Laser and Particle Beams (2015), 33, 519–524.

© Cambridge University Press, 2015 0263-0346/15

doi:10.1017/S0263034615000609

High-intensity terahertz generation by nonlinear

frequency-mixing of lasers in plasma with DC magnetic field

ANIL K. MALIK1,2 AND KUNWAR PAL SINGH3

1
Institute of Optics, University of Rochester, Rochester, New York
2
Department of Physics, Multani Mal Modi College Modinagar, Chaudhary Charan Singh University Meerut, Uttar Pradesh, India
3
Singh Simutech Pvt. Ltd., Bharatpur, Rasasthan, India
(RECEIVED 16 March 2015; ACCEPTED 13 May 2015)

Abstract
We propose a mechanism of highly focused, tunable and high-intensity terahertz (THz) radiation generation by frequency-
mixing of two super-Gaussian lasers with frequencies ω1, ω2 and wave numbers k1, k2 (laser profile index p > 2) in a
corrugated plasma in the presence of external static magnetic field B0 ẑ. In this process, a strong nonlinear
ponderomotive force is offered to the plasma electrons at frequency ω′ = ω1 − ω2 and wave number k′ = k1 − k2 by
laser beams. The ponderomotive force results in a strong, controllable nonlinear transverse oscillatory current,
which can be optimized by optimizing the external magnetic field, ripple parameters, and laser indexes. This
controllable current produces focused and intense THz radiation of tunable frequency and power along with a
remarkable efficiency ∼25%.
Keywords: Plasma; Radiation; Ripples; Terahertz

1. INTRODUCTION suited for nonlinear optical phenomena and nonlinear spec-

troscopic measurements (Shen et al., 2007).
There is growing interest in generating high-intensity and
Different types of schemes such as THz radiations by
tunable terahertz (THz) radiations to fill the frequency gap
super-luminous laser pulse interaction with large band-gap
ranging from 0.1 to 30 THz due to their enormous applica-
semiconductors and electro-optic crystals (Faure et al.,
tions in chemical and security identification (Shen et al.,
2004; Jiang et al., 2011) have been proposed to obtain in-
2005; Zheng et al., 2006), explosive and concealed
tense and efficient THz sources. The other routes for the
weapon detection (Appleby & Wallace, 2007), pharmaceuti-
THz radiation generation include synchrotron radiation
cal quality control and medicine (Zeitler & Gladden, 2008),
from bunched electrons, transition radiation from electron
material characterization, imaging, topography, remote sens-
beams, and THz generations from air plasma filaments
ing (Ferguson & Zhang, 2002), etc. The increasing availabil-
(Hamster et al., 1994; Loffler et al., 2000; Carr et al.,
ity of high-intensity THz fields is even capable of facilitating
2002; Leemans et al., 2003; Dai et al., 2006; Thomson
the study of nonlinear phenomena (Leinß et al., 2008; Hoff-
et al., 2007). It has been reported that the efficiency of
mann et al., 2009; Hirori et al., 2010). Considerable efforts
THz generation can be enhanced if two-color laser pulses
have been made by both the laser community (Köhler
are used to create the plasma (Chen et al., 2007). This
et al., 2002; Breunig et al., 2008) and the accelerator commu-
effect has been attributed to four-wave mixing (Bartel
nity (Krafft, 2004; Byrd et al., 2006; Shen et al., 2007; Neu-
et al., 2005; Thomson et al., 2010) or temporal asymmetries
mann et al., 2009) to fill this gap. The use of lasers to
in the E fields of the pulses (Wang et al., 2013). Weiss et al.
generate THz radiation has an advantage of being compact,
(2000) have demonstrated continuous increase in THz power
but it gives limited peak power. The accelerator-based THz
from semiconductors such as GaAs and InAs with increasing
sources are capable of providing intense THz radiation
magnetic field. Malik et al. (2010; 2012) have reported the
with Mega Watt (MW) peak power and are particularly
THz generation in the process of tunnel ionization of a gas
jet by femtosecond laser pulses and laser beating in plasmas.
Address correspondence and reprint requests to: Anil K. Malik, Institute
of Optics, University of Rochester, NY 14627, USA. E-mail: anilkmalik@ A corrugated plasma channel has been proposed for better
gmail.com phase-matched THz radiation generation by the ponderomotive
519
520 A.K. Malik and K.P. Singh

force of a laser pulse (Antonsen et al., 2007; Verma & et al., 2014) to the plasma electrons at frequency ω′ = ω1 −
Sharma, 2009; Varshney et al., 2014). In most of the ω2 and wave number k′ = k1 − k2, which is obtained as
schemes, the magnetic field has proved to be effective for en-
hancing the field of emitted radiations (McLaughlin et al.,
fω′ NL = − e2
2 )∗

1 · E
(∇E
2000; Weiss et al., 2000; Wu et al., 2007). 2me ω1 ω2
It can be observed that most of the THz radiation genera-

e2 E01 E02 4py2p−1 (1)
tion schemes produce either lower average output power =− x̂ik ′ − ŷ
2me ω1 ω2 w2p
(sensitivity) or emit poorly focused radiations. Actually tun- 0

/w0 2p )) i(k ′ x−ω′ t)

able and intense THz radiation with its optimal focusing and × e(−(2y
2p
e ,
collimation has not been realized so far. In the present paper,
we show that all these properties can be achieved simultane- where me is the mass of electron. In the presence of a nonlin-
ear ponderomotive force
fω′ and the static magnetic field
ously if we generate such radiations through nonlinear NL

frequency-mixing of super-Gaussian (spatial) lasers and B0 ẑ, we (Malik et al., 2014) calculate nonlinear density per-
employ an external DC magnetic field in a corrugated (den- turbation (say, nω′ NL ) using equation of continuity and equa-
sity) plasma. Owing to the higher index of the lasers and tion of motion as
hence, an enhancement in the steepness in their spatial inten-
sity gradient, a stronger transverse ponderomotive force is re-   
me c2 n0 ′

NL
·
f ′ NL × eB0 ẑ .
alized which drives a very high nonlinear current. This nω′ NL = iω ∇ · f ω′ + ∇ ω
iω′ (m2e c2 ω′ 2 − e2 B20 ) me c
strong, controllable nonlinear oscillatory current is the
(2)
source for generating THz radiation with tunable frequency,
power and focusing properties.
This nonlinear density perturbation produces a self-consistent
The organization of the paper is as follows. In Section 2,
space-charge potential f that leads to a linear density
we give analytical results of the electric field and efficiency
perturbation nω′ L using which we calculate using Piosson’s
of the emitted radiation due to nonlinear oscillatory current
equation as
developed as a result of frequency-mixing of two super-
Gaussian lasers of frequencies ω1, ω2 and wave numbers 

· ∇f
m2e c2 ω2p ∇
′
k1, k2 (profile index p > 2). Results and discussion are ω
nω′ L =
.
given in Section 3. Conclusions of the present paper are en- 4πe m2e c2 ω′ 2 − e2 B20
capsulated in Section 4.
Using equation of motion as


me ∂
vω′ NL /∂t =
fω′ +
fω′ − e
vω′ NL × B

0 under the com-
NL L
2. THZ RADIATION FIELD AND EFFICIENCY
NL L

′ and magnetic field B0 ẑ,
bined effect of
fω′ ,
fω′ = e∇f
Figure 1 shows the schematic for the THz generation scheme ω

in the corrugated plasma. We consider frequency-mixing of we calculate the nonlinear velocity of the electrons
vω′ NL as
two super-Gaussian lasers (beam width w0 and the general-
ized profile index p) with frequencies ω1 and ω2 and wave e2 E01 E02 e(−(2y /w0 )) [T1 x̂ + T2 ŷ]ei(k x−ω t)
2p 2p ′ ′

vectors k1 and k2, linearly polarized along the y-direction
vω′ NL = − , (3)
2m2e ω1 ω2 (ω′ 2 − ω2c )(ω′ 2 − ω2H )
[pump fields profile E
j = ŷE0j e(y2p /w0 2p ) ei(kj x−ωj t) together
with j = 1, 2], and co-propagating along the x-direction in
a corrugated plasma having density n = n0 + n′ (n′ = nα where ωc = eB0/mec,
eiαx together with nα as the amplitude and α as the wave
⎡  ⎤
number of the corrugation) under the effect of magnetic field

ω′ 2 ω′ 2 − ω2c + ω2c ω2p 4py
2p−1
ωc ω′ 2 + ω2p − ω2c
B0 ẑ. T1 = ⎣ + ⎦
The spatial gradient in the laser intensities offers a strong c w2p
0
nonlinear ponderomotive force (Malik & Malik, 2013; Malik

and
⎡  ⎤


iω′ ωc ω′ 2 + ω2p − ω2c 4py2p−1 ω′ 2 ω′ 2 − ω2c + ω2c ω2p
T2 = ⎣ − ⎦,
c iω′ w0 2p


together with ωH = ω2p + ω2c . The nonlinear current



Jω ≡ −(1/2)n′ e
vω′ NL comprises the contribution from non-
Fig. 1. Schematic representation for the THz generation in the corrugated
plasma. linear perturbations in the electron density nω′ NL and linear
High-intensity THz generation in the plasma with DC magnetic field 521
$ $
density perturbation nω′ L due to the self-consistent space- $ E0y $
$ $
charge potential f produced by nω′ NL. Hence, the current den- $E $
01
sity
$ ⎡⎧  ⎫
 ⎤$$
Jω is obtained as $ ⎨inα eω2p E02 ω2 (ω2−ω2c )+ωc 2 ω2p ⎬ 4pyp−1
$ ω ω 2 $
$ ⎢   − 2 2 ⎥
c p $
$ ⎢⎩ ⎭ c(ω −ωH ) ⎥$$ ⎥
$ x ⎢ 4n0 me c ω1 ω2 (ω −ωH ) ω −ωc
2 2 2 2 2 w 0
p

Jω = − nα e3 E01 E02 $ ⎢  ⎫ ⎥$

e−(2y /w0 2p ) =$ ⎢ ⎧
2p
⎥ $
4me ω1 ω2 (ω 2 − ω2c )(ω 2
2 − ω2H ) $2k⎢ ⎨ in eE ω ωω2 ω2+ω2−ω2 ⎬
⎥$
(4) $ ⎢ α 02 c ω 4py ωc ωp ⎥$
p−1 2
$ ⎣+ p

p c
 − ⎦$
× {x̂T1 − iŷT2 } ei(kx−ωt) . $ ⎩4n0 me c2 ω1 ω2 (ω2−ω2H ) ω2−ω2c ⎭ c w0 p ω(ω2−ω2H ) $$
$

× e(−2y /w0 2q )
2p
.
Here ω ≡ ω′ = ω1 − ω2 and
k =
k1 −
k2 + α

.
(7)
We calculate the THz field using Maxwell’s equations
along with the current
Jω as Here
"   #

∇
+ 4πiω
Jω − ω εE

· E)
2

− ∇2 E

= 0. ω2 εxy 2
∇( (5) ε yy + − k 2
=0
c2 c2 c2 εxx

In the presence of magnetic field, the electric permittivity of is a required phase-matching condition for maximum mo-
the plasma evolves into a tensor quantity ε with its compo- mentum transfer from the lasers to the plasma electrons.
nents as From Eq. (7), it is observed that the resonant emission of

THz radiations is achieved at ω ≈ ωH ≡ ω2p + ω2c . Since
ω2p kTHz ≠ k′ , a proper tuning of these wave numbers is also
εxx = εyy = 1 − ,
(ω2 − ω2c ) required for the resonant excitation of the THz radiation.
This tuning is achieved with the help of corrugation
iωc ω2p (wave number α) in the plasma density (as
k = α
+
k′ ), peri-
εyx = −εxy = , odicity (repetition) of which can be obtained from the phase
ω(ω2 − ω2c )
matching condition as
$ $
$2π$ 2πc
ω2p |λcorru | = $$ $$ = ⎧ %⎫ .
εzz = 1 − 2 , α ⎪ & 2 ⎪
⎪ &
ω ⎨ & ω2 − ω2p − ω2 ω2c ⎪ ⎬
ω− '
⎪
⎪ ω2 − ω2p − ω2c ⎪ ⎪
and εxz = εzx = εzy = εyz = 0. Equation (5) governs the THz ⎩ ⎭
radiation emission. Assuming fast phase variation of the field

we put E
E,
=E
0 (x, y) ei(kx−ωt) in Eq. (5) and separate out the The dependence of λcorru on ωc reveals that the magnetic field
x-and y-components of E.
The normalized transverse compo- plays a vital role in realizing the resonant/phase-matched ex-


nent of E gives the THz field E0y as citation of the THz radiation at the frequency ω ≅ ωH by
photo-mixing of the lasers.
    Finally, we calculate ηω as the ratio of average energy den-
∂2 E0y ∂E0y ω2 ε2xy
+2ik + 2 εyy + −k E0y
2 sities of the emitted THz radiation to that of the input lasers
∂x2 ∂x c εxx and that of the emitted THz radiation as follows (Rothwell &
⎡⎧   ⎫
⎤ Cloud, 2009):
⎨ inα eω2p E02 ω2 (ω2 −ω2c )+ω2c ω2p ⎬ 4pyp−1 ω ω 2 ⎡ ⎤
⎢ c ⎥
⎢ ⎩4n m c2 ω ω (ω2 −ω2 )ω2 −ω2 ⎭ w p − c(ω2 −ω2 ) ⎥
p
⎢ 0 e 1 2 0 ⎥ px2 2(1/2p) ℜ1 2 ⎢ 2
ω2 ℜ3 2 ⎥
⎢ 
H c
⎫

H
⎥ ⎢ 8pℜ2 ⎥
=⎢ ⎧  ⎥ ηω = ⎢ 2 (4−1/p) Γ(2 − 1/2p) + Γ(1/2p)⎥,
⎢ ⎨ in eE ω 2 ω2 +ω2 −ω2 ⎬ ⎥ 4k Γ(1/2p) ⎣w0 2
2 1 ⎦
⎢ α 02 c p p c ω 4py ωc ωp ⎥
p−1 2
⎣+   − ⎦ 4pc2 22p
⎩4n0 me c2 ω1 ω2 (ω2 −ω2H ) ω2 −ω2c ⎭ c w0 p ω(ω2 −ω2H )
(8)
× e(−2y /w0 )
2p 2q
where
(6)
nα eωω2p E02
ℜ1 =  ,
In order to solve Eq. (6), we neglect second-order term 4n0 mc2 ω 1 ω2 (ω
2 − ω2H ) ω2 − ω2c
and put
  
"   # ω2 (ω2 − ω2c ) + ω2c ω2p ω2c ω2p ω2 + ω2p − ω2c
ω2
εxy 2

ε + −k 2
=0. ℜ2 = + ,
c2
yy
εxx ω ω ω2 − ω2H
522 A.K. Malik and K.P. Singh

and Figure 3 shows that the THz field amplitude attains a maxi-
  mum value at a particular value of y/w0. For example, the
ωc ω2p ω2 (ω2 − ω2c ) + ω2c ω2p  THz radiation is focused at y/w0 = 0.72 in the case of super-
ℜ3 =
 − ωc ω2 + ω2p − ω2c , Gaussian lasers of index 2 ( p = 2), at y/w0 = 0.84 in the case
ω ω − ωH
2 2 2
of lasers of index 3 and at y/w0 = 0.89 in the case of lasers of
index 4. Moreover, the transverse profile becomes more sym-
where Γ is the usual gamma function.
metrical about the y-axis for the case of higher index lasers
and peak value of the THz field amplitude is increased
3. RESULTS AND DISCUSSION with laser index p. The peak field and the collimation of
the emitted radiation are further enhanced by increasing mag-
The steep corrugations in the density that are constituted at
netic field. The effect of magnetic field becomes more impor-
closer distances are suggested for obtaining strong THz radi- tant for the higher index lasers, where we can obtain the
ation (Antonsen et al., 2007). Equation (7) shows that the ra-
radiation of highest intensity at a desired position by chang-
diation with larger field is obtained for the case of higher
ing the index. This is attributed to the higher cyclotron
amplitude corrugation (higher nα). This is attributed to the motion of the electrons in the presence of stronger magnetic
more number of electrons which contribute to excitation of
field.
the strong nonlinear current
Jω .
Equation (8) shows that the present scheme of frequency-
Figure 2 shows that the THz amplitude is highest for ω/ mixing of two super-Gaussian lasers is very effective, where
ωP ≈ 1.3, that is, near the resonance condition ω ≈ ωH.
the efficiency of about 0.25 can be obtained (Fig. 4) if a com-
Moreover, the role of index (parameter p) of super-Gaussian
bination of the lasers of higher index and a strong magnetic
lasers in getting stronger radiation is evident from the figure, field is used. It can be inferred from the comparison of
where higher THz field amplitude is obtained for the higher
Figure 4 with Figures 2 and 3 that in the situation of
index. Actually for the higher index lasers, a stronger nonlin-
higher efficiency, the THz radiation field is stronger and
ear current J
ω is realized due to the stronger force
fω′ in the
NL
more focused. This is evident from all the figures that
presence of sharp gradient in the lasers’ intensity. This gradi- unlike other investigators (Carr et al., 2002; Wu et al.,
ent is higher in the case of lasers with smaller beamwidth 2007; 2008; Kim et al., 2008), we can get the THz radiation
(w0). Hence, the THz field of higher amplitude is achieved at a desired position along with its tunable power and fre-
when the lasers of smaller w0 are used (Fig. 2). A point to quency with the application of an external magnetic field
be noted in the present scheme is that the THz field and proper choice of index of the super-Gaussian lasers.
∼107 V/cm for the laser intensity ∼1014 W/cm2 is higher Jiang et al. (2011) demonstrated a scheme of THz generation
than the field obtained in other schemes (Hamster et al., scheme based on difference frequency generation by stacking
1994; Loffler et al., 2000; Jiang et al., 2011; Malik & the GaP plates. In their scheme, the conversion efficiency is
Malik, 2011; Carr et al., 2002; Leemans et al., 2003; Dai comparable with our model, but the emitted THz field is
et al., 2006; Chen et al., 2007; Thomson et al., 2007; Wu much lower than the emitted field in the proposed model.
et al., 2007; 2008; Kim et al., 2008). Wu et al. reported a scheme of THz generation from the
The most striking feature of the proposed photo-mixing laser wake-field in the inhomogeneous magnetized plasma
scheme is the tuning of power and focus (transverse profile: in which conversion efficiency of the THz radiation is pro-
y/w0) of the emitted THz radiation with the help of index of portional to the laser intensity when it is less than 1018 W/
the lasers and magnetic field. In this regard, it is clear from cm2 and it reaches about 10−5 when the intensity of the
laser is approximately 1019 W/cm2 (Wu et al., 2007). Kim

Fig. 2. Variation of the normalized peak THz electric field with index (pa- Fig. 3. Transverse profile ( y/w0) of the THz radiation with as a function of
rameter p) of the lasers and beamwidth (w0), when x = 100c/ωp, ω1 = 2.4 × magnetic field (B0) and the index of laser beams, when w0 = 0.05 mm, x =
1014 rad/s, ωp = 2 × 1013 rad/s, ωc/ωp = 0.2, nα/n0 = 0.2, y/w0 ≈ 0.7, and 100c/ωp, ω$ 1 ∗=$ 2.4 × 10 rad/s, ωp = 2 × 10 rad/s, nα/n0 = 0.1, ω/ωp =
14 13
$ ∗$
$
v2 $ = 0.3c. $
$
1.45, and v2 = 0.3c.
High-intensity THz generation in the plasma with DC magnetic field 523

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ACKNOWLEDGEMENTS
source. Phys. Rev. ST Accel. Beams 7, 060704.
The author, Anil K. Malik acknowledges UGC support for provid- LEEMANS, W.P., GEDDES, C.G.R., FAURE, J., TÓTH, C., TILBORG, J.V.,
ing Raman Post Doctoral Fellowship to conduct the research at the SCHROEDER, C.B., ESAREY, E., FUBIANI, G., AUERBACH, D., MARCE-
Institute of Optics, University of Rochester, Rochester, USA. LIS, B., CARNAHAN, M.A., KAINDL, R.A., BYRD, J. & MARTIN,
M.C. (2003). Observation of terahertz emission from a laser–-
plasma accelerated electron bunch crossing a plasma-vacuum
boundary. Phys. Rev. Lett. 91, 074802.
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