figure 4
    Figure 4

    (a) Low-energy band structure (orange) of the model (4) without CDW. Gray curves are first-principle calculations of Ta2Se8I. (b) Band structure with the CDW potential. Two CDW gaps, characterized by Chern numbers ±8, appear at low energies. (c) LDOS near the upper gap as a function of x¯ (in units of a˜) along the edge. Other parameters: V=0.3eV, EF=0.25eV, kBT=0.01V, Lx=216a˜ and Lz=114c.

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