Abstract
The even-denominator fractional quantum Hall state at a filling factor of νâ=â1/2 is an intriguing many-body phase in two-dimensional electron systems, as it appears in the ground state rather than an excited Landau level. It is observed in wide quantum wells where the electrons have a bilayer charge distribution with finite tunnelling between the layers. Whether this state takes an Abelian two-component form or a non-Abelian one-component form has been debated since its experimental discovery. Here we report the observation of the νâ=â1/2 state that is flanked by numerous Jain-sequence composite fermion states at νâ=âp/(2pâ±â1) up to νâ=â8/17 and 9/17. As we raise the density, the νâ=â1/2 state is strengthened, its energy gap increases up to 4âK and, at the same time, the 8/17 and 7/13 states abruptly become stronger than their neighbouring high-order fractions. The states at νâ=â8/17 and 7/13 are the theoretically predicted, simplest daughter states of the one-component Pfaffian νâ=â1/2 state. This means that our data suggest a topological phase transition of 8/17 and 7/13 states from the Jain-sequence states to the daughter states of the Pfaffian.
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Data availability
The data that support the plots within this paper and other findings of this study are available from the corresponding authors upon reasonable request. Source data are provided with this paper.
References
Nayak, C., Simon, S. H., Stern, A., Freedman, M. & Sarma, S. D. Non-Abelian anyons and topological quantum computation. Rev. Mod. Phys. 80, 1083â1159 (2008).
Willett, R. et al. Observation of an even-denominator quantum number in the fractional quantum Hall effect. Phys. Rev. Lett. 59, 1776â1779 (1987).
Moore, G. & Read, N. Nonabelions in the fractional quantum Hall effect. Nucl. Phys. B 360, 362â396 (1991).
Read, N. & Green, D. Paired states of fermions in two dimensions with breaking of parity and time-reversal symmetries and the fractional quantum Hall effect. Phys. Rev. B 61, 10267â10297 (2000).
Ki, D. K., Falâko, V. I., Abanin, D. A. & Morpurgo, A. F. Observation of even denominator fractional quantum Hall effect in suspended bilayer graphene. Nano Lett. 14, 2135â2139 (2014).
Falson, J. et al. Even-denominator fractional quantum Hall physics in ZnO. Nat. Phys. 11, 347â351 (2015).
Li, J. I. A. et al. Even-denominator fractional quantum Hall states in bilayer graphene. Science 358, 648â652 (2017).
Zibrov, A. A. et al. Tunable interacting composite fermion phases in a half-filled bilayer-graphene Landau level. Nature 549, 360â364 (2017).
Hossain, M. S. et al. Unconventional anisotropic even-denominator fractional quantum Hall state in a system with mass anisotropy. Phys. Rev. Lett. 121, 256601 (2018).
Shi, Q. et al. Odd- and even-denominator fractional quantum Hall states in monolayer WSe2. Nat. Nanotechnol. 15, 569â573 (2020).
Dutta, B. et al. Distinguishing between non-Abelian topological orders in a quantum Hall system. Science 375, 193â197 (2022).
Huang, K. et al. Valley isospin controlled fractional quantum Hall states in bilayer graphene. Phys. Rev. X 12, 031019 (2022); erratum 12, 049901 (2022).
Willett, R. L. et al. Interference measurements of non-Abelian e/4 & Abelian e/2 quasiparticle braiding. Phys. Rev. X 13, 011028 (2023).
Jain, J. K. Composite Fermions (Cambridge Univ. Press, 2007).
Suen, Y. W., Engel, L. W., Santos, M. B., Shayegan, M. & Tsui, D. C. Observation of a νâ=â1/2 fractional quantum Hall state in a double-layer electron system. Phys. Rev. Lett. 68, 1379â1382 (1992).
Eisenstein, J. P., Boebinger, G. S., Pfeiffer, L. N., West, K. W. & He, S. New fractional quantum Hall state in double-layer two-dimensional electron systems. Phys. Rev. Lett. 68, 1383â1386 (1992).
He, S., Das Sarma, S. & Xie, X. C. Quantized Hall effect and quantum phase transitions in coupled two-layer electron systems. Phys. Rev. B 47, 4394â4412 (1993).
Halperin, B. I. Theory of the quantized Hall conductance. Helv. Phys. Acta 56, 75â102 (1983).
Greiter, M., Wen, X. G. & Wilczek, F. Paired Hall states in double-layer electron systems. Phys. Rev. B 46, 9586â9589 (1992).
Greiter, M., Wen, X. G. & Wilczek, F. Paired Hall states. Nucl. Phys. B 374, 567â614 (1992).
Suen, Y. W., Manoharan, H. C., Ying, X., Santos, M. B. & Shayegan, M. Origin of the νâ=â1/2 fractional quantum Hall state in wide single quantum wells. Phys. Rev. Lett. 72, 3405â3408 (1994).
Shabani, J. et al. Phase diagrams for the stability of the νâ=â1/2 fractional quantum Hall effect in electron systems confined to symmetric, wide GaAs quantum wells. Phys. Rev. B 88, 245413 (2013).
Peterson, M. R. & Sarma, S. D. Quantum Hall phase diagram of half-filled bilayers in the lowest and the second orbital Landau levels: Abelian versus non-Abelian incompressible fractional quantum Hall states. Phys. Rev. B 81, 165304 (2010).
Thiebaut, N., Regnault, N. & Goerbig, M. O. Fractional quantum Hall states versus Wigner crystals in wide quantum wells in the half-filled lowest and second Landau levels. Phys. Rev. B 92, 245401 (2015).
Mueed, M. A. et al. Geometric resonance of composite fermions near the νâ=â1/2 fractional quantum Hall state. Phys. Rev. Lett. 114, 236406 (2015).
Mueed, M. A. et al. Geometric resonance of composite fermions near bilayer quantum Hall states. Phys. Rev. Lett. 117, 246801 (2016).
Zhu, W., Liu, Z., Haldane, F. D. M. & Sheng, D. N. Fractional quantum Hall bilayers at half filling: tunneling-driven non-Abelian phase. Phys. Rev. B 94, 245147 (2016).
Sharma, A., Balram, A. C. & Jain, J. K. Composite-fermion pairing at half-filled and quarter-filled lowest Landau level. Phys. Rev. B 109, 035306 (2024).
Suen, Y. W. et al. Missing integral quantum Hall effect in a wide single quantum well. Phys. Rev. B 44, 5947â5950 (1991).
Manoharan, H. C., Suen, Y. W., Santos, M. B. & Shayegan, M. Evidence for a bilayer quantum Wigner solid. Phys. Rev. Lett. 77, 1813â1816 (1996).
Shayegan, M., Manoharan, H. C., Suen, Y. W., Lay, T. S. & Santos, M. B. Correlated bilayer electron states. Semicond. Sci. Technol. 11, 1539â1545 (1996).
Hatke, A. T. et al. Microwave spectroscopic observation of a Wigner solid within the νâ=â1/2 fractional quantum Hall effect. Phys. Rev. B 95, 045417 (2017).
Halperin, B. I. Theories for νâ=â1/2 in single- and double-layer systems. Surf. Sci. 305, 1â7 (1994).
Chung, Y. J. et al. Ultra-high-quality two-dimensional electron systems. Nat. Mater. 20, 632â637 (2021).
Levin, M. & Halperin, B. I. Collective states of non-Abelian quasiparticles in a magnetic field. Phys. Rev. B 79, 205301 (2009).
Wen, X. G. Topological orders and edge excitations in fractional quantum Hall states. Adv. Phys. 44, 405â473 (1995).
Kumar, A., Csáthy, G. A., Manfra, M. J., Pfeiffer, L. N. & West, K. W. Nonconventional odd-denominator fractional quantum Hall states in the second Landau level. Phys. Rev. Lett. 105, 246808 (2010).
Halperin, B. I., Lee, P. A. & Read, N. Theory of the half-filled Landau level. Phys. Rev. B 47, 7312â7343 (1993).
Du, R. R., Stormer, H. L., Tsui, D. C., Pfeiffer, L. N. & West, K. W. Experimental evidence for new particles in the fractional quantum Hall effect. Phys. Rev. Lett. 70, 2944â2947 (1993).
Manoharan, H. C., Shayegan, M. & Klepper, S. J. Signatures of a novel Fermi liquid in a two-dimensional composite particle metal. Phys. Rev. Lett. 73, 3270â3273 (1994).
Villegas Rosales, K. A. et al. Fractional quantum Hall effect energy gaps: role of electron layer thickness. Phys. Rev. Lett. 127, 056801 (2021).
Zhao, T., Kudo, K., Faugno, W. N., Balram, A. C. & Jain, J. K. Revisiting excitation gaps in the fractional quantum Hall effect. Phys. Rev. B 105, 205147 (2022).
Lay, T. S., Jungwirth, T., SmrÄka, L. & Shayegan, M. One-component to two-component transition of the νâ=â2/3 fractional quantum Hall effect in a wide quantum well induced by an in-plane magnetic field. Phys. Rev. B 56, R7092âR7095 (1997).
Hasdemir, S. et al. νâ=â1/2 fractional quantum Hall effect in tilted magnetic fields. Phys. Rev. B 91, 045113 (2015).
Assouline, A. et al. Energy gap of the even-denominator fractional quantum Hall state in bilayer graphene. Phys. Rev. Lett. 132, 046603 (2024).
Hu, Y. et al. High-resolution tunneling spectroscopy of fractional quantum Hall states. Preprint at https://arxiv.org/abs/2308.05789 (2023).
Acknowledgements
We acknowledge support by the US Department of Energy (DOE) Basic Energy Sciences via grant no. DEFG02-00-ER45841 for measurements, the National Science Foundation (NSF) grant nos. DMR 2104771 and ECCS 1906253 for sample characterization and the Eric and Wendy Schmidt Transformative Technology Fund for sample fabrication. The Princeton University portion of this research is funded in part by the Gordon and Betty Moore Foundationâs EPiQS Initiative, grant GBMF9615.01, to L.N.P. Our measurements were partly performed at the National High Magnetic Field Laboratory (NHMFL), which is supported by the NSF Cooperative Agreement no. DMR 1644779, by the State of Florida, and by the DOE. This research is funded in part by QuantEmX grant from the Institute for Complex Adaptive Matter and the Gordon and Betty Moore Foundation through grant GBMF9616 to S.K.S., C.W., A.G., C.T.T. and C.S.C. We thank R. Nowell, G. Jones, A. Bangura and T. Murphy at NHMFL for technical assistance, and B. I. Halperin, J. K. Jain, P. Kumar, M. Levin and X.-G. Wen for illuminating discussions.
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S.K.S. and M.S. conceived the work. S.K.S., C.W., C.T.T. and C.S.C. performed the low-temperature transport measurements. S.K.S. and K.W.B. fabricated the sample. L.N.P., K.W.B. and A.G. produced the molecular-beam epitaxy samples and characterized them. S.K.S. and M.S. analysed the data and wrote the manuscript with input from all co-authors.
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Extended data
Extended Data Fig. 1 Evolution of the ground state at νâ=â1/2 in wide GaAs QWs.
a, Longitudinal resistance (Rxx) of 2D electrons confined to a 48-nm-wide GaAs QW shows the evolution from a compressible composite fermion Fermi sea to an incompressible phase, the 1/2 FQHS, as the 2D electron density is raised symmetrically. Except for the bottom trace, the traces are offset vertically for clarity. The 1/2 FQHS becomes stronger as the density is raised within an intermediate density range as evinced by the Rxx minimum at νâ=â1/2 getting deeper and eventually touching zero. The top trace shows the Hall resistance (Rxy) for nâ=â3.42âÃâ1011 cmâ2. Also noteworthy is that the numerous odd-denominator FQHSs at the lowest density nâ=â2.80 are also present together with the strong 1/2 FQHS at higher densities. The relative strengths of the odd-denominator FQHSs suggest that these are the usual Jain-sequence states at all densities. The inset shows the self-consistently calculated charge distribution for 2.80 (black) and 3.26âÃâ1011 cmâ2 (green). b, Experimentally determined phase diagram depicting the phase boundaries between the composite fermion Fermi sea and the 1/2 FQHS, and the 1/2 FQHS and insulating phase, by dashed and dotted lines, respectively. The 1/2 FQHS is stable for an intermediate density range, and is sandwiched between the compressible composite fermion Fermi sea at low densities and the incompressible insulating phase at high densities. Within the intermediate density range, as the density is increased away from the compressible boundary, the 1/2 FQHS gets stronger, but eventually begins to weaken as the nearby insulating phase begins to engulf it; see Ref. 22 for details. Figure reproduced with permission from ref. 22, APS.
Extended Data Fig. 2 Evolution of an electron system in a 70-nm-wide GaAs QW with varying density.
a,b, Longitudinal (Rxx) and Hall resistance (Rxy) as a function of 1/ν in a 70-nm-wide GaAs QW. Traces are offset vertically for clarity. Rxx for the lowest density nâ=â1.09 shows a compressible νâ=â1/2 composite fermion Fermi sea, with the characteristic Jain-sequence states up to νâ=â10/19 and 9/19 on its flanks. Note that the Rxx minima at νâ=â8/17 and 7/13 are strong, but their strength relative to other, nearby FQHSs is consistent with what is expected for Jain-sequence states. As the density is increased, the compressible composite fermion Fermi sea makes a transition into an incompressible FQHS at νâ=â1/2, which gets stronger as the density is further raised. The odd-denominator FQHSs flanking the 1/2 FQHS undergo a similar evolution as displayed in Fig. 1e, where the Jain-sequence states get weaker because of the increased electron layer thickness, but the 8/17 and 7/13 FQHSs suddenly transition into anomalously strong FQHSs, distinct from Jain-sequence states. Quantitatively, owing to the smaller well width, the transitions of the νâ=â8/17 and 7/13 FQHSs are both shifted to higher densities compared to the 72.5-nm-wide sample of Fig. 1. In panel b, self-consistently calculated charge distributions for a 2DES confined to a 70-nm-wide GaAs QW at nâ=â1.24 and 1.60âÃâ1011 cmâ2 are shown as bottom and top insets, respectively.
Extended Data Fig. 3 Evolution of an electron system in a 70-nm-wide GaAs QW with in-plane magnetic field.
a,b, Longitudinal (Rxx) and Hall (Rxy) resistances are shown as a function of 1/ν at various tilt angles for nâ=â1.24âÃâ1011 cmâ2. Qualitatively, once again the sample shows a similar evolution of FQHSs at and around νâ=â1/2 as the 72.5-nm-wide sample, albeit at higher tilt angles.
Extended Data Fig. 4 Longitudinal (Rxx) and Hall resistance (Rxy) as a function of perpendicular magnetic field for ultrahigh quality 2D electrons in a 72.5-nm-wide GaAs QW.
The strong FQHS observed at νâ=â1/2 and flanked by numerous high-order Jain-sequence FQHSs up to νâ=â9/19 and 10/19 (as shown in the top right inset) on its sides attest to the ultra high quality of our sample. Top left inset shows the self-consistently calculated charge distribution for nâ=â1.16âÃâ1011 cmâ2 electrons confined to a 72.5-nm-wide GaAs QW.
Extended Data Fig. 5 Arrhenius plots to extract the energy gaps of FQHSs in the N = 0 LL for nâ=â1.17.
a-c, Temperature dependence of Rxx minima for the FQHSs on the low-field side of νâ=â1/2, at νâ=â1/2, and on the high-field side of νâ=â1/2, respectively. The red lines through the data points are fits to the data points in the activated regimes for different fillings, and their slopes yield the energy gaps Îν, determined from \({R}_{xx}\propto {e}^{-{\Delta }_{\nu }/2kT}\). Note in panel a that the νâ=â7/13 FQHS is weaker than the 6/11 FQHS and has a smaller energy gap. The activated behavior of Rxx at the different FQHSs allows us to extract an energy gap, but one must be careful with the energy gaps of the weakest FQHSs which mostly serve as a measure of their strength. Because of the limited available temperature range and the effect of disorder, the small energy gaps of the higher-order FQHSs have a large error bar.
Extended Data Fig. 6 Arrhenius plots to extract the energy gaps of FQHSs in the Nâ=â0 LL for nâ=â1.35.
Data are for the 72.5-nm-wide GaAs QW with nâ=â1.35âÃâ1011 cmâ2. a-c, Temperature dependence of Rxx minima for the FQHSs on the low-field side of νâ=â1/2, at νâ=â1/2, and on the high-field side of νâ=â1/2, respectively. The red lines through the data points are fits to the data points in the activated regimes for different fillings, and their slopes yield the energy gaps Îν, determined from \({R}_{xx}\propto {e}^{-{\Delta }_{\nu }/2kT}\). Note in panel a that, at this density, the 7/13 FQHS has a larger gap than the 6/11 FQHS. On the high-field side of νâ=â1/2 (panel c), only the νâ=â8/17 FQHS yields an activation, and the other FQHSs at higher fields are consumed by the ensuing insulating phase; see Fig. 1e of main text.
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Singh, S.K., Wang, C., Tai, C.T. et al. Topological phase transition between Jain states and daughter states of the νâ=â1/2 fractional quantum Hall state. Nat. Phys. 20, 1247â1252 (2024). https://doi.org/10.1038/s41567-024-02517-w
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DOI: https://doi.org/10.1038/s41567-024-02517-w