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Shielding Radiation

Alphas,
p Betas, Gammas and Neutrons

7/05/2011 1
Contents
General
General

Shielding Alpha Emitters


Shielding Alpha Emitters

Shielding
Shi ldi B Beta
t PParticles
ti l
General
Beta Particle Range
Bremsstrahlung
Example Calculation

Shielding Positrons
Shielding Positrons 2
Contents
Shielding Gamma Rays
General
Basic Equation First Example Calculation
Basic Equation Second Example Calculation
Relaxation Length
Calculating the Required Shielding Thickness
Calculating the Required Shielding Thickness Example
Shielding Multiple Gamma Ray Energies
Shielding Multiple Gamma Ray Energies Example
Layered (Compound) Shielding
Layered (Compound) Shielding Example
Half Value Layers
3
Half Value layers Example
Contents
Shielding Neutrons continued
Multipurpose Materials for neutron Shields
Possible Neutron Shield Options
Neutron Shielding Calculations Fast Neutrons
Neutron Shielding Calculations Alpha-Beryllium Sources
Neutron Shielding Calculations

Gamma and Neutron Shields General


General
Radiation energy
Shielding Material
Shielding Material - Lead
4
Contents
Shielding Gamma Rays continued
Tenth Value layers
Buildup
Buildup Factor
Buildup Factor Example
Determining the Required shield Thickness with Buildup

Shielding Neutrons
The Three Steps
1. Slow the Neutrons
2. Absorb the Neutrons
3. Absorb the Gamma rays
5
Contents
Gamma and Neutron Shields General continued
Shielding Material Water
Shielding Material Concrete
Streaming
Streaming Door Design
Streaming Labyrinth
Shine

Appendices
Appendix A Densities of Common Materials
Appendix B How to do a Linear Interpolation
Appendix C Range and Energy of Beta particles
Appendix D Transmission Curves
6
Appendix F Buildup Factors
General

August 25, 2009 7


General
Shielding calculations done by hand are often ballpark
approximations

The most accurate shielding calculations are performed by


computers

Shi
Shields
ld are often
ft over-designed
d i d so that
th t th
they can h
handle
dl
more intense sources of radiation that might be used in the
future

The photon shielding calculations in this handout only


apply to monoenergetic photons (e.g., gamma rays).
Shielding x-rays, which have a continuous range of
energies, is a specialized topic not considered here
8
General
The required shield thickness depends on three things:

1. Radiation Energy. The greater the energy of the


radiation (e.g., beta particles, gamma rays, neutrons) the
thicker the shield must be.

2. The shield material. For photons (x-rays, gamma rays)


the lower the atomic number of the shield, the thicker it
must be. For neutrons, the general rule is that the lower
the hydrogen content, the thicker the shield must be.

3. Radiation intensity. The higher the radiation intensity,


and the more it must be reduced, the thicker the shield.
9
Shielding Alpha Emitters

August 25, 2009 10


Shielding Alpha Emitters

For external alpha emitting sources, the alpha particles


themselves are not a radiation hazard. However, we must
consider the possibility that other types of radiation might
be present. This possibility must always be considered
when shielding any type of radiation!

While we might assume that an alpha emitter doesnt emit


gamma rays, it might actually do so. Pu-239 for example
emits a large number of gamma rays. Nevertheless, we
often consider Pu-239 a pure alpha emitter because the
gamma intensity is low .

11
Shielding Alpha Emitters

Alpha emitters might also emit conversion electrons and


low energy x-rays.

Furthermore, alpha sources often contain trace quantities


of impurities some of which might emit beta particles.

These kinds of issues are primarily a concern when large


quantities of alpha emitters are handled, e.g., in glove
box facilities where curie and megacurie quantities might
be encountered.

12
Shielding Beta Particles

August 25, 2009 13


Shielding Beta Particles
General

The dose from an external source of beta particles is


primarily to the skin. The penetrating power of betas is low
- approximately a few mm in tissue.

Beta particles, like alpha particles, can be completely


stopped by a shield. It rarely requires more than 5- 10 mm
of material to do so.

The material the shield is made of is not very important in


terms of its ability to stop the beta particles.

14
Shielding Beta Particles
Beta Particle Range

Beta ranges are often expressed as a density thickness


which has units of g/cm2. These ranges can be
converted to centimeters as follows:

The easy way to estimate the range (in mg/cm2) of beta


particles is to obtain it from the graph on page 162 of the
PTP Radiological Health Handbook. The energy specified
on the graph is the maximum beta energy.

15
Shielding Beta Particles
Beta Particle Range

Several equations approximate the range of betas, i.e., the


thickness of the shield required to stop all the betas.

The equation below (Feather's Rule) applies to betas with


a maximum energy above 0.6 MeV:

Range (g/cm2) = 0.542 E 0.133

E is the maximum energy (MeV)

The following equation applies to betas with a maximum


energy below 0.8 MeV:

Range (g/cm2) = 0.407 E1.38 16


Shielding Beta Particles
Bremsstrahlung

While it is easy to completely stop beta particles, the very


act of doing so produces bremsstrahlung, a more
penetrating type of radiation. Shielding bremsstrahlung can
be more of a problem than shielding gammas.

A good
d shielding
hi ldi material
t i l ffor b
betas
t minimizes
i i i
bremsstrahlung i.e., low Z material such as plastic.

Like beta particles, bremsstrahlung photons have a range of


energies up to a maximum. The maximum energy of the
bremsstrahlung photons is the same as the maximum
energy of the betas. When shielding bremsstrahlung, we
can take the very conservative approach that all the
bremsstrahlung photons have this maximum energy. 17
Shielding Beta Particles
Example calculation
A 1 Ci P-32 source (50 mls aqueous) is in a polyethylene
bottle (0.93 g/cm3). The effective atomic numbers of the
solution and vial wall are assumed to be 7.5.

a. How thick should the vial be?

b. What is the exposure rate at 1 meter due to


bremsstrahlung?

18
Shielding Beta Particles
Example calculation
a. How thick should the vial be?

The maximum beta energy for P-32 is 1.71 MeV. From the
curve (p 162) in the PTP Radiological Health Handbook, the
maximum range of the P-32 betas is 800 mg/cm2 (0.8 g/cm2).

Essentially the same result is obtained using the equation:


Range (g/cm2) = 0.542 E 0.133
= 0.542 x 1.71 0.133
= 0.79 g/cm2

As such, the vial should be at least 0.86 cm thick ( 0.8 g/cm2


divided by 0.93 g/cm3).
19
Shielding Beta Particles
Example calculation

b. What is the exposure rate at 1 meter due to


bremsstrahlung?

The fraction of the beta energy released in the form of


bremsstrahlung g from interactions in the solution ((and to a
lesser extent in the vial wall) is calculated as follows:

20
Shielding Beta Particles
Example calculation
b. What is the exposure rate at 1 meter due to
bremsstrahlung? - continued

The beta energy emission rate from the 1 Ci P-32 source is:

= 3.7
3 7 x 1010 dps
d x 00.7
7MMeV
V per d
decay
= 2.59 x 1010 MeV/s

The bremsstrahlung energy emission rate is therefore:

= 0.0043 x 2.59 x 1010 MeV/s


= 1.11 x 108 MeV/s
21
Shielding Beta Particles
Example calculation
b. What is the exposure rate at 1 meter due to
bremsstrahlung? - continued

The energy fluence rate (R) through a 1 cm2 area at 1 meter


is:

22
Shielding Beta Particles
Example calculation

b. What is the exposure rate at 1 meter due to


bremsstrahlung? - continued

The dose rate to air is the energy fluence rate (MeV, cm-2, s-1)
times the mass energy absorption coefficient for air (cm2/g).

Absorbed dose rate = R x uen/D

Mass energy absorption coefficients apply to single photon


energies but bremsstrahlung photons have a range of
energies. A conservative assumption is that they all have an
energy of 1.71 MeV (the maximum energy for P-32).

The mass energy absorption coefficient for 1.71 MeV photons


23
in air is approximately 0.025 cm2/g.
Shielding Beta Particles
Example calculation
b. What is the exposure rate at 1 meter due to
bremsstrahlung? - continued

Absorbed dose rate = R x u/D


= 883 ((MeV cm-2 s-1) x 0.025 cm2/g
g
= 22.1 MeV g-1 s-1
= 22.1 x 106 eV g-1 s-1

Since one ion pair is produced for every 34 eV absorbed by


the air, the ion pair production rate is:
= 22.1 x 106 (eV, g-1, s-1) / 34 (eV/ion pair)
= 0.65 x 10 6 ion pairs per gram per second
24
Shielding Beta Particles
Example calculation
b. What is the exposure rate at 1 meter due to
bremsstrahlung? - continued

Since the charge produced in air for one member of each


ion pair is 1
1.6
6 x 10-19 C,
C the rate of charge production is :

= 0.65 x 10 6 (ion pairs g-1 s-1) x 1.6 x 10-19 C


= 1.23 x 10-13 C g-1 s-1
= 1.23 x 10-10 C kg-1 s-1
= 4.44 x 10-7 C kg-1 hr-1

25
Shielding Beta Particles
Example calculation
b. What is the exposure rate at 1 meter due to
bremsstrahlung? - continued

Finally, the answer:

Since 2.58 x 10-4 C/kg equals 1 roentgen, the exposure rate


in R/hr is

= 4.44 x 10-7 (C kg-1 hr-1)/2.58 x 10-4 (C/kg)

= 1.72 x 10-3 R/hr


26
Shielding Positrons

August 25, 2009 27


Shielding Positrons
In general, positron energies (and the bremsstrahlung they
produce) tend to be higher than beta energies. Even so, the
positrons themselves are easy to stop. It requires at most a
cm or so of plastic.

The most important positron emitter, F-18, emits positrons


th t are off ffairly
that i l llow energy: maximum
i 633
633.5
5 kkeV,
V average
249.8 keV.

What we dont want to forget is that each emitted positron


will produce two 511 keV annihilation photons that must be
shielded. These annihilation photons are not always
mentioned in tables of decay data.
28
Shielding Gamma Rays

August 25, 2009 29


Shielding Gamma Rays
General
X0 is the exposure rate in the absence of shielding.

X0
Source

30
Shielding Gamma Rays
General
We want an equation that gives the exposure rate (X) when
shielding of a given thickness (x) is present.

X
Source

x
d
31
Shielding Gamma Rays
Basic Equation

The following basic equation assumes a narrow beam of


radiation penetrating a thin shield (a situation referred to as
"good geometry").

X is the exposure rate with the shield in place (e.g., R/hr)


Xo is the exposure rate without the shield (e.g., R/hr)
x is the thickness of the shield (e.g., cm)
u is the linear attenuation coefficient (e.g., cm-1).

The linear attenuation coefficient (u) is the probability of any


type of interaction (PE, CS, PP) per unit path length. 32
Shielding Gamma Rays
Basic Equation

Listings of the linear attenuation coefficient (u) are hard to


find. However, listings of a related quantity, the mass
attenuation coefficient (u/D), are easy to find.

The classic
Th l i listing
li ti off mass attenuation
tt ti coefficients
ffi i t iis th
thatt off
Hubbell. Hubbells tables can be found in the PTP
Radiological Health Handbook beginning on page 90.

The mass attenuation coefficient (u/D) is the probability of an


interaction (PE, CS, PP) per unit density thickness. Its units
are cm2/g. In other words, u/D is the probability of
interactions per g/cm2 travelled by the photon.
33
Shielding Gamma Rays
Basic Equation

The value of the mass attenuation coefficient depends on the


shielding material and the energy of the photons.

Nevertheless, mass attenuation coefficients for different


materials are very similar. For example, the following table
li t some mass attenuation
lists tt ti coefficients
ffi i t ffor 1 M
MeV
V photons.
h t
Shield Material u/D (cm2/g)
water 0.0707
concrete 0.0637
air 0.0636
iron 0.0599

The mass attenuation coefficient is the linear attenuation


34
divided by the density of the material.
Shielding Gamma Rays
Basic Equation

When using the mass attenuation coefficient instead of the


linear attenuation coefficient, the basic shielding equation is:

/ is the mass attenuation coefficient (cm2/g)


is the density of the shielding material (g/cm3)

Note, the units in the exponent must cancel out:


cm2/g x g/cm3 x cm
35
Shielding Gamma Rays
Basic Equation First example calculation

The exposure rate at a particular point is 100 R/hr due to


1332 keV gamma rays from Co-60. What would be the
resulting exposure rate if a 1 cm lead shield were employed
between the source and the point?

Warning!
In this example, we will use the basic equation which
assumes we have good geometry, i.e., a narrow beam and
thin shield. As we will see later, in the real world we rarely
have good geometry and this equation would result in an
underestimate of the exposure rate.

36
Shielding Gamma Rays
Basic Equation First example calculation

u/ is approximately 0.057 cm2/g (I eyeballed this)

actual is assumed to be the same as the theoretical density,


11.35 g/cm3

37
Shielding Gamma Rays
Basic Equation Second example calculation

The exposure rate at a particular point is 100 R/hr due to 662


keV gamma rays from Cs-137. What would be the resulting
exposure rate if a 1 cm lead shield were employed?

u/
is approximately
pp y 0.11 cm2/g
g ((I eyeballed
y this))

38
Shielding Gamma Rays
Relaxation Length

The relaxation length is the thickness of a shielding material


that will reduce the intensity of the radiation to 1/e (37%) of
its original intensity.

Relaxation length (cm) = 1/u

u is the linear attenuation coefficient (cm-1)

39
Shielding Gamma Rays
Calculating the required shielding thickness

The preceding equation can be rewritten as follows so as to


calculate the shielding thickness (x) necessary to achieve the
desired reduction in the exposure rate:

40
Shielding Gamma Rays
Calculating the required shielding thickness - Example

What thickness of a lead shield would be required to reduce


the exposure rate due to Cs-137 from 100 R/hr to 1 R/hr?

41
Shielding Gamma Rays
Shielding multiple gamma ray energies

Since the mass attenuation coefficient (u/D) depends on the


energy of the photons, the preceding shielding calculations
only work if the exposure rate is due to a single gamma ray
energy.

This works fine for Cs-137 which has a single gamma ray.

How do we handle the situation where the exposure rate is


due to more than one gamma ray energy, e.g., the two
gamma rays of Co-60 at 1173 keV and 1332 keV?

42
Shielding Gamma Rays
Shielding multiple gamma ray energies

We could take a conservative approach and do the


calculation only using the highest of the gamma ray energies.
This overestimates the exposure rate and the required
shielding.

This approach might be reasonable for something like Co-60


where the two gamma rays are of similar energy and
contribute nearly equally to the exposure rate.

On the other hand, this approach could be a disaster for the


situation where the highest gamma ray energy contributes
only a little to the exposure rate (e.g., a high activity Am-241
source combined with a low activity Cs-137 source.) 43
Shielding Gamma Rays
Shielding multiple gamma ray energies

The correct approach is to determine the exposure rate for


each gamma ray energy. Then we determine the attenuation
of each gamma ray energy as an independent calculation.

Here is an example problem of how this can be done


done.

The exposure rate at a particular point is 100 R/hr due to the


1173 and 1332 keV Co-60 gamma rays. What would be the
resulting exposure rate if a 1 cm lead shield were employed
between the source and the point? Once again, we assume
good geometry, i.e., a narrow beam and thin shield.
44
Shielding Gamma Rays
Shielding multiple gamma ray energies - Example

The 100 R/hr is the sum of the 1173 keV gamma ray (X1173)
and 1332 keV gamma ray (X1332 ) exposure rates.

X1173 and
d X1332 can be
b d
determined
t i d ffrom th
their
i specific
ifi gamma
ray constants: '1173 and '1332

The specific gamma ray constant for Co-60 (1.3 R m2 hr-1 Ci-1 )
is the sum of the specific gamma ray constants for the 1173
and 1332 keV gamma rays:

45
Shielding Gamma Rays
Shielding multiple gamma ray energies - Example

The specific gamma ray constant for a given gamma ray


energy can be calculated with the equation:

' is the specific gamma ray constant in R hr-1 m2 Ci-1


E is the gamma ray energy in MeV,
I is the gamma ray intensity (abundance)
uen/p is the mass energy absorption coefficient

46
Shielding Gamma Rays
Shielding multiple gamma ray energies - Example

The specific gamma ray constants for the two gammas are:

47
Shielding Gamma Rays
Shielding multiple gamma ray energies - Example

48
Shielding Gamma Rays
Shielding multiple gamma ray energies - Example

First we calculate the effect of 1 cm of lead on the 47 R/hr


due to the 1173 keV photons. The mass attenuation
coefficient is estimated to be 0.0625 cm2/g

49
Shielding Gamma Rays
Shielding multiple gamma ray energies - Example

Second we calculate the effect of 1 cm of lead on the 53 R/hr


due to the 1332 keV photons. The mass attenuation
coefficient is estimated to be 0.057 cm2/g

50
Shielding Gamma Rays
Shielding multiple gamma ray energies - Example

Finally we add the exposure rates for the 1173 and 1332 keV
gamma rays:

As expected, the exposure rate (51 R/hr) is not much


different from what we calculated when we assumed the
exposure rate was only due to the 1332 keV gamma ray (52
R/hr).
51
Shielding Gamma Rays
Layered (compound) Shielding

It is often the case that the shielding material consists of


several layers

X
Source

x1 x2

52
Shielding Gamma Rays
Layered (compound) Shielding

X
Source

x1 x2

53
Shielding Gamma Rays
Layered (compound) Shielding Example

The exposure rate at a particular point is 100 R/hr due to 662


keV gamma rays. Estimate the resulting exposure rate if a
shield consisting of 1 cm of lead and 2 cm of iron were
employed between the source and the point? Assume
good
good geometry,
geometry ii.e.,
e a narrow beam and thin shield
shield.

u/ is approximately 0.11 cm2/g for lead


u/ is approximately 0.075 cm2/g for iron

for the lead is assumed to be the same as its


theoretical density of 11.35 g/cm3
for the iron is assumed to be the same as its
theoretical density of 7.86 g/cm3 54
Shielding Gamma Rays
Layered (compound) Shielding Example

55
Shielding Gamma Rays
Half Value Layers

Instead of using attenuation coefficients to perform shielding


calculations, we can use half (or tenth) value layers. A half
value layer is the thickness of material that reduces the
radiation intensity by one-half.

The following equation using HVL's looks very similar to the


radioactive decay equation:

56
Shielding Gamma Rays
Half Value Layers

A mathematically equivalent form of this equation is:

Half value and tenth value layers for some materials can be
found in PTPs Radiological Health Handbook on page 79.

Dont be surprised if you see slightly different values in the


literature for the half value layers of different nuclides, e.g.,
0.6 cm or 0.65 cm for Cs-137 in lead.

57
Shielding Gamma Rays
Half Value Layers

The following table gives an idea as to the approximate half


value layer thicknesses for several shielding materials.

Energy Approximate Half Value Layers in cm (TVL in parentheses)


(MeV) Uranium Tungsten
g Lead Iron Concrete Water
0.5 0.51 1.0 3.30 7.62
1.0 0.76 1.52 4.57 9.91
1.5 1.27 1.78 5.84 12.19
2.0 1.52 2.03 6.60 13.97
Ir-192 0.28 0.33 0.48 1.27 4.5
Cs-137 0.65 (2.16) 1.6 (5.3) 4.8 (15.7)
Co-60 0.69 0.79 1.2 (4.0) 2.1 (6.9) 6.2 (20.6)
Ra-226 1.66 (5.5) 2.2 (7.4) 6.9 (23.4) 58
Shielding Gamma Rays
Half Value Layers - Example

The exposure rate is 100 R/hr due to a Cs-137 source. What


would the exposure rate be if the source were shielded with 2
cm of lead?

59
Shielding Gamma Rays
Tenth Value Layers

In a similar manner, a tenth value layer (TVL) is defined as


that thickness which will reduce the radiation intensity to one-
tenth of its original value. The equations for using TVL's are
as follows:

60
Shielding Gamma Rays
Buildup

When the exposure rate at a given distance from a point


source is calculated using the standard equation, we assume
scattered radiation doesnt contribute to the exposure rate.
Only those gamma rays originally directed to the point of
interest contribute.
contribute

Source

X
61
Shielding Gamma Rays
Buildup

Similarly, the shielding equations considered so far


assume no contribution from radiation scattered by the
shield towards the point of interest. This is the so-called
good geometry only possible with a narrow (collimated
beam) and a thin shield.

Collimated X
Source Shield 62
Shielding Gamma Rays
Buildup

For a broad beam or thick shield situation like that below,


radiation scattered in the shield contributes to the exposure
rate. This is the real world (bad geometry). Scattering of
radiation towards the point of interest is referred to as
buildup.

Source X
Shield 63
Shielding Gamma Rays
Buildup

To account for buildup, we can


incorporate a fudge factor known as
the buildup factor into our equations.

Source X
Shield
64
Shielding Gamma Rays
Buildup Factor

The buildup factor is a unitless


number greater than 1.

The value we assign to the buildup factor depends on three


things:

Shield material
Energy of the photons
Value of the equations exponent (:/D) D x (i.e., :x)

Buildup factors can be found on page 88 of PTPs


Radiological Health Handbook.
65
Shielding Gamma Rays
Buildup Factor

The equations exponent, the product ux , is sometimes


referred to as the number of mean free paths.

The mean free path (mfp) is the average distance a photon


travels before an interaction takes place. It is the reciprocal
off the
th linear
li attenuation
tt ti coefficient
ffi i t (u).
( )

66
Shielding Gamma Rays
Buildup Factor - Example

The exposure rate at a particular point is 100 R/hr due to


1332 keV gamma rays. What would be the resulting
exposure rate if a 1 cm lead shield were employed between
the source and the point? Assume poor geometry, i.e., a
broad beam and thick shield.

u/ is approximately 0.057 cm2/g

actual is assumed to be 11.35 g/cm3

B is estimated to be 1.2, based on an energy of 1332, and


a value of 0.647 for ux (number of mean free paths)
67
Shielding Gamma Rays
Buildup Factor - Example

68
Shielding Gamma Rays
Determining the Required Shield Thickness with Buildup

The following equation gives the shield thickness (x)


necessary to reduce the exposure rate from X0 to X:

A problem with this equation is that the buildup factor (B)


depends on the thickness of the shield (x), which is exactly
what we are trying to determine.

In other words, we cant determine B before we know x. 69


Shielding Gamma Rays
Determining the Required Shield Thickness with Buildup

First approach - iteration

We could estimate B by guessing what x is likely to be.


Then we could plug B and x into the following equation, and
see how close we g
get to the required
q exposure
p rate X.

If X is too high, increase the shield thickness and redo the


calculation. Keep doing this until we find the shield thickness
that achieves the desired exposure rate. This approach is
referred to as iteration. An unsavory sledgehammer 70

approach to be sure, but it works.


Shielding Gamma Rays
Determining the Required Shield Thickness with Buildup

Second approach energy absorption coefficient

We could eliminate the buildup factor in our equations by


substituting the mass energy absorption coefficient (:en/D) for
the mass attenuation coefficient (:/D) . Then we use the
following equation for x:

71
Although not technically correct, this approach is simple .
Shielding Gamma Rays
Determining the Required Shield Thickness with Buildup

Third approach- computers

Swallow our pride and use a computer.

Computer
p calculations can p
produce very
y accurate results for
complicated shield and source geometries.

Computer modeling typically uses the Discrete Ordinates


Technique (DOT for short) or the Monte Carlo Technique.

The DOT is a numerical integration technique used to derive


solutions of the Boltzmann Transport equation in certain
simplified cases. 72
Shielding Gamma Rays
Determining the Required Shield Thickness with Buildup

Third approach - computers

The Monte Carlo method uses extensive data tables and a


random number generator to mathematically "track"
thousands of simulated emissions of radiation through a
shield.

Perhaps the best known shielding code is Microshield

73
Shielding Gamma Rays
Determining the Required Shield Thickness with Buildup

Fourth approach transmission curves

One way to determining the required shielding thickness (or


reduction in exposure rate due to a given shield thickness) is
to use a transmission curve that accounts for buildup.

Transmission curves are plots of transmission (X/Xo) versus


shield thickness for various radionuclides. Examples curves
are on page 82 of PTPs Radiological Health Handbook.

Alas, transmission graphs are only available for a limited


number of radionuclides and shield materials and therefore
have somewhat limited applicability. 74
Shielding Gamma Rays
Determining the Required Shield Thickness with Buildup

Fourth approach transmission curves example

What thickness of lead shielding is required to reduce the


exposure rate due to Co-60 from 100 R/hr to 22 mR/hr?

75
Shielding Gamma Rays
Determining the Required Shield Thickness with Buildup

Fourth approach transmission curves example

From the curve on page 83 of PTPs Radiological Health


Handbook, approximately 15 cm of lead correspond to a
transmission factor of 2.2 x 10-4

76
Shielding Neutrons

77
Neutron Shielding

The Three Steps

Shielding neutrons involves three steps:

1. Slow the neutrons

2. Absorb the neutrons

3. Absorb the gamma rays

78
Neutron Shielding
1. Slow the neutrons
Neutrons are slowed to thermal energies with
hydrogenous material: water, paraffin, plastic.

Water can evaporate or leak, paraffin is flammable and


plastic
l ti iis expensive.
i

To slow down very fast neutrons, iron or lead might be


used in front of the hydrogenous material.

79
Neutron Shielding
2. Absorb the neutrons
Hydrogenous materials are also very effective at
absorbing neutrons - the cross section for neutron
capture by H-1 is 0.33 barns.

Unfortunately, a difficult to shield 2.2


Unfortunately 2 2 MeV gamma ray is
emitted when H-1 absorbs a neutron.

Boron might be incorporated into the shield because it


has a large cross section for neutron absorption and only
emits a low energy capture gamma ray.

To slow down very fast neutrons, iron or lead might be


used in front of the hydrogenous material.
80
Neutron Shielding
3. Absorb the gamma rays

Gamma rays are produced in the neutron shield by


neutron (radiative) capture, inelastic scattering, and the
decay of activation products.

81
Neutron Shielding

Multipurpose Materials for Neutron Shields


Concrete, especially with barium mixed in, can slow and
absorb the neutrons, and shield the gamma rays.

Plastic with boron is also a g


good multipurpose
p p shielding
g
material.

82
Neutron Shielding
Possible Neutron Shield Options

Hydrogenous Gamma n
material shield

Combination material e.g.,


borated plastic or concrete
n
with barium

Hi Z moderator for fast


83
neutrons
Neutron Shielding
Neutron Shielding Calculations fast neutrons
Neutron shielding calculations are best done by computers.
Nevertheless, in some limited situations, it is possible to
employ a simplistic exponential equation similar to that used
for monoenergetic photons.

The following equation (Schaeffer 1973) describes the effect


of a given shielding material (e.g., steel) on fast neutron dose
rate. It only works if the there is at least 50 cm of water (or
equivalent hydrogenous material) behind the shield.

84
Neutron Shielding
Neutron Shielding Calculations fast neutrons

t H2O D

D is the dose rate with shield

D0 is the dose rate without shield


t is the shield thickness (e.g., cm)
ER is the neutron removal cross section (e.g., cm-1) 85
Neutron Shielding
Neutron Shielding Calculations
alpha-beryllium sources

The following equation (modified from one in from NBS


Handbook 63) describes the effect of shield thickness on
the neutron dose rate associated with a radioactive neutron
source (e.g., AmBe).

B is a buildup factor usually assumed to be 5

86
Neutron Shielding
Neutron Shielding Calculations
The following values for removal cross sections are from
NBS Handbook 63.
Removal Cross Section
Material
ER (cm-1)
water 0 103
0.103
iron 0.1576
ordinary concrete 0.0942
barytes concrete 0.0945
graphite 0.0785

For what it is worth, the removal cross section is


approximately 2/3 to 3/4 of the total cross section. 87
Neutron Shielding
Neutron Shielding Calculations
In neutron shielding calculations, we might also use the
mass attenuation coefficient symbolized ER/D

According to Schaeffer (1973), the mass attenuation


coefficient (ER/D) for fast neutrons can be approximated with
your choice of one of the following:

ER/D = 0.19 Z-0.743 cm2/g (Z 8)


= 0.125 Z-0.565 cm2/g (Z > 8)

ER/D = 0.206 A-1/3 Z-0.294 ~ 0.206 (A Z)-1/3

ER/D = 0.21 A-0.58 88


Neutron Shielding
Neutron Shielding Calculations

When the neutron mass attenuation coefficient (ER/D) is


employed instead of the neutron removal cross section, the
previous equation becomes:

89
Neutron Shielding
Neutron Shielding Calculations

Another simple approach that might be possible is to


employ the neutron transmission/attenuation curves of
Allen and Futterer which can be found beginning on page
12 of PTPs Radiological Health Handbook.

These graphs provide dose reduction factors for neutrons


of specified energies as a function of shield thickness. The
shield is indicated to be polyethylene, but the graphs
provide conversion factors for water, concrete and soil
(NTS).

90
Gamma and Neutron Shields -
General

91
Gamma and Neutron Shields - General
General

Consider the possible use of temporary shielding (mobile or


fixed) rather than, or in addition to, permanent shielding.

Consider the consequences of the shield becoming


contaminated or
or, if neutrons are present
present, activated
activated.

If permanent shielding is used, consider the cost and ease


associated with dismantling it this might be necessary
when the facility is decommissioned. Concrete shields are
sometimes built with an inner (closest to the source) layer
that is intended to be removed at the end of the facilitys life.

92
Gamma and Neutron Shields - General
General

If a source emits gamma rays at a variety of energies, the


high energy gamma rays sometimes determine the
shielding requirements. For example, even though the
1764 and 2204 keV gamma rays of radium sources
normally contribute very little to the exposure rate
rate, they
become the controlling radiation once the shield has
eliminated the more predominant low energy photons. The
HVL for Ra-226 is even larger than that for Co-60!

93
Gamma and Neutron Shields - General
General

Consider the possible use of local shielding inside shielded


vaults/areas not normally occupied. For example shields
might be installed inside accelerator vaults near those
accelerator components most prone to activation. This
reduces doses during maintenance when the area is
temporarily occupied.

94
Gamma and Neutron Shields - General
Radiation Energy

The lower the energy of the gamma rays or neutrons, the


easier it is to shield them (i.e., the thinner the shield needs
to be).

If a source emits gamma rays at a variety of energies, the


high energy gamma rays sometimes determine the
shielding requirements. For example, even though the
1764 and 2204 keV gamma rays of radium sources
normally contribute very little to the exposure rate, they
become the controlling radiation once the shield has
eliminated the more predominant low energy photons. The
HVL for Ra-226 is even larger than that for Co-60!
95
Gamma and Neutron Shields - General
Shielding Material

For gamma rays, the higher the atomic number of the shield
material, the greater the attenuation of the radiation.

For neutrons, the lower the atomic number of the shielding


material,
t i l th
the greater
t ththe attenuation
tt ti off the
th radiation.
di ti

For both radiations, the greater the density of the shield


material the greater the attenuation of the radiation. Even
though water and air have essentially the same effective
atomic number, water is a better shield because it is
denser.
96
Gamma and Neutron Shields - General
Shielding Material Lead
For attenuating photons
Advantages: C high atomic number (Z=82)
C moderately high density (11.34 g/cm3)
C easily machined and melted
C relatively inexpensive
Disadvantages:

lack of mechanical strength


chemical toxicity (some facilities require gloves for
handling) . Oxidized lead (white) is especially bad.
new lead can be naturally radioactive (Pb-210)
97
recycled lead is often contaminated
Gamma and Neutron Shields - General
Shielding Material Lead

Lead is available in a variety of forms including:

standard bricks (4 x 8 x 2 approx 25-30 lbs)


interlocking bricks
sheets (typically 1/64 to 1/8
1/8 thick),
thick) including lead
backed drywall board and plywood
tape
wire
pipe
shot for filling voids
wool for filling voids
98
Gamma and Neutron Shields - General
Shielding Material Lead

Leaded hardware/items of various types:

leaded louvers for vents


leaded hinges and handles for doors
lead covers for electrical switches and covers
lead-headed nails for installing lead sheets
lead plugs, caps for screw hole covers.
batten strips for joints and corners
lead glass for windows - it varies, but 4 mm of
typical lead glass is roughly equivalent to 1 mm of pure
lead
99
Gamma and Neutron Shields - General
Shielding Material Tungsten Alloys

For attenuating photons. Tungsten alloys can contain


iron, copper, cobalt and nickel.

Advantages: C tungstens high atomic number (Z=74)


C veryy high
g density
y ((ca. 14 - 18 g
g/cm3)
C strong
C non-toxic
C thinner shields possible than with lead

Disadvantages:

very difficult to machine and fabricate


expensive 100
Gamma and Neutron Shields - General
Shielding Material Depleted Uranium

For attenuating photons.

Advantages: C very high atomic number (Z= 92)


C very high density (19.1 g/cm3)
C good mechanical strength
C thinner shields possible than with lead

Disadvantages:

pyrophoric
expensive, but less so than tungsten
radioactive, hence there are regulatory issues with it
101
Gamma and Neutron Shields - General
Shielding Material Water

For attenuating photons and neutrons

Advantages:
completely fills all voids unlike a solid shield
transparent
p
can manipulate source and equipment in water
inexpensive
source leaks can be detected by sampling water

Disadvantages: C it can leak


C it can evaporate
C a leaking source can contaminate large
102
volumes of the water
Gamma and Neutron Shields - General
Shielding Material Concrete

For attenuating photons and neutrons

Advantages:

can also serve a structural role


can incorporate additives such as barium to improve
its characteristics
can be used to shield both neutrons and gamma rays

Disadvantages:

very thick walls can be needed


it can be difficult to modify and dismantle
103
Gamma and Neutron Shields - General
Streaming

Cracks or voids in the shield can allow narrow beams


radiation to stream through the shield.

Such openings in a shield might be unavoidable, e.g.,


d
doors, penetrations
t ti for
f piping,
i i d
ducts,
t cables
bl ,etc.
t
Whenever possible, such openings should be curved or
angled so as to prevent the radiation from having a
straight shot through the shield. Even so, some gamma
rays and especially neutrons can scatter their way through
these openings.

Quantifying such streaming is best done with a computer.


104
Gamma and Neutron Shields - General
Streaming

Penetrations in the shield should generally be at least


seven feet above the floor.

Consider filling any voids in such penetrations (e.g., with


lead shot).

Penetrations should not be directed toward occupied


areas or areas where there is traffic, e.g., stairways.

Determine if shields could be employed at ends of the


penetration.
105
Gamma and Neutron Shields - General
Streaming Door design

Neutron streaming can be harder to minimize than gamma


streaming.

Wall Wall
Wall Wall

Door
Door
Overlap Overlap

106
Gamma and Neutron Shields - General
Streaming Door design

It can be very difficult to prevent radiation from going


through the gap under a door.

Door

Scattered Radiation

Floor Insert
High atomic number inserts under a door can minimize
scattered gamma radiation. 107
Gamma and Neutron Shields - General
Streaming - Labyrinth

A labyrinth (aka maze) might be employed at the entrance to


a shielded area.

This labyrinth prevents a line of site view of the source


while allowing equipment and material to be moved in or out
with relative ease.

It avoids the need for complicated door designs like those


shown in the previous slides.

The general rule is that the radiation must scatter at least


twice to reach the entrance.
108
Gamma and Neutron Shields - General
Streaming - Labyrinth

SOURCE
LOCATION

Labyrinth/maze at
entrance to
minimize streaming
through door 109
Gamma and Neutron Shields - General
Shine

Shine is a term that usually refers to radiation that has


penetrated a weak spot in the shielding and scattered.
One such weak spot is often the ceiling.

Sk shine
Sky hi

Shield
Source Ground shine

110
Gamma and Neutron Shields - General
Shine

Radiation that goes over the shield and scatters in the air
towards the ground is known as sky shine.

Radiation that has gone through the floor and scattered


upwards in the ground is known as ground shine. The
latter is rarely a major concern.

The primary dose to the public near a nuclear facility (e.g.,


accelerator) is often due to sky shine. This is especially
true for neutrons.

111
Appendices

112

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