FIRAS
FIRAS
FIRAS
ABSTRACT
Cross sections for inelastic electron scattering and energy distributions of Ml and E2 strengths of
K = l+ excitations in titanium, rare-earth, and actinide nuclei are studied microscopically within
QRPA. The spin Ml strength has two peaks, isoscalar and isovector, residing between the low- and
high-energy orbital Ml strength. The latter is strongly fragmented and lies in the region of the
IVGQR, where the (e, e) cross sections are almost one order of magnitude larger for E2 than for Ml
excitations. Comparison with the quantized isovector rotor allows the interpretation of all the orbital
Ml excitations at both low and high energies as manifestation of the collective scissors mode.
KEYWORDS
Ml excitations in deformed nuclei, cross sections for inelastic electron scattering, energy distribution
of Ml (spin and orbital) and E2 strengths, quantized isovector rotor, scissors mode, isovector giant
quadrupole resonance, quasiparticle random-phase approximation.
GENERAL
FEATURES
AND
INTERPRETATION
PROBLEMS
Magnetic monopole excitations are strictly forbidden because of the nonexistence of magnetic charge.
Thus, the strongest magnetic excitations, i. e. those with lowest multipolarity, are magnetic dipole
(Ml) excitations. They have been extensively studied in the past mainly in spherical nuclei through
inelastic electron scattering at backward angles, see e. g. the review article of Raman et al. (1991).
Recent experiments use also polarized tagged photons (Laszewski et al., 1988) and polarized protons
(Lisantti et al., 1991).
Some general features of the Ml excitations can be easily understood by examining the Ml operator,
which consists of orbital and spin parts:
MI =
&
gf = 0.7gf(free),
gi(free) = 5.5855,
(1)
where gi, g: are the spin gyromagnetic factors for protons and neutrons. A particle-hole Ml excitation
involves the transition matrix element of the Ml operator (1) b etween two different single-particle
* Supported by the Deutsche Forschungsgemeinschaft.
** Permanent address: Institute for Nuclear Research and Nuclear Energy, Bulgarian Academy of
Sciences, BG-1784, Sofia, Bulgaria. E-mail: nojarov@mailserv.zdv.uni-tuebingen.de
297
R.
298
states.
In a spherical
matrix
elements
basis
they
rules
AN
matrix
= 0, An
elements
transitions,
but
peak,
= 0, Ae = 0, Aj
one should
g; - g: = 9.4 relative
In addition
mainly
Ml
are present
isovector
obeys in a spherical
2n + L. It has,
elements
Ml
of the orbital
in spherical
strength
is dominated
predominantly
by Morpurgo
spin transitions
with 1K
= l+l
are spin-flip
momentum
L are
by spin contributions
to the
spin gyromagnetic
ratio
(1958).
between
become
are
non-vanishing
= 1. These
angular
nuclei
elements
therefore,
excitations
J whose transition
the matrix
to gi - gz = I, as noticed
to these
orbital
stronger
elements.
momentum
the orbital
N =
where
partners
contributions
Such orbital
Ml transition
that
angular
Thus,
The Ml operator
= 0, fl,
spin-orbit
note
of the total
symmetry.
and out-of-phase.
only between
not vanishing.
Ml
are eigenstates
Nojarov
two different
possible
j-shells,
in deformed
nuclei
energy:
i) The
tations
deformation
within
ii) The
AN
splitting
orbital
= 2, giving
angular
determined
The
strength
providing
interpretation
Lo Iudice
perform
The
collective
The
(Lo Iudice
collective
Neutrons
model
model
in deformed
and protons
oscillations
of Bohr
degrees
for spherical
nuclei
isovector
1+ mode
and Palumbo,
1978,
in deformed
1979),
(1975)
of freedom
was quantized
recently
Richter
1991,
1993,
1994).
(Richter,
1994).
They
by the two-rotor
in this collective
classically
model
vibrations
1994)
to
to the nuclear
is purely
by the
were
model of
(Nojarov,
were
et al., 1990;
to isovector
described
states
(1992,
was extended
nuclei,
a high-
et al., 1984a),
an axis perpendicular
and Mottelson
to isoscalar
nuclei
through
is still controversial.
are assumed
around
rule.
by Kneissl
Ml strength
mode predicted
with
nuclei.
extensive
values of these
(Frekers
nuclei
Their
(Bohle
reviewed
orbital
shells
in deformed
(1988).
Ml excitations
and B(M1)
reactions
major
in spherical
excitations
in Darmstadt
fluorescence,
exci-
elements.
= 0 spin selection
et al.
orbital
Energies
with (p,p)
rotational
on l+
of Nojarov
accelerator
1994).
different
do not exist
of the AN
of low-lying
resonance
excitations
between
which
information
on the high-energy
1979).
it was restricted
quantum
(1966).
Ml
(out-of-phase)
axis.
because
(1978,
1993,
recently
et al., 1984a,
and Palumbo
isovector
symmetry
mode,
(1991,
via nuclear
was studied
elements
the introduction
particle-hole
case, because
on the linear
also information
excitations,
in the latter
scattering
of Richter
(Bohle
Ml
the experimental
of the orbital
initially
L has matrix
orbital
see e. g.
1994),
identified
The
articles
j-shells
by large orbital
electron
spin Ml
1993,
The
started
inelastic
nuclei,
in the past,
study
resolution
momentum
are negligible
to spherical
characterized
rise to high-energy
of the spherical
such a
spurious.
by Faessler
two-rotor
model
in canonical
relative
variables.
Microscopic
calculations
rable interactions
of isovector
rotational
1990,
Faessler,
Qz,*r,
1993;
generating
It should
acter
only after
that
or a weakly
The
residual
rotations
the orbital
restoration
(e. g. De Coster
collective
interaction
around
QRPA
of the rotational
in terms of scissors
and Heyde,
Speth
and Zawischa,
Speth
the scissors
We are going
vibrations
1992).
random-phase
of the orbital
approximation
1+ excitations
scissors
mode
is constructed
an axis perpendicular
1+ excitations
invariance
acquire
(Nojarov
(QRPA)
in deformed
(Nojarov
using
nuclei
sepa-
in terms
and Faessler,
1988,
operators
to the nuclear
symmetry
axis.
a well-pronounced
scissors
char-
and Faessler,
1988)
violated
by the
The interpretation
Ml response
the quasiparticle
the interpretation
infinitesimal
be stressed
deformation
within
support
1988,
1991),
1989;
mode is supported
but rejected
Zawischa
of the collective
to present
motion
here
some
and Speth,
QRPA
related
by others
(e. g. Hamamoto
1990).
at high energy,
of our results
related
approaches
and Aberg,
1984,
1986;
In the above
works
of Zawischa
and
Etheor. % 22-24
MeV.
It represents
the
giant quadrupole
with
resonance
the electromagnetic
(IVGQR).
excitations
of
states
in deformed
manifestation
nuclei
of the scissors
and supporting
Our QRPA
pairing,
results
rotational
ORBITAL
STRENGTH
symmetry-restoring
with
quadrupole
invariance,
299
Ml
excitations
as
violated
EXCITATIONS
a deformed,
axially-symmetric
interactions
by the deformation
procedure
AND
DISTRIBUTION
are obtained
and separable
the interpretation
mode.
LOW-ENERGY
SPIN
Nuclei
(Nojarov
of the mean
and Faessler,
Woods-Saxon
(Faessler
field,
potential,
and Nojarov,
is restored
1990).
in RPA
BCS
The
using
1988).
1.5
1.0
0.5
0.0
1.0
N
-
0.5
3
0.0
15Gd
g1.0
a
0.5
0.0
lsaGd1
1.0
0.5
E(MeV)
Fig. 1.
Energy
1994).
distribution
are displayed
(circles
and Ziegler
as bars
et al.
in rare-earth
excitations
and compared
1990),
(1993).
is compared
to
and Richter
(1991,
(Sarriguren
et al.,
experimental
et al. (1992),
data
Margraf
spin Ml
et
strength
B(M1)
values of single l+
2 and 4 MeV.
They
to (7,-y)
The predominatly
as bars.
nuclei
Friedrichs
are plotted
lying between
QRPA
(circles)
strength
0.1 p$
al. (1993),
excitations
of Ml
300
R. Nojarov
The energy
distribution
and compared
5 and
10 MeV.
neutron
1994;
strong
nuclei
(Lipparini
isoscalar
from
inelastic
typical
et aI., 1993)
(Fig.
l),
some orbital
is deduced
peak
admixtures.
The latter
Fig. 2.
Ml
as noted
of almost
spectrum
(bars
same
spectrum
orbital)
general
squared
features
of 238U in Fig.
B(M1)
values
40%
FORM
Transverse
Ml
transition
l+ excitations.
ward inelastic
electron
Instead
of single
overlap
different
overlaps
FACTORS
densities
They
are obtained
scattering
(Heisenberg
by the small
shows
value
of the
in the introduction.
one contains
also
with B(Ml)>
in the bottom
region
between
energy
plot
0.1 &
with
(e, e)
with experiment.
Bars
in the top
deformed
nuclei,
strength
are plotted.
shown
as seen
alone,
As seen from
in more
detail
from
the
the total
Ml
(spin
in the bottom
plot,
state.
FOR INELASTIC
ELECTRON
microscopically
of spherical
spin strength
the isoscalar
excitations
excitations,
scissors
state.
up to 10 MeV
orbital
of
et
for comparison.
an enlarged
also in heavier
of histograms
excitations
low-lying
versus
the agreement
are manifested
2.
of Fig.
The energy
plot is displayed
to see better
QRPA
are compared
between
analysis
to the case
and mentioned
while
in the histograms,
of 23sU. Theoretical
isoscalar,
respect
damped
(1958)
The
plot in order
in this
spin excitations,
resides
qualitatively.
excitations
one is strongly
by Morpurgo
purely
experiments
QRPA
et al., 1988).
the isoscalar
factor,
is reproduced
is similar
in bins of 80 keV
Laszewski
because
is given by histograms
Most
structure
spin strength
1984;
consists
strength
scattering.
of the involved
that
The
and Richter,
spin gyromagnetic
isovector
elements
is isovector.
peaks
spin Ml
proton
double-bumped
spin matrix
Nojarov
peak
up in both
The
Its
and proton
al., 1993,
lying
of the calculated
to data
from
the corresponding
and Blok,
1983).
The
SCATTERING
the QRPA
DWBA
theoretical
wave functions
form factors
of
for back-
form factors
of the
Magnetic
0.5
00
3.
Transverse
165
The
QRPA
(1.h.s.
2.0
1.5
versus
momentum
(full curves)
total
orbdxsl
: /
! i
,1,,..1,,,.
4,,:
respectively.
301
---
05
of 48Ti in DWBA
the effective
form factors
plot)
Nuclei
Wl
WI
Ml form factors
0 =
in Deformed
10-e
1.0
q,,,
Fig.
Excitations
The
latter
experimental
form factor
data.
curves:
QRPA
angle
ct al., 1991).
at 3.78 MeV
with experimental
et al. (1990)
was predicted
Dot-dashed
(Nojarov
Ml excitations
are compared
from Guhr
15
transfer
of strong
plot)
I1
1
and Richter
before
the subsequently
the collective
contribution
data
(1990),
scissors
form
in the r.h.s.
plot,.
Fig.
Ml
4.
transition
QRPA
total
transition
vection
two strong
Ml
excitations
orbital
contribution
transfer.
density
current
in 48Ti,
The
(dot-dashed
(dot-dashed)
long-dashed)
high momentum
densities
excitation
curve
(1.h.s.
curves)
and magnetization
plot)
and the
et al. (1991).
The
con-
(neutrons:
short-dashed,
protons:
the experimental
data
contributions.
shown
state
(continuous
state
in Fig.
at 7.2 MeV
in the r.h.s.
3, agree
well with
is almost
purely
plot)
spin-flip
is very small.
transition,
Its QR.PA
form
even at
because
the
factor
was
302
R. Nojarov
predicted
The
before
transition
of Fig.
the corresponding
density
4 and compared
transition
densities
differences
currents
amplitudes
of the QRPA
factor
excitation.
are present
and transition
fact that
collective
the scissors
QRPA
excitations
Ml
plot,
(Nojarov
12
above similarity
should
Although
from
apart
the large
overlap
densities
density
to that
of the low-energy
orbital
orbital
in 232Th
at 3.3 MeV
nature
spin
form
is due to the
to the weakly
1993).
low-lying
orbital
curve
Ml
(continuous
transition
Ml
10
excitation
ob-
in the upper
plot,
curve
in the lower
densities:
continuous
of the scissors
also in heavier
(dot-dashed
in 54Sm
Scissors
be well pronounced
of 238U. Larger
more similar
et al., 1990).
will be relevant
3 and 4. This
of the strongest
at 2 MeV
is very similar
plot
the two
transition
its shape
as seen from
in lighter
in the r.h.s.
It is seen that
the scissors
et al., 1993),
Faessler
plot.
to each other,
be expected
3 is displayed
momentum.
and Faessler,
scales
Fig.
in the 1.h.s.
in QRPA:
Nojarov
density
transition
tained
available.
Fig. 5.
should
mode,
in lighter
density
became
MeV from
the different
This
contributions
transition
data
at 3.78
excitations
excitation
to the scissors
in the proton
has larger
experimental
of the Ml
nuclei,
mode,
that
excitations
the
have
Magnetic
a stronger
in Fig.
orbital
contribution
have larger
excitations
Faessler,
to the corresponding
arises
from
the
amplitudes,
because
density.
convection
of the strong
of rare-earth
of the strongest
transition
proton
factors
in Fig.
but
main
of the
6. They
exhibit
nuclei,
orbital)
Ml
shown
excitation
The
components
strongest
low-lying
orbital
again
contribution
scissors
scissors
transition
densities
a similar
shape,
to the QRPA
which is typical
Ml
data,
excitations
QRPA
(Nojarov
form factor
originates
lo-@1n
and
0.5
Fig. 6.
QRPA
(e, e) form
excitations
The comparison
factors
rotational
allows
1992).
and
factors
calculated
(Bohle
et al.,
et al., 1993)
Dot-dashed
form
factor
curve:
the scissor
curves:
and QRPA
the low-lying
or a weakly
the convection
collective
densities
wave functions,
Ml
current
scissors
mode
Ml transition
excitations
(Nojarov
curves:
low-lying
Ml
orbital
for 238U
Continuous
scissors
for a scattering
1984b).
[Im-I
in DWBA
(dots
QRPA
between
1.5
0.5
to experiment
154Sm
(Nojarov
et al., 1990).
us to interpret
vibrations
1988)
form factor
obtained
1.5
serf
Ml
et al.,
5.
curve
.\I
in Fig.
(dot-dashed
RlA
Pm-I
Theoretical
compared
part
are
are much
1.0
serf
densities
154Sm
form factors
Q,
0.0
in 238U and
Faessler,
and actinide
(low-lying
current.
collectivity.
two-quasiparticle
303
Nuclei
on the example
density
scissors
(orbital)
in Deformed
1993).
(e, e) form
larger,
the transition
displayed
The
This is confirmed
is very similar
The
character.
Excitations
and Faessler,
plot are
5.
densities,
in deformed
to the
Dashed
nuclei
1988,
as isovector
1990,
1993;
304
R.
Nojarov
energy
distributions
are displayed
quadrupole
et al.,
of Ml
as histograms
type with a ratio
1994b).
invariance.
The
latter
It influences
well determined
and E2 strengths
in Fig.
7.
r = -2
constant
mainly
for QRPA
They
are obtained
between
its isovector
is calculated
the low-energy
OF HIGH-ENERGY
excitations
and isoscalar
microscopically
strength
with
from a symmetry-restoring
coupling
from
1+ in rsoGd
interaction
constants
the condition
(E < 12 MeV)
of
(Nojarov
of rotational
relatively
10
15
20
25
30
energy [MeV]
Fig. 7.
Energy
distributions
two plots)
et al., 1994b).
gle schematic
Only
the K = fl
Ml
to the E2 strength
in E2 transitions
accompanying
of Fig.
7, is peaked
B(E2)
value agrees
top
neighbouring
B(E2;0+0
with
strength
O-30
(Bohr
isovector
distribution
strength
(above
exhausts
and Mottelson,
at 11 MeV
is plotted
17 MeV)
(lower
(Nojarov
Ml strength.
plot produces
a sin-
99.5%
17-25
from
S(E2;
is almost
purely
MeV.
1994).
as shaded
orbital.
whose
data
strength
quadrupole
(Van
is peaked
This
result
The
QRPA
7, because
is shown
resonance
in
(ISGQR),
B(E2;0+0
the corresponding
class.)
for K = l+ excitations
separately
giant
with
(IVGQR)
excitations,
with experimental
counterpart
1975),
are displayed
the Ml
on 154Sm (Richter,
data
MeV
only orbital
incorporating
of the isoscalar
The Ml strength
the orbital
K = 1 component
The
experimental
in the interval
component
The
nuclei.
+
recent
plot
MeV.
and Ml
strength.
seen
9-11
plot)
= l+ in 16Gd
(at 22 MeV),
The
in the
with K
of E2 (top
excitations
basis cut-off
excitation
contributions
we are interested
histograms)
of QRPA
Shaded
The quasiparticle
orbital
(contour
strengths
der Woude,
between
1987,
is in a qualitative
energy-weighted
classical
1991)
22 and 23 MeV
sum-rule
on
with
agreement
E2 strength
for the K = 1
= 5.76 e* bMeV.
is shown in the lower two plots of Fig. 7, where
histograms.
It follows
It is seen that
roughly
the energy
the high-energy
distribution
Ml
of the
Magnetic
IVGQR.
The
schematic
from
two-quasiparticle
QRPA
the middle
(Richter,
plot
1994).
The
same strength
plot.
isovector
iu relative
rotor
than
of the deformed
harmonic
within
t,he same
within
the collective
the whole
non-spurious
(Zawischa
the exist,ence
within
1993),
Ml
carrying
strength
the predictions
experimental
20 MeV
estimates
1979)
fragmentation
was quantized
mode
splits
shells
recently
in deformed
(Nojarov,
in the schematic
1994)
two-level
corresponding
that
the scissors
This
nuclei,
results
at both
basis
to trar-
AN = 2, respectively.
with
1994)
case
in the
at high energy.
components,
(Nojarov,
region
mode
strongly
It was
exhausts
supports
mode.
model
1990)
that
mode.
into account,
rotor
the collective
However,
Ml
model,
taking
model
additionally
This
result
elasticity
as well (Zawischa
is already
scissors
the nuclear
strength.
apart
hydrodynamical
after
a low-energy
of the orbital
of the isovector
a single,
above
Ml excitations
scissors
most
model
strength
recent
excitation
AN = 0 and between
rotor
plot to produce
and Speth,
of a low-energy
Speth,
resulting
isovector
of the scissors
with
of the considerable
1978,
as manifestation
between
scissors
shell with
orbital
in the bottom
v al ue of a single
The
oscillator
sitions
the interpretation
B(M1)
305
Nuclei
in agreement
and Palumbo,
variables.
shown
= 3.6 pk,
0.25 p L, because
(Lo Iudice
canonical
It incorporates
is distributed
The largest
plot is smaller
in Deformed
(at 22 MeV).
The
basis
excitation
Excitations
in agreement
nature
and
with
of the low-energy
model.
I,
I,,
I,,
--
I,,
Ml
I,
I I,
I,
I,
75
50
_
\
\
I
100
DWBA
(e, e)
excitation
electron
Ih
cross
energy
= l+l;
(Nojarov
dotted
The
Ml
sections
(0
165)
sections
curve:
for the
single
schematic
et al., 199413).
Dashed
E2 excitation
with 1K
curve:
Ml
= 2+1;
QRPA
versus
incident
excitation
continuous
with
curve:
of the schematic
QRPA
state
at 22 Mev from
the bottom
plot
8. It is seen that the two cross sections have a very similar shape, but
(0 = 165) the E2 cross section is about one order of magnitude
larger
than
Thus,
the Ml
the IVGQR
scattering.
transfer
(Nojarov
cross
section.
(0.4
that
et al.. 1994a;
Dir&elder
the E2 electroexcitation
orbital
Ml
substantial
strength
is dominant
could hardly
E2 contributions
are present
in the high-energy
be seen through
at intermediate
of low-energy
orbital
region
inelastic
Ml
of
electron
momentum
excitations
R.
306
Nojarov
CONCLUSIONS
We have studied
using
theoretically
a deformed
densities,
tions
experimental
clusions
data
about
from
resides
matrix
elements
with
orbital
admixtures,
small
isovector.
However,
strength
density
nuclei,
MeV)
Ml
contain
(actinide)
22-23
small.
apart
Accompanying
is separated
The
case
The comparison
allows
rotational
between
scissors
or a weakly collective
rotor
in relative
conjugate
that
the scissors
mode
These
nuclei,
at both
results
MeV)
variables
exhausts
strongly
almost
to the
better
caused
purely
the isoscalar
known
case
by the higher
orbital
(titanium)
excitations
is almost
purely
orbital,
It is strongly
peaked
fragmented
of low-lying
region
orbital
Ml
scissors
transferred
(E > 15 MeV)
Ml transition
support
the interpretation
as fragmentation
orbital
Ml
done.
as isovector
of the isovector
harmonic
oscillator
at both
Ml excitations
and manifestation
at
are
nuclei
quantization
strength
even
angle of 165.
have been
densities,
momenta,
in deformed
The canonical
in heavy
are expected
even at scattering
excitations
mode.
in the schematic
excitations
wave functions,
at
and
value.
at intermediate
orbital
(2-4
up to 150 MeV,
and QRPA
and
because
nuclei,
of the IVGQR.
In the high-energy
the low-lying
isoscalar,
wider,
The low-energy
us to interpret
energy.
(17-28
E2 contributions
energies
of neutron
similar
in lighter
scattering.
for incident
vibrations
regions.
with
con-
nuclei.
The analysis
peaks,
in deformed
distribution
region
to the following
splitting.
strength
to states
substantial
electron
is true at least
factors
Ml
and E2 excita-
is predominantly
is stronger,
is, therefore,
fragmentation
the energy
The experimental
in this
backward
strength
Ml
5 and 10 MeV.
shows up in both
in two energy
high-energy
E2 transitions
nuclei.
to receive
almost
spin
its stronger
no single excitation
deformed
The
leads
nuclei
Transition
with numerous
in deformed
of this strength
peak
spin strength
for Ml
The agreement
scattering
between
and actinide
in QRPA.
strengths
of the 1+ excitations
the higher-lying
nuclei.
MeV,
and proton
strength
of transition
in heavy nuclei
while
from
of single-particle
The orbital
photon
shows that
is very
of spherical
electron,
rare-earth
interactions
wave functions.
residual
distributions
inelastic
the nature
in titanium,
and separable
and energy
microscopically
and proton
Ml
potential
are calculated
Most
Woods-Saxon
shows
of the collective
scissors
mode.
The
results
author
presented
is expressing
de Guerra,
M. Dingfelder,
with A. Richter,
gratefully
P. Sarriguren,
U. Kneissl,
acknowledged.
P. 0.
N. Lo Iudice,
Thanks
in collaboration
A. Raduta,
with many
engagement:
F. G. Scholtz,
H.-J.
colleagues,
Amand
and M. Grigorescu.
Wortche,
to whom
Faessler,
Discussions
for providing
the
E. Moya
are
code.
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