p116 Chap01
p116 Chap01
p116 Chap01
I
Particle physics
y- ray sources 1 GeV
Particle acceleration
Fusion schemes
1020 -
1 MeV
Fig. 1.1 Progress in peak intensity since the invention of the laser in 1960.
I,. As lasers grew more powerful in the 1960s and 70s, however, (Fig. 1.1)
it became possible to consider multiphoton ionisation, expressed by the
condition
This subject actually goes much further back than most newcomers to the
femtosecond business would probably guess; predating the invention of the
laser a t the beginning of the 1960s by some margin. One of the first analy-
ses of the behavior of free electrons in the presence of intense radiation was
made by Volkov (1935), who introduced the concept of a dressed state to
describe the enhanced inertia experienced by an electron when oscillating
in an electromagnetic field. Later, motivated by the first experiments with
synchrotrons, Schwinger made a detailed analysis of the radiated power
emitted by accelerated electrons (Schwinger, 1949), pointing out that radi-
ation is preferentially emitted in the direction of motion at high energies.
These early ideas were refined and explored with more urgency when
the invention of the laser brought the prospect of an experimental means
t o study relativistic photon-electron physics in the laboratory (Brown and
Kibble, 1964; Vachaspati, 1962; EberIy and Sleeper, 1968; Sarachik and
Schappert, 1970). These authors defined the figure of merit for 'laser-
4 Short Pulse Laser Interactions with Matter
where e, m and c are the electronic charge, electron mass and speed of
light respectively; EL is the laser electric field strength and w the light
frequency. Needless to say, these theoretical works all lamented the impos-
sibility of achieving truly relativistic conditions (q > 1) with the optical
lasers available a t the time, but speculated that they might be might one
day be reached with 'future' technology. Forty years later, this wishful
thinking has become reality, and in Chapter 3 we will see how these vision-
ary models have inspired new lines of experimental investigation.
Independently of the laser's arrival, astrophysicists were beginning to
suggest mechanisms for cosmic ray generation in the vicinity of pulsars via
the interaction of intense electromagnetic (EM) radiation with free elec-
trons (Ostriker and Gunn, 1969; Gunn and Ostriker, 1971). The numbers
involved here are of course vastly different from laser-plasma interactions:
pulsar radiation has a frequency between 0.3 and 30 Hz, and magnetic field
strengths near the star surface in the region of 1012 Gauss; causing gar-
gantuan oscillation amplitudes of particles in the surrounding plasma. The
interaction physics is very similar however, and is just one of many instances
of scalable laboratory astrophyszcs, where one can emulate the conditions in
astrophysical objects using high-power lasers.
The fact that plasmas can support large-amplitude, nonlinear waves has
been known for almost as long as plasma physics established itself as a main-
stream branch of science. Early seminal works by Akhiezer and Polovin
(1956) and Dawson (1959) set the scene for numerous studies on the behav-
ior of both large-amplitude Langmuir (electrostatic) waves and the prop-
agation of high-intensity electromagnetic radiation in plasmas (Davidson,
1972). One attraction of this then rather obscure field was the tantaliz-
ing possibility of producing long-lived solitons in plasmas (Zakharov, 1972;
Decoster, 1978; Shukla et al., 1986).
The publication of a method for laser-acceleration of electrons in un-
derdense plasmas by Tajima and Dawson (1979) sparked off a fresh wave
of interest in wave propagation. This enthusiasm also encompasses mem-
bers of the accelerator community, who are actively on the look-out for
Introduction 5
The story of laser interactions with solids also has a nineteenth century
prologue. The simple observation that polished metals behave as almost
perfect reflectors, whereas other materials either absorb or transmit light,
could not be satisfactorily explained until Drude set out his 'Electron The-
ory' (Drude, 1900). Although solid state physics has advanced beyond
recognition since then, the so-called Drude model of electron conduction
still retains its appeal and usefulness in describing the main features of
metal optics (see, for example: Ashcroft and Mermin, 1976, Chapter 1).
Drude's original idea -just three years after J. J. Thomson7sdiscovery
of the electron - was t o suppose that the atoms in a metal somehow share
a limited number of 'valence' electrons, forming a conduction band. These
can wander as far as they like from their parent atoms, carrying current and
heat through the material in the process. For an element with mass density
p and atomic weight A, the free electron density is given by ne = NAZ*p/A,
where NA is Avogadro's constant and Z* is the number of valence electrons
per atom.
The conductivity of a metal will depend on the rate a t which these
free electrons are slowed due to collisions with the ions. Mathematically
this can be expressed by the relation: a, = nee2r/me,where r is the
collision or relaxation time. Even today, precise theoretical treatments to
determine the relaxation time in solids remain a challenge, since the latter
depends on details of the crystal structure, electronic configuration and so
on. For this reason, nearly all the available data on metallic conductivity
has been obtained through experimental measurements using Ohm's law:
j = a,E. This technique - applying a DC voltage and finding the
6 Short Pulse Laser Interactions with Matter
advances in the short pulse field would have been nowhere near as rapid
without the considerable prior scientific and technical knowledge of laser
science and interaction physics generated by the ICF programs over the
last 30 years. Luckily, training in ICF physics is not necessary to work
on short pulse interactions, but it is nonetheless useful to know where to
find the original literature, on, say, hydrodynamics, parametric instabilities,
energetic particle generation, and so on. A brief outline of ICF would
therefore appear to be in order, even if to mainly draw contrasts between the
new femtosecond phenomena and this long pulse regime in later chapters.
Laser fusion became official in 1972 (having previously been under mil-
itary classification) with the publication of a classic but over-optimistic
paper in Nature by Nuckolls et al., (1972). In this work, the authors de-
scribe how a small micrometer-sized pellet filled with deuterium and tri-
tium fuel can be compressed to enormous densities by irradiating it with
laser beams focused symmetrically onto its surface (Brueckner and Jorna,
1974). By converting the laser energy into thermal plasma energy, the pel-
let shell material ablates radially outwards, thus pushing the fuel inwards
via a rocket-like reaction. By virtue of the spherical symmetry, the fuel
implodes, eventually reaching densities p of several hundred g ~ m -and ~
temperatures T of 10 keV (lo7 degrees Kelvin), thus meeting the require-
ments for thermonuclear confinement encapsulated by the product:
- - Raman: em- em + 1
, '
Inverse bremsstrahlung
shall see in later chapters, nearly all of them turn up again in femtosec-
ond interactions. Parametric instabilities such as Raman and Brillouin
scattering (Kruer, 1988) are generally bad for the implosion because they
generate fast electrons. Because of their long range, these electrons preheat
the target core, making the compression less efficient. Resonance absorp-
tion (which we will meet in Sec. 5.5.1) is also undesirable for this reason: in
fact, up to 50% of the laser energy can be wasted on superheated electrons
in this way. The classic signature of such 'anomalous absorption' processes
is a bi-Maxwellian electron distribution, see Fig. 5.17. In the case of reso-
nance absorption, the hot electron component has a temperature TH given
by (Forslund et al., 1975a; Estabrook et al., 1975):
Introduction 9
Hopefully, it will be clear by now that the intention of this book is not
t o supply assembly instructions for a Terawatt laser system, but rather to
examine the physics which can be explored with the help of such a device.
The material contained in the chapters which follow is thus very much
aimed a t those researchers either physically or mentally gathered around
the target chamber (see Fig. 5.15), whose knowledge of the laser operation
consists primarily of the four magic numbers: wavelength, energy, pulse
duration and focal spot size. That said, the only way t o appreciate where
10 Short Pulse Laser Interactions with Matter
these numbers are conjured up from is to lift the lid off the box and take a
peek a t the optical wizardry inside.
'A tip for theoreticians being shown around a laser lab for the first time: resist the
temptation to fiddle with the pieces on the table - it can take several days to put right
again.
Introduction
12 Short Pulse Laser Interactions with Matter
-
sition of many electromagnetic waves (or laser modes), and is transform
limited, so that rP l / A v , where Av is the bandwidth. Clearly a large
bandwidth is essential t o generate a short pulse. Consider, for example, a
10 fs Gaussian pulse, for which A v r = 0.44. This gives Av = 4.4 x 1013 Hz,
which for a central wavelength of 800 nm, translates to:
X2
Ax = Av- = 94 nm.
C
is inserted between the crystal and back mirror, which imposes an equal but
opposite dispersion on the pulse (blue faster than red). The combination
of cavity plus dispersion-correction constitutes a highly stable and reliable
femtosecond laser, which these days can even be purchased 'off-the-shelf'.
The true art of femtosecond laser physics comes when we try to amplify
the pulse, as we shall see shortly.
The fs pulse from the oscillator typically contains just a few nJ of energy;
yet we wish to increase its power to the TW level and beyond. As already
mentioned, t o avoid damaging optical elements, the pulse must first be
stretched by a factor of lo3-lo4 or so. This is usually done with a pair
of diffraction gratings, which impose a positive chirp on the pulse, so that
longer wavelengths emerge before shorter wavelengths. Early CPA systems
(Maine et al., 1988) actually used enormous km-length optical fibres to
broaden the bandwidth via self-phase modulation. However, the stretch-
factors obtained by this method are limited because there is no practical
means of correcting the nonlinear, high-order phase distortion introduced
by the fibre, ultimately restricting the final pulse length to values of just
under 1 ps.
The stretched pulse can now be amplified - a process which is usu-
ally split into two or more stages, depending on the final beam energy
required. The Jena system comprises three different modules: a regenera-
tive preamplifier and two multipass power amplifiers. Most of the gain of
the system (- lo7) is obtained by the regenerative amplifier, which works
in a very similar fashion t o the laser resonator itself. The difference is that
it seeded by the chirped pulse, which subsequently makes up t o 20 round
trips through a low gain medium, before being switched out by a combined
Pockels cell/polarizer combination. Since the regenerative amplifier even-
tually becomes saturated a t a few mJ, additional cavity-free techniques are
then used to amplify up t o and beyond the 1 J level. The multipass con-
figuration in Fig. 1.4 is typical of modern tabletop-TW systems, producing
gains of lo2-lo3.
The amplified, long chirped pulse is then recompressed using a grating
pair (or quadruplet in the Jena system shown), ideally reducing the pulse
length back down to a value slightly above the one originally emitted by
the oscillator. Some pulse lengthening is inevitable due t o a combination of
nonlinear dispersion effects and gain-narrowing. The latter arises because
the amplifier medium preferentially enhances central wavelengths over pe-
ripheral ones, leading t o a reduction in bandwidth and hence lengthening
of pulse duration.
14 Short Pulse Laser Interactions with Matter
Fig. 1.5 Sharp end of the Jena Ti:sapphire femtosecond laser system: a focal spot of
3 pm diameter containing more than 50% of the pulse energy. The peak intensity reached
here is 4 x 1019 ~ c m - ~ .
Naturally there are variations of this generic short pulse system depend-
ing on the intended application. What I have just described is a multi-TW
system typical for a university laboratory. For a high-end user facility, of-
fering powers above 100 TW, one still has to go to one of the dedicated laser
laboratories listed in Table 1.1. On the other hand, there is also a growing
number of smaller, high-repetition-rate (kHz) systems for high throughput
applications such as x-ray sources. More recently, state-of-the-art few-cycle
(< 10 fs) lasers have opened up a new field of attosecond physics, a theme
which crops up again in Chapter 7.
As seen in the table, there are currently three or four Petawatt Nd:glass
lasers coming on line over the next two years (VULCAN has already passed
the P W mark). These will deliver focused intensities of about lo2' WcmP2
- perhaps a bit higher after some tuning and by increasing the energy -
Petawatta LLNL USA Nd:glass 1053 700 500 1300 - > loz0
VULCAN~ RAL UK Nd:glass 1053 423 410 1030 10 1.06 x 1021
P W laserC ILE Japan Nd:glass 1054 420 470 1000 30 loz0
PHELIX~ GSI Germany Nd:glass 1064 500 500 1000 - -
LULI lOOTW LULI France Ti:Sa 800 30 300 100 -
A P R 100 T W APR Japan Ti:Sa 800 2 20 100 11 2 x l0l9
HERCULES FOCUS USA Ti:Sa 800 1.2 27 45 (1) (8 x 10")
ALFA 2 FOCUS USA Ti:Sa 800 4.5 30 150 (1) (loz2)
Salle Jaune LOA France Ti:Sa 800 0.8 25 35 l0l9
Lund T W LLC Sweden Ti:Sa 800 1.0 30 30 10 > l0l9
MBI Ti:Sa MBI Germany Ti:Sa 800 0.7 35 20 > l0l9
Jena T W IoQ Germany Ti:Sa 800 1.0 80 12 3 5 x l0l9
ASTRA RAL UK Ti:Sa 800 0.5 40 12 l0l9
USP LLNL USA Ti:Sa 800 1 (10) 100 (30) 10 (100) 5 x l0l9
UHI 10 CEA France Ti:Sa 800 0.7 65 10 5 x 1019
a 1996-1999
Petawatt performance achieved on October 5, 2004.
Projected upgrade of PWM - PetaWatt Module.
Commissioned for end 2005.
16 Short Pulse Laser Interactions with Matter