Magnetochiral tunneling in paramagnetic Co1/3NbS2

S Lim, S Singh, FT Huang, S Pan… - Proceedings of the …, 2024 - National Acad Sciences
S Lim, S Singh, FT Huang, S Pan, K Wang, J Kim, J Kim, D Vanderbilt, SW Cheong
Proceedings of the National Academy of Sciences, 2024National Acad Sciences
Electric currents have the intriguing ability to induce magnetization in nonmagnetic crystals
with sufficiently low crystallographic symmetry. Some associated phenomena include the
non-linear anomalous Hall effect in polar crystals and the nonreciprocal directional
dichroism in chiral crystals when magnetic fields are applied. In this work, we demonstrate
that the same underlying physics is also manifested in the electronic tunneling process
between the surface of a nonmagnetic chiral material and a magnetized scanning probe. In …
Electric currents have the intriguing ability to induce magnetization in nonmagnetic crystals with sufficiently low crystallographic symmetry. Some associated phenomena include the non-linear anomalous Hall effect in polar crystals and the nonreciprocal directional dichroism in chiral crystals when magnetic fields are applied. In this work, we demonstrate that the same underlying physics is also manifested in the electronic tunneling process between the surface of a nonmagnetic chiral material and a magnetized scanning probe. In the paramagnetic but chiral metallic compound Co1/3NbS2, the magnetization induced by the tunneling current is shown to become detectable by its coupling to the magnetization of the tip itself. This results in a contrast across different chiral domains, achieving atomic-scale spatial resolution of structural chirality. To support the proposed mechanism, we used first-principles theory to compute the chirality-dependent current-induced magnetization and Berry curvature in the bulk of the material. Our demonstration of this magnetochiral tunneling effect opens up an avenue for investigating atomic-scale variations in the local crystallographic symmetry and electronic structure across the structural domain boundaries of low-symmetry nonmagnetic crystals.
National Acad Sciences