1. Introduction
Recently, with the development of industry, the use of fossil fuels and the demand for personal vehicles are increasing. Therefore, the quantity of fine dust is also increasing. Most fine dust is composed of sulfates and nitrates, which cause smog and have adverse effects on human health (
Figure 1).
General dust can be observed by the naked eye and easily removed. On the other hand, fine dust has a very small particle size of 10 μm or less and is difficult to recognize visually. Hence, it cannot be removed completely without the help of a fine dust removal system [
1,
2]. Even on a clear day without smog, these fine particles can enter the respiratory tract when their concentration is high. If this occurs, the dust can be discharged through the respiratory tract depending on its size.
Once fine dust enters our body, the cells responsible for the immunity function act to remove dust and protect our body, a side effect of which is inflammation. These inflammatory reactions in the organs of our body, such as airways, lungs, cardiovascular, and brain can cause asthma, respiratory or cardiovascular diseases [
3]. In addition, fine dusts affect not only the human body but also industries and ecosystems. For industrial activities, the semiconductor and display industries are dust-sensitive areas, where only 0.1 μg of dust particles are allowed in a 30 cm × 30 cm × 30 cm space. This is because the defect rate increases when exposed to fine dust. The automobile industry may be adversely affected by the coating process, and in the case of automation equipment, malfunctions due to fine dust may occur. In addition, the visibility distances are reduced, which also hinders the operation of airplanes and passenger.
Fine dust can cause acid rain to sanitize soils and water, cause soil degradation, damage to ecosystems and other vegetation damage. Even heavy metals such as cadmium in the air can cause damage to crops, soil and aquatic organisms. In addition, when fine dust adheres to the leaves of a plant, it blocks the pores of the leaves and inhibits photosynthesis and the like, thereby delaying the growth of the crops [
4].
Nowadays, fine dust is attracting much attention. However, air pollutants are not only fine dust. Air pollutants are classified into organic pollutants, inorganic pollutants, and biological pollutants. Biological pollutants are mites, insects, etc. and their harmfulness is relatively low. Organic pollutants are typically HCHO, TVOC, and inorganic pollutants including dust, asbestos fibers, and so on. Readers may refer to
Table 1, to check air pollutants and their health effects.
In this paper, we focused on the elimination of HCHO, TVOC, which are the most harmful organic substances for the human body and focusing on fine dust. HCHO and TVOC are defined as follows:
HCHO is a flammable colorless gas with an irritating odor and is used as a sterilizing preservative. Indoors are mainly found in building materials, insulation, adhesives, household goods, chemical fiber, gas combustion, and tobacco smoke.
TVOC is a general term for organic compounds at a boiling point of 50–260 °C and consisting of benzene, toluene, ethylbenzene, xylene and styrene. The sources of TVOC are building materials, finishing materials and adhesives, cleaning supplies, cleaning agents, photocopier toners, and indoor combustion. In addition,
Table 2 shows the contamination status of fine dust, HCHO, and TVOC.
Air cleaning methods are based largely on centrifugal force using a filter and corona discharge. The dust collection efficiency using centrifugal force is low for fine particles. In addition, centrifugal force cannot be used for adhesive, corrosive, and abrasive gases, and it produces a large amount of noise. The use of a filters is uneconomical because it is necessary to replace the filter periodically. If the filter is not replaced, bacteria grow, which can also be harmful to the human body. In the case of a corona discharge, the electrode of the dust collector is made of aluminum, and the filter does not need to be replaced. When the filter is saturated, however, the electrodes cannot be collected smoothly. Therefore, the dust must be removed. To remove the collected fine dust, the electrodes are sprayed with water after disconnecting them from the power supply. This method of using a corona discharge for removing fine dust has high performance [
5,
6]. Previous studies have suggested that the optimal frequency is a very important factor for a fine dust removal system but it is difficult to understand the mechanism of fine dust removal using just the optimal frequency and its effect on polluted air [
7]. A literature survey showed that most papers focus on a fine dust monitoring system using an Arduino board and an optical sensor but these cannot solve the fine dust problem [
8,
9].
A large electrode is needed to obtain a corona discharge. To remove the fine dust rapidly [
10], this study focused on decreasing the electrode size. This paper suggests a new electrode shape with greater efficiency compared to other electrodes with the same area. To achieve better performance with the same area, the size of the electrode should be optimized. To demonstrate this, this study assessed the optimal frequency and CADR index during the fine dust removal experiments.
6. Results and Discussion
6.1. Analysis of the CADR Index
This experiment is conducted on cigarette smoke to confirm the effectiveness of the proposed D electrode. The particle attenuation ratio was obtained using Equation (17). For the initial concentration of 500m/m3, the initial attenuation is reduced to less than 30% after 60 min. On the other hand, 98% of particles decrease after 25 min after operation of the air cleaning system. The particle attenuation constant Ke (0.1564809) and the natural attenuation constant Ki (0.0037) are obtained by this experiment with this air cleaning system. By substituting in Equation (18), the CADR index can be obtained. The volume V is (4150 mm × 4330 mm × 2900 mm). The test is performed into the center of the height of 1400 mm. The following experimental results of CADR index is about 480 m3/h. To obtain a more accurate CADR index, further experiments are required in a place larger than this experimental volume.
6.2. Analysis of Changes in Air Pollution Status
The removal times of smoke, fine dust, HCHO, and TVOC were measured using the JSM-100 system. If using the instrument for a long time, odors and gases may accumulate in the instrument and affect the measurement/test result. In order to calibrate it, after the first experiment, we turn on the detector and check it in a well-ventilated place for more than one hour. Thereafter, additional experiments were repeated. In addition, the removal times were compared according to the hole size. First, the removal time of smoke, which contains large dust particles, was examined. The optimal switching frequency was determined and the optimal conditions of the other experiments were also demonstrated.
As shown in
Figure 13a, electrodes (A)–(E) are the fastest at the switching frequency of 13 kHz in removing smoke. The experiments of HCHO, TVOC, and PM
2.5 (particle material) are also performed with the switching frequency of 13 kHz in the (20 cm × 20 cm × 50 cm) acrylic box with the input DC voltage of 30 V.
Formaldehyde (HCHO) is a flammable colorless gas that has a long-lasting, irritating odor with adverse effects on the human body, such as headache/amnesia and emotional disturbances. If the HCHO density value is large than 0.30 mg/m3, the present air is not good.
Referring to
Figure 13b, the data are derived by comparing with electrodes (A)–(E). Electrode (A) showed the fastest purging. The air is purified within 3 min by the (D), (B), (C), whereas, more than 6 min is needed in case of using electrodes (A) and (E).
TVOC is a precursor of photochemical reaction and means harmful substance to the human body/environment by generating secondary pollutants, such as ozone and aldehydes. The experimental results show that it takes approximately 4 min for (D), (C), (B) models. However, it takes 7 min for (A), (C) models shown in
Figure 13c.
If the PM
2.5 concentration is greater than 101
g/m
3, the present air is not clean. The experimental results show that electrode (D) cleans the fine dust within almost 2 min. And electrodes (B) and (C) clean almost the same time (3 min) but electrode (C) cleans a little faster than electrode (B). On the other hand, the electrodes (A) and (D) clean the fine dust more than 6 min as shown in
Figure 13d.
Electrode (D) shows the excellent results under all the conditions. Referring to Equation (13), it can be seen that the larger the area of the electrode, the greater the ability to remove fine dust. However, the experiment with the largest area electrode (A) showed the worst result. Because the faster of the moving speed of gas, the higher the efficiency of dust collection. In case of electrode (A), the electrode area is the largest, but the movement speed of gas is the lowest, so the fine dust cannot be removed quickly. By adopting holes on the electrode surface, the gas is easily moved through the holes and the removal speed is increased due to the smooth movement. Based on these experimental results, it is confirmed that the gas motion speed can be controlled by the diameter of hole. In the case of too large a hole, the discharge area is narrow and it isn’t effective. On the contrary, in the case of too small a hole, the gas motion speed is slow and doesn’t give good results. From these experiments, we know that the diameter of 0.2 cm has the best fine dust removal quality. In the near future, it will be necessary to carry out the comparative experiment using a larger size electrode for practical industrial use.
6.3. Data Sets and Standard Deviation
Table 5,
Table 6,
Table 7 and
Table 8, is data sets and standard deviation. The standard deviation was obtained by using the experimental data. The standard deviation data shows that electrode (D) is the least deviating in all data. Also, referring to
Figure 13, it can be seen that electrode (A) has the lowest removal rate and the standard deviation also has the largest deviation in the whole experiment. Except for the optimum frequency experiment of Smoke, the standard deviation is (D) < (C) < (B) < (E) < (A) (removal time). In the case of the smoke experiment, the standard deviation is recorded in the order of (D) < (B) < (C) < (E) < (A) (removal time). The smoke removal experiment is to find the optimum frequency. Therefore, the closer to the optimum frequency, the faster the removal. There is not much difference in voltage when it goes away from the optimum frequency. The electrode (B) model was recorded as low when viewed only by the deviation of the electrode (C) model and the electrode (B) model. However, when comparing electrodes (B) and (C) only for each removal time, electrode (C) shows a quick removal time as a whole.