Mark Weiser predicted in 1991 that computing would lead to individuals interacting with countless computing devices, seamlessly integrating them into their daily lives until they disappear into the background [42]. However, achieving this seamless integration while addressing the associated environmental concerns is challenging. Trillions of smart devices with varied capabilities and form-factor are needed to build a networked environment of this magnitude. Yet, conventional computing paradigms require plastic housings, PCB boards, and rare-earth minerals, coupled with hazardous waste, and challenging reclamation and recycling, leading to significant e-waste. The current linear lifecycle design of electronic devices does not allow circulation among different life stages, neglecting features like recyclability and repairability during the design process. In this position paper, we present the concept of computational materials designed for transiency as a substitute for current devices. We envision that not all devices must be designed with performance, robustness, or even longevity as the sole goal. We detail computer systems challenges to the circular economy of computational materials and provide strategies and sketches of tools to assess a device's entire lifetime environmental impact.