Abstract
Results of investigations of structural and magnetic properties of Fe/Cr/Gd superlattices that differ in the thicknesses of the Cr interlayer have been reported. The insertion of the Cr interlayer between Gd and Fe layers has been found to lead to structural changes in Gd layers and the appearance of an additional fcc phase in them along with the main hcp phase. The new fcc phase is uniformly distributed across the thickness of the layer and is not localized near layer boundaries or in the center of Gd layers. Polarized-neutron reflectometry was used to show that the aforementioned structural changes are accompanied by a substantial (two-fold to threefold) decrease in the average magnetization of gadolinium over a wide temperature range. Near interfaces of the Gd layer, a layer appears that is two-to-three monatomic layers thick and characterized by increased magnetic moment.
Similar content being viewed by others
References
C. F. Majkrzak, J. Kwo, M. Yjng, Y. Yafet, D. Gibbs, C. L. Chen, and J. Bohr, “Magnetic rare earth superlattices,” Adv. Phys. 40, 99–189 (1991).
Ultrathin Magnetic Structures, Ed. by B. Heinrich and J. A. C. Bland (Springer-Verlag, Berlin, 2005), Vols. I–IV.
D. Haskel, G. Srajer, J. C. Lang, J. Pollmann, C. S. Nelson, J. S. Jiang, and S. D. Bader, “Enhanced interfacial magnetic coupling of Gd/Fe multilayers,” Phys. Rev. Lett. 87, 207201 (2001).
E. Kravtsov, D. Haskel, S. G. E. te Velthuis, J. S. Jiang, and B. J. Kirby, “Complementary polarized neutron and resonant X-ray magnetic reflectometry measurements in Fe/Gd heterostructures: Case of inhomogeneous intralayer magnetic structure,” Phys. Rev. B: Condens. Matter Mater. Phys. 79, 134438 (2009).
B. Sanyal, C. Antoniak, T. Burkert, B. Krumme, A. Warland, F. Stromberg, Ch. Praetorius, K. Fauth, H. Wende, and O. Eriksson, “Forcing ferromagnetic coupling between rare-earth-metal and 3d ferromagnetic films,” Phys. Rev. Lett. 104, 156402 (2010).
A. B. Drovosekov, N. M. Kreines, A. O. Savitskii, E. A. Kravtsov, D. V. Blagodatkov, M. V. Ryabukhina, M. A. Milyaev, V. V. Ustinov, E. M. Pashaev, I. A. Subbotin, and G. V. Prutskov, “Interlayer coupling in Fe/Cr/Gd multilayer structures,” J. Exp. Theor. Phys. 120, 1041–1054 (2015).
M. V. Ryabukhina, E. A. Kravtsov, D. V. Blagodatkov, L. I. Naumova, V. V. Proglyado, V. V. Ustinov, and Yu. Khaydukov, “Polarized neutron reflectometry of Fe/Cr/Gd superlattices,” J. Surf. Invest.: X-ray, Synchr. Neutr. Techn. 8, 983–986 (2014).
M. V. Ryabukhina, E. A. Kravtsov, D. V. Blagodatkov, L. I. Naumova, Yu. V. Nikitenko, V. V. Proglyado, and Yu. Khaidukov, “Magnetism of Fe/Cr/Gd superlattices,” J. Surf. Invest.: X-ray, Synchr. Neutr. Techn. 9, 41–43 (2015).
C. Ward, G. Scheunert, W. R. Hendren, R. Hardeman, M. A. Gubbins, and R. M. Bowman, “Realizing a high magnetic moment in Gd/Cr/FeCo: The role of the rare earth,” Appl. Phys. Lett. 102, 092403 (2013).
G. Scheunert, W. R. Hendren, C. Ward, and R. M. Bowman, “Magnetization of 2.6 T in Gadolinium Thin Films,” Appl. Phys. Lett 101, 142407 (2012).
G. Scheunert, C. Ward, W. R. Hendren, A. A. Lapicki, R. Hardeman, M. Mooney, M. A. Gubbins, and R. M. Bowman, “Influence of strain and polycrystalline ordering on magnetic properties of high moment rare earth metals and alloys,” J. Phys. D: Appl. Phys. 47, 415005 (2014).
I. N. Yakovkin, Komesu. Takashi, and P. A. Dowben, “Band structure of strained Gd (0001) films,” Phys. Rev. B: Condens. Matter Mater. Phys. 66, 035406 (2002).
T. Komesu, C. Waldfried, and P. A. Dowben, “The origin of enhanced magnetization in strained gadolinium,” Phys. Lett. A 256, 81–87 (1999).
H. F. Kirby, D. D. Belyea, J. T. Willman, and C. W. Miller, “Effects of preparation conditions on the magnetocaloric properties of Gd thin films,” J. Vac. Sci. Technol., A 31, 031506 (2013).
F. Stromberg, C. Antoniak, U. von Horsten, W. Keune, B. Sanyal, O. Eriksson, and H. Wende, “Textured growth of the high moment material Gd(0 0 0 1)/Cr(0 0 1)/Fe(0 0 1),” J. Phys. D: Appl. Phys. 44, 265004 (2011).
T. P. Bertelli, E. C. Passamani, C. Larica, V. P. Nascimento, and A. Y. Takeuchi, “Ferromagnetic properties of fcc Gd thin films,” J. Appl. Phys. 117, 203904 (2015).
G. Scheunert, O. Heinonen, R. Hardeman, A. Lapicki, M. Gubbins, and R. M. Bowman, “A review of high magnetic moment thin films for microscale and nanotechnology applications,” Appl. Phys. Rev. 3, 011301 (2016).
A. E. Curzon and H. G. Chlebek, “The observation of face centred cubic Gd, Tb, Dy, Ho, Er and Tm in the form of thin films and their oxidation,” J. Phys. F: Met. Phys. 3, 1–5 (1979).
Chin-Jui Hsu, S. V. Prikhodko, Wang Chiu-Yen, Chen Lih-Juann, and G. P. Carman, “Magnetic anisotropy in nanostructured gadolinium,” J. Appl. Phys. 111, 053916 (2012).
M. Bouroushian and T. Kosanovic, “Characterization of thin films by low incidence X-ray diffraction,” Cryst. Struct. Appl. 1, 35–39 (2012).
M. F. Toney and S. Brennan, “Structural depth profiling of iron oxide thin films using grazing incidence asymmetric Bragg X-ray diffraction,” J. Appl. Phys. 65, 4763–4768 (1989).
R. J. Elliott, Magnetic Properties of Rare Earth Metals (Springer-Verlag, New York, 1972).
P. E. Chizhov, A. N. Kostigov, and V. I. Petinov, “Structure and magnetic properties of rare earth small particles,” Solid State Commun. 42, 323–326 (1982).
Author information
Authors and Affiliations
Corresponding author
Additional information
Original Russian Text © M.V. Ryabukhina, E.A. Kravtsov, L.I. Naumova, V.V. Proglyado, Yu.N. Khaidukov, V.V. Ustinov, 2017, published in Fizika Metallov i Metallovedenie, 2017, Vol. 118, No. 2, pp. 151–157.
Rights and permissions
About this article
Cite this article
Ryabukhina, M.V., Kravtsov, E.A., Naumova, L.I. et al. Crystal structure and magnetic properties of Fe/Cr/Gd superlattices. Phys. Metals Metallogr. 118, 143–149 (2017). https://doi.org/10.1134/S0031918X17020119
Received:
Accepted:
Published:
Issue Date:
DOI: https://doi.org/10.1134/S0031918X17020119