Laser Cooling and Trapping
Laser Cooling and Trapping
Laser Cooling and Trapping
2.1 L ASER C O O L I N G
The primary force used in laser cooling and trapping is the recoil when momentum is transferred
from photons scattering off an atom. This radiation-pressure force is analogous to that applied to a
bowling ball when it is bombarded by a stream of ping pony balls. The momentum kick that the atom
receives from each scattered photon is quite small; a typical velocity change is about 1 cm/s. However,
by exciting a strong atomic transition, it is possible to scatter more than 107 photons per second and
produce large accelerations (104 g). The
radiation-pressure force is controlled in such
n laser + Dn Doppler a way that it brings the atoms in a sample to a
Scattering Rate (force)
N (t ) = N0 (1 - e - t / t ) , (1)
where t is the time constant for the trap to fill to its steady state value N 0 and is also the average time an
atom will remain in the trap before it is knocked out by a collision. This time is just the inverse of the loss
rate from the trap due to collisions. Under certain conditions, collisions between the trapped atoms can be
important, but for conditions that are usually encountered, the loss rate will be dominated by collisions
with the room temperature background gas. These "hot" background atoms and molecules (rubidium and
contaminants) have more than enough energy to knock atoms out of the trap. The time constant t can be
expressed in terms of the cross sections s , densities n, and velocities of rubidium and non-rubidium
components as:
1
= nRbs Rb vRb + nnons non vnon . (2)
t
The steady-state number of trapped atoms is that value for which the capture and loss rates of the
trap are equal. The capture rate is simply given by the number of atoms which enter the trap volume (as
defined by the overlap of the laser beams) with speeds less than vmax . It is straightforward to show that
4
this is proportional to the rubidium density, vmax , and the surface area A of the trap. When the
background vapor is predominantly rubidium, the loss and capture rates are both proportional to
rubidium pressure. In this case N0 is simply:
4
A Ê vmax ˆ
N0 = 0.1 , (3)
s Rb ÁË vavg ˜¯
where vavg = (2 kT / m) , the average velocity of the rubidium atoms in the vapor. If the loss rate due to
1/ 2
collisions with non-rubidium background gas is significant, Eq. (3) must be multiplied by the factor
( )
nRbs Rb vavg / nRbs Rb vavg + nnons non vnon . The densities are proportional to the respective partial pressures.
Finally, if the loss rate is dominated by collisions with non-rubidium background gas, the number of
atoms in the trap will be proportional to the rubidium pressure divided by the non-rubidium pressure, but
t will be independent of the rubidium pressure.
As a final note on the theory of trapping and cooling, we emphasize certain qualitative features that
are not initially obvious. This trap is a highly over-damped system; hence damping effects are more
important for determining trap performance than is the trapping force. If this is kept in mind it is much
easier to gain an intuitive understanding of the trap behavior. Because it is highly over-damped, the
critical quantity vmax is determined almost entirely by the Doppler slowing which provides the damping.
Also, the cross sections for collisional loss are only very weakly dependent on the depth of the trap, and
therefore the trap lifetime is usually quite insensitive to everything except background pressure. As a
result of these two features, the number of atoms in the trap is very sensitive to laser beam diameter,
power, and frequency, all of which affect the Doppler cooling and hence vmax However, the number of
trapped atoms is insensitive to factors which primarily affect the trapping force but not the damping, such
as the magnetic field (stray or applied) and the alignment and polarizations of the laser beams. For
example, changing the alignment of the laser beams will dramatically affect the shape of the cloud of
trapped atoms since it changes the shape of the trapping potential. However, these very differently
shaped clouds will still have similar numbers of atoms until the alignment is changed enough to affect the
volume of the laser beam overlap. When this happens, the damping in three dimensions is changed and
the number of trapped atoms will change dramatically. Of course, if the trapping potential is changed
enough that there is no potential minimum (for example, the zero of the magnetic field is no longer within
the region of overlap of the laser beams), there will be no trapped atoms. However, as long as the
damping force remains the same, almost any potential minimum will have about the same number of
atoms and trap lifetime.
Hyperfine
Variable
pumping laser attenuator
Pump
beam
Laser driver
Rb
cell
Probe
beams
Thick M
beamsplitter
Vortex™
diode laser
l/4
BS BS
l/4
Thick
M M
beamsplitter
l/4
Unused BS l/4 Vacuum
Rb
Pump
beam cell
cell
Probe Photo-
beams Variable diodes
attenuator
Output
signal
Amplifier
Ramp M
generator
Vortex™
diode laser M
M
Servo
electronics
Laser driver
Trapping
laser
Figure 6. Overall optical layout for laser trap experiment including both saturated absorption
spectrometers.
PZT (piezo)
servo gain
adjust
Error in
(from photodiode Polarity +/-
preamplifier) V err Vset - Verr Monitor out
(to oscilloscope)
BNC
-1 BNC
Servo
amplifier Servo loop
open/closed
Vset
Ramp in
(from ramp
generator) Ramp on/off
PZT/piezo out
(to Vortex™ controller)
BNC
BNC
Ramp
amplifier
BNC
Figure 9. Laser frequency stabilization servo control box. Shaded and dashed boxes indicate the knobs and switches on the
controller unit.
controller box are schematically illustrated in Figure 9. The shaded, dashed-outline boxes label the
various switches and knobs that are on the controller.
The next item of business is to zoom in on the rubidium hyperfine atomic transition of interest (e.g.,
the 5S F = 2 Æ 5P F ¢ = 3 transition of 87Rb.) To do so you will use the ramp gain adjust and PZT bias
controls. Connect the photodiode preamplifier output to the “Error In” BNC of the servo controller. Also
observe the photodiode preamplifier output with the scope. Set the ramp gain to a relatively high value
until you see the various rubidium lines as described in the Doppler Free Saturated Absorption
Spectroscopy experiment. Center the line of interest on the oscilloscope. You can do so by adjusting the
PZT bias knob (coarse, at first) on the servo controller —you can also do it by setting the piezo voltage
on the Vortex™ controller directly. Actually, the latter is a bit safer, as the input specifications will not
inadvertently be exceeded. To zero-in on the line requires an iterative process. The idea is to reduce the
sweep voltage of the piezo by decreasing the ramp gain, then re-centering the scan range to the desired
frequency with the piezo offset or the Vortex™ controller piezo setting, then reducing the ramp gain
again, and so onUsing the second channel of the oscilloscope used to monitor the photodiode
preamplifier output, connect the “Monitor output” of the servo controller box. Be sure to note the
position of the scope trace zero for this channel. At the same time, notice the value Vref of the photodiode
preamplifier output when it is halfway up the transition. The next step is to adjust the “Setpoint” value of
the servo controller. It determines value of the voltageVset shown in Figure 9. Notice what the circuit
does —the input to the servo amplifier is the difference, Verr - Vset , where Verr is the photodiode
preamplifier output voltage. This difference is amplified and then (will later be) fed back to the piezo
voltage input of the Vortex™ controller. You should adjust the Setpoint knob so that the monitor output
passes through zero exactly at the point where the laser is halfway up the transition curve. You can
overlap the monitor and photodiode preamplifier traces on the oscilloscope, then adjust the setpoint knob
so former traces crosses zero at the appropriate place.
Here we just mention a few potential problems and solutions Check that the baseline on the saturated
absorption spectrum well off resonance is not fluctuating by more than several percent of the
F = 2 Æ F ¢ = 3 peak height. If there are larger fluctuations, they are likely caused by light feeding back
into the laser or by the probe beams vibrating across the surface of the photodiodes. Changing the
alignment and making sure that all the optical components are rigidly mounted will normally solve these
problems. Under quiet conditions and reasonably constant room temperature, the laser should stay
locked for many minutes and sometimes hours at a time. Bumping the table or the laser or making a loud
noise will likely knock the laser out of lock
4 OPTICAL SYSTEM
The beams from the lasers must now be sent into the cell to form the trap. The basic requirement is
to send light beams from the trapping laser into the cell in such a way that the radiation-pressure force has
a component along all six directions. To motivate the discussion of the optical design for this lab, we first
mention the design used in most of the traps in research programs. In these research traps, the light from
the trapping laser first passes through an optical isolator and then through beam shaping optics that make
the elliptical diode laser beam circular and expand it to between 1 and 1.5 cm in diameter. The beam is
then split into three equal intensity beams using dielectric beam splitters. These three beams are circularly
polarized with quarter-wave plates before they pass through the trapping cell where they intersect at right
angles in the center of the cell. After leaving the trapping cell each beam goes through a second
quarter-wave plate and is then reflected back on itself with a mirror. This accomplishes the goal of having
three orthogonal pairs of nearly counter-propagating beams, with the reflected beams having circular
polarization opposite to the original beams.
4.1 G EOMETRY
For this lab you use a modified version of this setup, as shown in Fig. 5. A number of the
expensive optical components (optical isolator, dielectric beam splitters, and large aperture high quality
quarter-wave plates) have been eliminated from the research design. The light from the trapping diode
laser is sent into a simple two-lens telescope that expands it. This is then split into three beams. The
operation of the trap is insensitive to the relative amounts of power in each of the beams. [You should
check how much the number of trapped atoms change with a factor-of-two difference in relative powers.]
However, the beam size as set by the telescope is of some importance. The number of trapped atoms
increases quite rapidly as the beam size increases and, as discussed below, the larger the beam, the less
critical the alignment. However, if the beams are too large they will not fit on the mirrors and it becomes
harder to see the beams due to their reduced intensity. Beams of about 1.5 cm diameter work well, but
avoid using beams much smaller than 1.5 cm in diameter because of the decrease in the number of
trapped atoms and the increased alignment sensitivity. The lenses in the lab will make a simple telescope
that expands the beam from the diode laser to this size.
Two of the three beams remain in a horizontal plane and are sent into the cell as shown in Figure 7.
The third is angled down and reflects up from the bottom of the cell. To simplify the adjustment of the
polarizations, the light should be kept linearly polarized until it reaches the quarter-wave plates. This will
be the case as long as all the beams have their axes of polarization either parallel (p) or perpendicular (s)
to the plane of incidence of each mirror. This is easy to achieve for the beams in the horizontal plane, but
difficult for the beam that comes up through the bottom of the cell. However, with minimal effort to be
close to this condition, the polarization will remain sufficiently well linearly polarized. If you think this
might be a problem you can check the ellipticity of the polarization by using a photodiode and a rotatable
linear polarizer. An eccentricity of 10 or greater on the polarization ellipse is adequate.
After they pass through the cell, the beams are reflected approximately (but not exactly!) back on
themselves. The reason for having an optical isolator in the research design is that even a small amount of
laser light reflected back into the laser will dramatically shift the laser frequency and cause it to jump out
of lock. In the absence of an optical isolator, this will always happen if the laser beams are reflected
nearly back on themselves. Feedback can be avoided by insuring that the reflected beams are steered
away from the incident beams so that they are spatially offset by many (5-10) beam diameters when they
arrive back at the position of the laser. Fortunately, for operation of the trap the return beam need only
overlap most of the incident beam in the cell, but its exact direction is unimportant. Thus by making the
beams large and placing the retro mirrors close to the trap (within 10 cm for example) it is possible to
have the forward and backward going beams almost entirely overlap even when the angle between them
is substantially different from 180°. This design eliminates the need for the very expensive ($2500)
optical isolator and, as an added benefit, makes the operation of the trap very insensitive to the alignment
of the return beams.
It is easy to tell if feedback from the return beams is perturbing the laser by watching the signal from
the saturated absorption spectrometer on the oscilloscope. If the amplitude of the fluctuations is affected
by the alignment of the reflected beam or is reduced when the beam to the trapping cell is blocked,
unwanted optical feedback is occurring.
4.2 P OLARIZATION
The next task is to set the polarizations of the three incident beams. The orientations of the respective
circular polarizations are determined by the orientation of the magnetic field gradient coils. The two
transverse beams that propagate through the cell perpendicular to the coil axis should have the same
circular polarization, while the beam that propagates along the axis of the coils should have the opposite
circular polarization. Although in principle it is possible to initially determine and set all three
polarizations correctly with respect to the magnetic field gradient, in practice it is much simpler to set the
three polarizations relative to each other and then try both directions of current through the magnetic field
coils to determine which sign of magnetic field gradient makes the trap work. To set the relative
polarization of the three beams, first identify the same (fast or slow) axis of the three quarter-wave (l/4)
plates. For the two beams that are to have the same polarization, this axis is set at an angle of 45°
clockwise with respect to the linear polarization axis when looking along the laser beam. For the axial
beam, the axis is oriented at 45° counterclockwise with respect to the linear polarization. This orientation
needs only to be set to within about ±10°. The orientation of the l/4 plates through which the beams pass
after they have gone through the trapping cell ("retro l/4 plates") is arbitrary. No matter what the plates'
orientations are, after the beams have passed though them twice, the light's circular polarization will be
reversed.
An optional experiment is to see what happens when you replace one or more of the three retro l/4
plates with retro-reflecting right angle mirrors. [1] Although this combination of mirrors does not provide
ideal l/2 retardance, it is fairly close. An added benefit of this approach is that two reflections off a
mirror usually result in much less light loss than one reflection and two passes through a l/4 plate.
Epoxied
glass cell
zero length
Pumpout adapter
valve
Ion Pump
Rubidium
dispenser
bottom
window
Figure 10. Drawing of trapping cell. The tubes on the cross have been elongated in the drawing
for ease of display. The Rb dispenser is inside a stainless steel vacuum tube; we show a
cut-away view in this drawing.
difficult to see them because of the bright fluorescence from the un-trapped background atoms. Also, the
absorption of the trapping beams when passing through the cell will be significant. Thus you should
maintain the rubidium at well below its room temperature vapor pressure. Because it is necessary to
continuously pump on the system to avoid the buildup of hydrogen and helium vapor, it is necessary to
have a constant source of rubidium to maintain the correct pressure. Through chemical reactions and
physisorption, the walls of the cell usually remove far more rubidium than the ion pump does and the rate
of pumping by the walls depends on how well they are coated with rubidium.
In this experiment the rubidium vapor is produced by a commercial “rubidium dispenser” (locally
sometimes also referred to as a “rubidium getter”. The dispenser is several milligrams of a rubidium
compound that is contained in a small (1.0 x 0.2 x 0.2 cm) stainless steel oven. Two of these ovens are
spot-welded onto two pins of a vacuum feed-through, one of which is illustrated in Figure 10. When
current (3-5 A) is sent through the oven, rubidium vapor is produced. The higher the current, the higher
the rubidium pressure in the chamber. With this system it is unnecessary to coat the entire surface with
rubidium, and is in fact undesirable since the dispenser is likely to be exhausted before the surface is
entirely saturated. You should be able to produce enough rubidium pressure to easily see the background
fluorescence with as little as 3.4 A through the dispenser oven. The current through the dispenser is
controlled by the power supply under the table. Be careful not to turn the current higher than 6.5 amps
under any circumstances! If you do it will burn out the dispenser and ruin the experiment! You can see
how much rubidium is in the cell by sending the laser beams into the cell, setting the laser frequency to
the trapping transition (the saturated absorption cell should glow brightly) and look for fluorescence from
the atoms in the cell. If you can see any glow from inside the cell that goes away when the laser
frequency is tuned off the transition, there is more than enough rubidium for trapping.
After the current through the dispenser has been turned on, the rubidium vapor comes to an
equilibrium pressure with a time constant of about 5 min. When the current through the dispenser is
turned off, the rubidium pressure drops with a time constant of about 4 s if the dispenser has been on for
only a short while. With prolonged use of the dispenser, this time constant can increase up to a few
minutes as rubidium builds up on the walls, but it decreases to the original value if the dispenser is left
off for several days.
The superior rubidium pressure control provided by the dispenser makes it possible to use high
pressures to easily observe fluorescence from the background vapor. This allows one both to check
whether the laser and cell are operating properly, and to have rapid response in the number of atoms
while optimizing trapping parameters. Once these tasks are complete, simply reducing the dispenser
current provides low pressures almost immediately. Low pressures are desirable for many experiments
because they yield relatively long trap lifetimes (seconds) and little background light from the
fluorescence of un-trapped atoms.
measurements, in the standard operation of the trap, use the setting on the dispenser current and/or the
observation of the fluorescence to check that the pressure is reasonable.
After an adequate rubidium pressure has been detected, the magnetic field gradient is turned on and
the lasers are set to the appropriate transitions. If the apparatus is being used for the first time, it will be
necessary to try both directions of current through the field coils to determine the correct sign for
trapping. The trapped atoms should appear as a small bright cloud, much brighter than the background
fluorescence. Pieces of dust on the windows may appear nearly as bright, but they will be more localized
and can be easily distinguished by the fact they do not change with the laser frequencies or magnetic
field. If the trap does not work (and the direction of magnetic field and the laser polarizations are set
correctly) the lasers are probably not set on the correct transitions. The trapped atom cloud may vary in
size; it can be anywhere from less than 1 mm in diameter to several millimeters. Blocking any of the
beams is also a simple method for distinguishing the trapped atoms from the background light.
6.3 M EASUREMENTS
Although many other more complicated measurements could be made with the trap, you should start
by making the two most straightforward measurements: the number of trapped atoms and the time that
atoms remain in the trap. If you have time after completing these, you can consider other experiments.
These measurements are both made by observing the fluorescence from the trapped atoms with a
photodiode. The number of atoms is determined by measuring the amount of light coming from the
trapped atoms and dividing by the amount of light scattered per atom, which is calculated from the
excited state lifetime. The time the atoms remain in the trap is found by observing the trap filling time and
using Eq.(1). To make a reliable measurement of the number of trapped atoms, it is crucial to accurately
separate the fluorescence of the trapped atoms from the scattered light and the fluorescence of the
background vapor. To do this one must compare the signal difference between having the trap off and
on. Therefore, the trap must be disabled in a way that has a negligibly small effect on the background
light. We have found that turning off or, even better, reversing the magnetic field is usually the best way
to do this. The magnetic field may alter the background fluorescence, but this change is generally smaller
than the signal of a typical cloud of trapped atoms. Check how big an effect this is. Once you have
determined the photocurrent due to just the trapped atoms, the total amount of light emitted can be found
using the photodiode calibration of 0.3 mA/mW and calculating the detection solid angle. The rate R at
which an individual atom scatters photons is given by
pG( I / Is )
R= (4)
1 + ( I / Is ) + 4( D / G )
2
where I is the sum of the intensities of the six trapping beams, G is the 6 MHz natural linewidth of the
transition, D is the detuning of the laser frequency from resonance, and I s, is the 4.1 mW/cm2 saturation
intensity. The simplest way to find D is to ramp over the saturated absorption spectrum and, when
looking at the locking error signal, find the position of the lock point (zero crossing point) relative to the
peak of the line. The frequency scale for the ramp can be determined using the known spacing between
two hyperfine peaks. A typical number for R is 6 x 106 photons / (s ¥ atoms) . One can optimize the
number of atoms in the trap by adjusting the position of the magnetic field coils, the size of the gradient,
the frequencies of both trapping and hyperfine pumping lasers, the beam alignments, and the polarization
of the beams. More than 107 trapped atoms have been obtained when the rubidium pressure is large
enough to dominate the lifetime.
The filling of the trap can also be observed using the same photodiode signal. This is best done by
suddenly turning on the current to the field coils to produce a trap. The fluorescence signal from the
photodiode will then follow the dependence given by Eq. (1), as shown in Figure 11. This can be most
easily observed by sending the photodiode signal into a storage scope. The value of the 1/e trap lifetime t
7 REFERENCES
1. K. B. MacAdam, A. Steinbach, and C. Wieman, "A narrow-band tunable diode laser
system with grating feedback and a saturated absorption spectrometer for Cs and Rb," Am.
J. Phys., 60, 1098-1111 (1992) and the Senior Lab manual.
2. S. L. Gilbert and C. E. Wieman, "Laser Cooling and Trapping for the Masses," Optics and
Photonics News, 4, 8-14 (1993).
3. The initial demonstration and discussion is E. L. Raab, M. Prentiss, A. Cable, S. Chu, and D.
Pritchard, "Trapping of neutral sodium atoms with radiation pressure," Phys. Rev. Lett. 59,
2631-2634 (1987). More detailed analysis of the trap is given in A. M. Steane, M. Chowdhury, and
C. J. Foot, "Radiation force in the magneto-optical trap," J. Opt. Soc. Am B 9, 2142 (1992), while
a discussion of many of the novel aspects of the behavior of atoms in the trap is given in D. Sesko,
T. Walker and C. Wieman, "Behavior of neutral atoms in a spontaneous force trap," J. Opt. Soc.
Am. B 8, 946-958 (1991).
4. C. Monroe, W. Swann, H. Robinson, and C. Wieman, "Very cold atoms in a vapor cell," Phys.
Rev. Lett. 65, 1990, 1571-1574; K. Lindquist, M. Stephens, and C. Wieman, "Experimental and
theoretical study of the vapor-cell Zeeman optical trap," Phys. Rev. A 46, 4082-4090 (1992).
5. T.W. Hansch and A. L. Schawlow, "Cooling of gases by laser radiation," Opt. Commun. 13,
68-69 (1975).
8 Prelab Exercises
1. (Section 2.1)
Calculate the force on, and the acceleration of, the atoms when they are scattering photons at the
maximum rate from a laser beam. Include this result in your write-up. An atom can absorb and reemit a
photon every 2 natural lifetimes when it is in very intense laser light that is at the resonance frequency of
the atom.
2. (Section 2.2)
a) What is the purpose of the re-pumping laser? What would happen in the MOT without it? b)
Your MOT uses the 5S1/ 2 F = 2 Æ 5P3/ 2 F ¢ = 3 transition for the trapping and cooling transition and
requires a re-pumping laser for the 5S1/ 2 F = 1 Æ 5P3/ 2 F ¢ = 2 transition. What other transition scheme
might work for trapping and cooling 87Rb with two lasers? Explain.
3. (Section 3)
Calculate how large a change in the length of a 3 cm laser cavity will shift the frequency by 1 MHz.
Hint: an integer number m of half wavelengths must fit in the cavity so 3 cm = ml / 2 , and c = ln .
4. (Section 5.3)
Recall that the magnetic field is provided by two freestanding coils 1.3 cm in diameter with 25 turns
each of 24 gauge magnet wire and a separation of 3.3 cm. How much current do you need to get a
gradient of 15 G/cm? How much power? (Hint, the coils should get warm, but not burn up!).