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Fundamentals: by Stimulated Emission of Radiation

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A laser is a device that emits light through a process of optical amplification based on the stimulated emission of electromagnetic radiation.

The term "laser" originated as an acronym for Light Amplification [1][2] by Stimulated Emission of Radiation. Lasers differ from other sources of light because they emit light coherently. Its spatial coherence allows a laser to be focused to a tight spot, and this enables applications like laser cutting and laser lithography. Its spatial coherence also keeps a laser beam collimated over long distances, and this enables laser pointers to work. Laser also have high temporal coherence which allows them to have a very narrowspectrum, i.e., they only emit a single color of light. Their temporal coherence also allows them to emit pulses of light that only last afemtosecond. Lasers have many important applications. They are used in common consumer devices such as DVD players, laser printers, and barcode scanners. They are used in medicine for laser surgery and various skin treatments, and in industry for cutting and welding materials. They are used in military and law enforcement devices for marking targets and measuring range and speed. Laser lighting displays use laser light as an entertainment medium. Lasers also have many important applications in scientific research.

Fundamentals
Lasers are distinguished from other light sources by their coherence. Spatial coherence is typically expressed through the output being a narrow beam which is diffraction-limited, often a so-called "pencil beam." Laser beams can be focused to very tiny spots, achieving a very high irradiance, or they can be launched into beams of very low divergence in order to concentrate their power at a large distance. Temporal (or longitudinal) coherence implies a polarized wave at a single frequency whose phase is [3] correlated over a relatively large distance (the coherence length) along the beam. A beam produced by a thermal or other incoherent light source has an instantaneous amplitude and phase which vary randomly with respect to time and position, and thus a very short coherence length. Most so-called "single wavelength" lasers actually produce radiation in several modes having slightly different frequencies (wavelengths), often not in a single polarization. And although temporal coherence implies monochromaticity, there are even lasers that emit a broad spectrum of light, or emit different wavelengths of light simultaneously. There are some lasers which are not single spatial mode and consequently their light beams diverge more than required by the diffraction limit. However all such devices are classified as "lasers" based on their method of producing that light: stimulated emission. Lasers are employed in applications where light of the required spatial or temporal coherence could not be produced using simpler technologies.

A laser consists of a gain medium, a mechanism to supply energy to it, and something to provide [7] optical feedback. The gain medium is a material with properties that allow it to amplify light by stimulated emission. Light of a specific wavelength that passes through the gain medium is amplified (increases in power). For the gain medium to amplify light, it needs to be supplied with energy. This process is called pumping. The energy is typically supplied as an electrical current, or as light at a different wavelength. Pump light may be provided by a flash lamp or by another laser.

The most common type of laser uses feedback from an optical cavitya pair of mirrors on either end of the gain medium. Light bounces back and forth between the mirrors, passing through the gain medium and being amplified each time. Typically one of the two mirrors, the output coupler, is partially transparent. Some of the light escapes through this mirror. Depending on the design of the cavity (whether the mirrors are flat or curved), the light coming out of the laser may spread out or form a narrow beam. This type of device is sometimes called a laser oscillator in analogy to electronic oscillators, in which an electronic amplifier receives electrical feedback that causes it to produce a signal. Most practical lasers contain additional elements that affect properties of the emitted light such as the polarization, the wavelength, and the shape of

aser physics
See also: Laser science Electrons and how they interact with electromagnetic fields are important in our understanding of chemistry and physics.

Stimulated emission
In the classical view, the energy of an electron orbiting an atomic nucleus is larger for orbits further from the nucleus of an atom. However, quantum mechanical effects force electrons to take on discrete positions in orbitals. Thus, electrons are found in specific energy levels of an atom, two of which are shown below: When an electron absorbs energy either from light (photons) or heat (phonons), it receives that incident quantum of energy. But transitions are only allowed in between discrete energy levels such as the two shown above. This leads to emission lines and absorption lines. When an electron is excited from a lower to a higher energy level, it will not stay that way forever. An electron in an excited state may decay to a lower energy state which is not occupied, according to a particular time constant characterizing that transition. When such an electron decays without external influence, emitting a photon, that is called "spontaneous emission". The phase associated with the photon that is emitted is random. A material with many atoms in such an excited state may thus result in radiation which is very spectrally limited (centered around onewavelength of light), but the individual photons would have no common phase relationship and would emanate in random directions. This is the mechanism of fluorescence and thermal emission. An external electromagnetic field at a frequency associated with a transition can affect the quantum mechanical state of the atom. As the electron in the atom makes a transition between two stationary states (neither of which shows a dipole field), it enters a transition state which does have a dipole field, and which acts like a small electric dipole, and this dipole oscillates at a characteristic frequency. In response to the external electric field at this frequency, the probability of the atom entering this transition state is greatly increased. Thus, the rate of transitions between two stationary states is enhanced beyond that due to spontaneous emission. Such a transition to the higher state is called absorption, and it destroys an incident photon (the photon's energy goes into powering the increased energy of the higher state). A transition from the higher to a lower energy state, however, produces an additional photon; this is the process of stimulated emission. Gain medium and cavity

The gain medium is excited by an external source of energy into an excited state. In most lasers this medium consists of population of atoms which have been excited into such a state by means of an outside light source, or an electrical field which supplies energy for atoms to absorb and be transformed into their excited states. The gain medium of a laser is normally a material of controlled purity, size, concentration, and shape, which amplifies the beam by the process of stimulated emission described above. This material can be of any state: gas, liquid, solid, or plasma. The gain medium absorbs pump energy, which raises some electrons into higher-energy ("excited") quantum states. Particles can interact with light by either absorbing or emitting photons. Emission can be spontaneous or stimulated. In the latter case, the photon is emitted in the same direction as the light that is passing by. When the number of particles in one excited state exceeds the number of particles in some lower-energy state, population inversion is achieved and the amount of stimulated emission due to light that passes through is larger than the amount of absorption. Hence, the light is amplified. By itself, this makes an optical amplifier. When an [8] optical amplifier is placed inside a resonant optical cavity, one obtains a laser oscillator. In a few situations it is possible to obtain lasing with only a single pass of EM radiation through the gain medium, and this produces a laser beam without any need for a resonant or reflective cavity (see for [9] example nitrogen laser). Thus, reflection in a resonant cavity is usually required for a laser, but is not absolutely necessary. The optical resonator is sometimes referred to as an "optical cavity", but this is a misnomer: lasers use open resonators as opposed to the literal cavity that would be employed at microwave frequencies in a maser. The resonator typically consists of two mirrors between which a coherent beam of light travels in both directions, reflecting back on itself so that an average photon will pass through the gain medium repeatedly before it is emitted from the output aperture or lost to diffraction or absorption. If the gain (amplification) in the medium is larger than the resonator losses, then the power of the recirculating light can rise exponentially. But each stimulated emission event returns an atom from its excited state to the ground state, reducing the gain of the medium. With increasing beam power the net gain (gain minus loss) reduces to unity and the gain medium is said to be saturated. In a continuous wave (CW) laser, the balance of pump power against gain saturation and cavity losses produces an equilibrium value of the laser power inside the cavity; this equilibrium determines the operating point of the laser. If the applied pump power is too small, the gain will never be sufficient to overcome the resonator losses, and laser light will not be produced. The minimum pump power needed to begin laser action is called the lasing threshold. The gain medium will amplify any photons passing through it, regardless of direction; but only the photons in a spatial modesupported by the resonator will pass more than once through the medium and receive substantial amplification.

The light emitted


The light generated by stimulated emission is very similar to the input signal in terms of wavelength, phase, and polarization. This gives laser light its characteristic coherence, and allows it to maintain the uniform polarization and often monochromaticity established by the optical cavity design. The beam in the cavity and the output beam of the laser, when travelling in free space (or a homogenous medium) rather than waveguides (as in anoptical fiber laser), can be approximated as a Gaussian beam in most lasers; such beams exhibit the minimum divergence for a given diameter. However some high power lasers may be multimode, with the transverse modes often approximated using Hermite-

Gaussian or Laguerre-Gaussian functions. It has been shown that unstable laser resonators (not used in [10] most lasers) produce fractal shaped beams. Near the beam "waist" (or focal region) it is highly collimated: the wavefronts are planar, normal to the direction of propagation, with no beam divergence at that point. However due todiffraction, that can only remain true well within the Rayleigh range. The beam of a single transverse mode (gaussian beam) laser eventually diverges at an angle which varies inversely with the beam diameter, as required by diffraction theory. Thus, the "pencil beam" directly generated by a commonhelium-neon laser would spread out to a size of perhaps 500 kilometers when shone on the Moon (from the distance of the earth). On the other hand the light from a semiconductor laser typically exits the tiny crystal with a large divergence: up to 50. However even such a divergent beam can be transformed into a similarly collimated beam by means of a lens system, as is always included, for instance, in a laser pointer whose light originates from a laser diode. That is possible due to the light being of a single spatial mode. This unique property of laser light, spatial coherence, cannot be replicated using standard light sources (except by discarding most of the light) as can be appreciated by comparing the beam from a flashlight (torch) or spotlight to that of almost any laser.

Quantum vs. classical emission processes


The mechanism of producing radiation in a laser relies on stimulated emission, where energy is extracted from a transition in an atom or molecule. This is a quantum phenomenon discovered byEinstein who derived the relationship between the A coefficient describing spontaneous emission and the B coefficient which applies to absorption and stimulated emission. However in the case of the free electron laser, atomic energy levels are not involved; it appears that the operation of this rather exotic device can be explained without reference to quantum mechanics.

Continuous and pulsed modes of operation


A laser can be classified as operating in either continuous or pulsed mode, depending on whether the power output is essentially continuous over time or whether its output takes the form of pulses of light on one or another time scale. Of course even a laser whose output is normally continuous can be intentionally turned on and off at some rate in order to create pulses of light. When the modulation rate is on time scales much slower than the cavity lifetime and the time period over which energy can be stored in the lasing medium or pumping mechanism, then it is still classified as a "modulated" or "pulsed" continuous wave laser. Most laser diodes used in communication systems fall in that category.

Continuous wave operation


Some applications of lasers depend on a beam whose output power is constant over time. Such a laser is known as continuous wave (CW). Many types of lasers can be made to operate in continuous wave mode to satisfy such an application. Many of these lasers actually lase in several longitudinal modes at the same time, and beats between the slightly different optical frequencies of those oscillations will in fact produce amplitude variations on time scales shorter than the round-trip time (the reciprocal of the frequency spacing between modes), typically a few nanoseconds or less. In most cases these lasers are still termed "continuous wave" as their output power is steady when averaged over any longer time periods, with the very high frequency power variations having little or no impact in the intended application. (However the term is not applied to mode-locked lasers, where the intention is to create very short pulses at the rate of the round-trip time).

For continuous wave operation it is required for the population inversion of the gain medium to be continually replenished by a steady pump source. In some lasing media this is impossible. In some other lasers it would require pumping the laser at a very high continuous power level which would be impractical or destroy the laser by producing excessive heat. Such lasers cannot be run in CW mode.

Pulsed operation
Pulsed operation of lasers refers to any laser not classified as continuous wave, so that the optical power appears in pulses of some duration at some repetition rate. This encompasses a wide range of technologies addressing a number of different motivations. Some lasers are pulsed simply because they cannot be run in continuous mode. In other cases the application requires the production of pulses having as large an energy as possible. Since the pulse energy is equal to the average power divided by the repetition rate, this goal can sometimes be satisfied by lowering the rate of pulses so that more energy can be built up in between pulses. In laser ablation for example, a small volume of material at the surface of a work piece can be evaporated if it is heated in a very short time, whereas supplying the energy gradually would allow for the heat to be absorbed into the bulk of the piece, never attaining a sufficiently high temperature at a particular point. Other applications rely on the peak pulse power (rather than the energy in the pulse), especially in order to obtain nonlinear optical effects. For a given pulse energy, this requires creating pulses of the shortest possible duration utilizing techniques such as Q-switching. The optical bandwidth of a pulse cannot be narrower than the reciprocal of the pulse width. In the case of extremely short pulses, that implies lasing over a considerable bandwidth, quite contrary to the very narrow bandwidths typical of CW lasers. The lasing medium in some dye lasers and vibronic solid-state lasers produces optical gain over a wide bandwidth, making a laser possible which can thus generate 15 pulses of light as short as a few femtoseconds (10 s).

Q-switching
Main article: Q-switching In a Q-switched laser, the population inversion is allowed to build up by introducing loss inside the resonator which exceeds the gain of the medium; this can also be described as a reduction of the quality factor or 'Q' of the cavity. Then, after the pump energy stored in the laser medium has approached the maximum possible level, the introduced loss mechanism (often an electro- or acousto-optic al element) is rapidly removed (or that occurs by itself in a passive device), allowing lasing to begin which rapidly obtains the stored energy in the gain medium. This results in a short pulse incorporating that energy, and thus a high peak power.

Mode-locking
Main article: Mode-locking A mode-locked laser is capable of emitting extremely short pulses on the order of tens of picoseconds down to less than 10 femtoseconds. These pulses will repeat at the round trip time, that is, the time that it takes light to complete one round trip between the mirrors comprising the resonator. Due to the Fourier limit (also known as energy-time uncertainty), a pulse of such short temporal length

has a spectrum spread over a considerable bandwidth. Thus such a gain medium must have a gain bandwidth sufficiently broad to amplify those frequencies. An example of a suitable material is titaniumdoped, artificially grown sapphire (Ti:sapphire) which has a very wide gain bandwidth and can thus produce pulses of only a few femtoseconds duration. Such mode-locked lasers are a most versatile tool for researching processes occurring on extremely short time scales (known as femtosecond physics, femtosecond chemistry and ultrafast science), for maximizing the effect of nonlinearity in optical materials (e.g. in second-harmonic generation, parametric down-conversion, optical parametric oscillators and the like) due to the large peak power, and in ablation [citation needed] applications. Again, because of the extremely short pulse duration, such a laser will produce pulses which achieve an extremely high peak power.

Pulsed pumping
Another method of achieving pulsed laser operation is to pump the laser material with a source that is itself pulsed, either through electronic charging in the case of flash lamps, or another laser which is already pulsed. Pulsed pumping was historically used with dye lasers where the inverted population lifetime of a dye molecule was so short that a high energy, fast pump was needed. The way to overcome this problem was to charge up large capacitors which are then switched to discharge through flashlamps, producing an intense flash. Pulsed pumping is also required for three-level lasers in which the lower energy level rapidly becomes highly populated preventing further lasing until those atoms relax to the ground state. These lasers, such as the excimer laser and the copper vapor laser, can never be operated in CW mode.

History
Foundations
In 1917, Albert Einstein established the theoretical foundations for the laser and the maser in the paper Zur Quantentheorie der Strahlung (On the Quantum Theory of Radiation); via a re-derivation of Max Planck's law of radiation, conceptually based upon probability coefficients (Einstein coefficients) for the absorption, spontaneous emission, and stimulated emission of electromagnetic radiation; in 1928, Rudolf W. Ladenburg confirmed the existences of the phenomena of stimulated emission and [11] negative absorption; in 1939, Valentin A. Fabrikant predicted the use of stimulated emission to amplify [12] "short" waves; in 1947, Willis E. Lamb and R. C. Retherford found apparent stimulated emission in [11] hydrogen spectra and effected the first demonstration of stimulated emission; in 1950, Alfred Kastler (Nobel Prize for Physics 1966) proposed the method of optical pumping, experimentally [13] confirmed, two years later, by Brossel, Kastler, and Winter.

Maser
Main article: Maser n 1953, Charles Hard Townes and graduate students James P. Gordon and Herbert J. Zeiger produced the first microwave amplifier, a device operating on similar principles to the laser, but amplifying microwave radiation rather than infrared or visible radiation. Townes's maser was incapable of [citation needed] continuous output. Meanwhile, in the Soviet Union, Nikolay Basov and Aleksandr Prokhorov were independently working on the quantum oscillator and solved the problem of continuousoutput systems by using more than two energy levels. These gain media could release stimulated

emissions between an excited state and a lower excited state, not the ground state, facilitating the maintenance of a population inversion. In 1955, Prokhorov and Basov suggested optical pumping of a multi-level system as a method for obtaining the population inversion, later a main method of laser pumping. Townes reports that several eminent physicists among them Niels Bohr, John von Neumann, Isidor Rabi, Polykarp Kusch, and Llewellyn Thomas argued the maser violated Heisenberg's uncertainty [14] principle and hence could not work. In 1964 Charles H. Townes, Nikolay Basov, and Aleksandr Prokhorov shared theNobel Prize in Physics, "for fundamental work in the field of quantum electronics, which has led to the construction of oscillators and amplifiers based on the maserlaser principle".

Laser
In 1957, Charles Hard Townes and Arthur Leonard Schawlow, then at Bell Labs, began a serious study of the infrared laser. As ideas developed, they abandonedinfrared radiation to instead concentrate upon visible light. The concept originally was called an "optical maser". In 1958, Bell Labs filed a patent application for their proposed optical maser; and Schawlow and Townes submitted a manuscript of their theoretical calculations to the Physical Review, published that year in Volume 112, Issue No. 6 sFiber

lasers

Main article: Fiber laser Solid-state lasers or laser amplifiers where the light is guided due to the total internal reflection in a single mode optical fiber are instead called fiber lasers. Guiding of light allows extremely long gain regions providing good cooling conditions; fibers have high surface area to volume ratio which allows efficient cooling. In addition, the fiber's waveguiding properties tend to reduce thermal distortion of the beam. Erbium and ytterbium ions are common active species in such lasers. Quite often, the fiber laser is designed as a double-clad fiber. This type of fiber consists of a fiber core, an inner cladding and an outer cladding. The index of the three concentric layers is chosen so that the fiber core acts as a single-mode fiber for the laser emission while the outer cladding acts as a highly multimode core for the pump laser. This lets the pump propagate a large amount of power into and through the active inner core region, while still having a high numerical aperture (NA) to have easy launching conditions. Pump light can be used more efficiently by creating a fiber disk laser, or a stack of such lasers. Fiber lasers have a fundamental limit in that the intensity of the light in the fiber cannot be so high that optical nonlinearities induced by the local electric field strength can become dominant and prevent laser operation and/or lead to the material destruction of the fiber. This effect is called photodarkening. In bulk laser materials, the cooling is not so efficient, and it is difficult to separate the effects of photodarkening from the thermal effects, but the experiments in fibers show that the photodarkening can be attributed to [citation needed] the formation of long-living color centers.

Photonic crystal lasers


imultaneously, at Columbia University, graduate student Gordon Gould was working on a doctoral thesis about the energy levels of excited thallium. When Gould and Townes met, they spoke of radiation emission, as a general subject; afterwards, in November 1957, Gould noted his ideas for a "laser", including using an open resonator (later an essential laser-device component). Moreover, in 1958,

Prokhorov independently proposed using an open resonator, the first published appearance (the USSR) of this idea. Elsewhere, in the U.S., Schawlow and Townes had agreed to an open-resonator laser design apparently unaware of Prokhorov's publications and Gould's unpublished laser work. At a conference in 1959, Gordon Gould published the term LASER in the paper The LASER, Light [1][5] Amplification by Stimulated Emission of Radiation. Gould's linguistic intention was using the "-aser" word particle as a suffix to accurately denote the spectrum of the light emitted by the LASER device; thus x-rays: xaser, ultraviolet: uvaser, et cetera; none established itself as a discrete term, although "raser" was briefly popular for denoting radio-frequency-emitting devices. Gould's notes included possible applications for a laser, such as spectrometry, interferometry, radar, and nuclear fusion. He continued developing the idea, and filed a patent application in April 1959. The U.S. Patent Office denied his application, and awarded a patent to Bell Labs, in 1960. That provoked a twenty-eight-year lawsuit, featuring scientific prestige and money as the stakes. Gould won his first minor patent in 1977, yet it was not until 1987 that he won the first significant patent lawsuit victory, when a Federal judge ordered the U.S. Patent Office to issue patents to Gould for the optically pumped and the gas discharge laser devices. The question of just how to assign credit for inventing the laser remains [15] unresolved by historians. On May 16, 1960, Theodore H. Maiman operated the first functioning laser, at Hughes Research Laboratories, Malibu, California, ahead of several research teams, including those of Townes, [18] at Columbia University, Arthur Schawlow, at Bell Labs, and Gould, at the TRG (Technical Research Group) company. Maiman's functional laser used a solid-state flashlamp-pumped synthetic ruby crystal to produce red laser light, at 694 nanometres wavelength; however, the device only was capable of pulsed operation, because of its three-level pumping design scheme. Later in 1960, the Iranianphysicist Ali Javan, and William R. Bennett, and Donald Herriott, constructed the first gas laser, using helium and neon that was capable of continuous operation in the infrared (U.S. Patent 3,149,290); later, Javan received the Albert Einstein Award in 1993. Basov and Javan proposed the semiconductorlaser diode concept. In 1962, Robert N. Hall demonstrated the first laser diode device, made of gallium arsenide and emitted at 850 nm the near-infrared band of the spectrum. Later, in 1962, Nick Holonyak, Jr. demonstrated the first semiconductor laser with a visible emission. This first semiconductor laser could only be used in pulsed-beam operation, and when cooled to liquid nitrogentemperatures (77 K). In 1970, Zhores Alferov, in the USSR, and Izuo Hayashi and Morton Panish of Bell Telephone Laboratories also independently developed room-temperature, continual-operation diode lasers, using the heterojunction structure.
[16][17]

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